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Two-Qubit Geometric Gates Based on Ground-State Blockade of Rydberg Atoms
Ji-Ze Xu, Li-Na Sun, J.-F. Wei, Y.-L. Du, Ronghui Luo, Lei-Lei Yan, M. Feng, and Shi-Lei Su
Chin. Phys. Lett.    2022, 39 (9): 090301 .   DOI: 10.1088/0256-307X/39/9/090301
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We achieve the robust nonadiabatic holonomic two-qubit controlled gate in one step based on the ground-state blockade mechanism between two Rydberg atoms. By using the Rydberg-blockade effect and the Raman transition mechanism, we can produce the blockade effect of double occupation of the corresponding ground state, i.e., ground-state blockade, to encode the computational subspace into the ground state, thus effectively avoiding the spontaneous emission of the excited Rydberg state. On the other hand, the feature of geometric quantum computation independent of the evolutionary details makes the scheme robust to control errors. In this way, the controlled quantum gate constructed by our scheme not only greatly reduces the gate infidelity caused by spontaneous emission but is also robust to control errors.
Cobalt-Dimer Nitrides: A Potential Novel Family of High-Temperature Superconductors
Yuhao Gu, Kun Jiang, Xianxin Wu, and Jiangping Hu
Chin. Phys. Lett.    2022, 39 (9): 097401 .   DOI: 10.1088/0256-307X/39/9/097401
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We predict that the square lattice layer formed by [Co$_2$N$_2$]$^{2-}$ diamond-like units can host high-temperature superconductivity. The layer appears in the stable ternary cobalt nitride, BaCo$_2$N$_2$. The electronic physics of the material stems from Co$_2$N$_2$ layers where the dimerized Co pairs form a square lattice. The low energy physics near Fermi energy can be described by an effective two-orbital model. Without considering interlayer couplings, the two orbitals are effectively decoupled. This electronic structure satisfies the “gene” character proposed for unconventional high-temperature superconductors. We predict that the leading superconducting pairing instability is driven from an extended $s$-wave ($s^\pm$) to a $d$-wave by hole doping, e.g., in Ba$_{1-x}$K$_x$Co$_2$N$_2$. This study provides a new platform to establish the superconducting mechanism of unconventional high-temperature superconductivity.
Quantum Cloning of Steering
Dian Zhu, Wei-Min Shang, Fu-Lin Zhang, and Jing-Ling Chen
Chin. Phys. Lett.    2022, 39 (7): 070302 .   DOI: 10.1088/0256-307X/39/7/070302
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Quantum steering in a global state allows an observer to remotely steer a subsystem into different ensembles by performing different local measurements on the other part. We show that, in general, this property cannot be perfectly cloned by any joint operation between a steered subsystem and a third system. Perfect cloning is viable if and only if the initial state is of zero discord. We also investigate the process of cloning the steered qubit of a Bell state using a universal cloning machine. Einstein–Podolsky–Rosen (EPR) steering, which is a type of quantum correlation existing in the states without a local-hidden-state model, is observed in the two copy subsystems. This contradicts the conclusion of no-cloning of quantum steering (EPR steering) [C. Y. Chiu et al., npj Quantum Inf. 2, 16020 (2016)] based on a mutual information criterion for EPR steering.
Large Room-Temperature Magnetoresistance in van der Waals Ferromagnet/Semiconductor Junctions
Wenkai Zhu, Shihong Xie, Hailong Lin, Gaojie Zhang, Hao Wu, Tiangui Hu, Ziao Wang, Xiaomin Zhang, Jiahan Xu, Yujing Wang, Yuanhui Zheng, Faguang Yan, Jing Zhang, Lixia Zhao, Amalia Patanè, Jia Zhang, Haixin Chang, and Kaiyou Wang
Chin. Phys. Lett.    2022, 39 (12): 128501 .   DOI: 10.1088/0256-307X/39/12/128501
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A magnetic tunnel junction (MTJ) is the core component in memory technologies, such as the magnetic random-access memory, magnetic sensors and programmable logic devices. In particular, MTJs based on two-dimensional van der Waals (vdW) heterostructures offer unprecedented opportunities for low power consumption and miniaturization of spintronic devices. However, their operation at room temperature remains a challenge. Here, we report a large tunnel magnetoresistance (TMR) of up to 85% at room temperature ($T = 300$ K) in vdW MTJs based on a thin ($ < 10$ nm) semiconductor spacer WSe$_{2}$ layer embedded between two Fe$_{3}$GaTe$_{2}$ electrodes with intrinsic above-room-temperature ferromagnetism. The TMR in the MTJ increases with decreasing temperature up to 164% at $T = 10$ K. The demonstration of TMR in ultra-thin MTJs at room temperature opens a realistic and promising route for next-generation spintronic applications beyond the current state of the art.
A 700 W$\cdot$h$\cdot$kg$^{-1}$ Rechargeable Pouch Type Lithium Battery
Quan Li, Yang Yang, Xiqian Yu, and Hong Li
Chin. Phys. Lett.    2023, 40 (4): 048201 .   DOI: 10.1088/0256-307X/40/4/048201
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High-energy-density rechargeable lithium batteries are being pursued by researchers because of their revolutionary potential nature. Current advanced practical lithium-ion batteries have an energy density of around 300 W$\cdot$h$\cdot$kg$^{-1}$. Continuing to increase the energy density of batteries to a higher level could lead to a major explosion development in some fields, such as electric aviation. Here, we have manufactured practical pouch-type rechargeable lithium batteries with both a gravimetric energy density of 711.3 W$\cdot$h$\cdot$kg$^{-1}$ and a volumetric energy density of 1653.65 W$\cdot$h$\cdot$L$^{-1}$. This is achieved through the use of high-performance battery materials including high-capacity lithium-rich manganese-based cathode and thin lithium metal anode with high specific energy, combined with extremely advanced process technologies such as high-loading electrode preparation and lean electrolyte injection. In this battery material system, the structural stability of cathode material in a widened charge/discharge voltage range and the deposition/dissolution behavior of interfacial modified thin lithium electrode are studied.
Digital Simulation of Projective Non-Abelian Anyons with 68 Superconducting Qubits
Shibo Xu, Zheng-Zhi Sun, Ke Wang, Liang Xiang, Zehang Bao, Zitian Zhu, Fanhao Shen, Zixuan Song, Pengfei Zhang, Wenhui Ren, Xu Zhang, Hang Dong, Jinfeng Deng, Jiachen Chen, Yaozu Wu, Ziqi Tan, Yu Gao, Feitong Jin, Xuhao Zhu, Chuanyu Zhang, Ning Wang, Yiren Zou, Jiarun Zhong, Aosai Zhang, Weikang Li, Wenjie Jiang, Li-Wei Yu, Yunyan Yao, Zhen Wang, Hekang Li, Qiujiang Guo, Chao Song, H. Wang, and Dong-Ling Deng
Chin. Phys. Lett.    2023, 40 (6): 060301 .   DOI: 10.1088/0256-307X/40/6/060301
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Non-Abelian anyons are exotic quasiparticle excitations hosted by certain topological phases of matter. They break the fermion-boson dichotomy and obey non-Abelian braiding statistics: their interchanges yield unitary operations, rather than merely a phase factor, in a space spanned by topologically degenerate wavefunctions. They are the building blocks of topological quantum computing. However, experimental observation of non-Abelian anyons and their characterizing braiding statistics is notoriously challenging and has remained elusive hitherto, in spite of various theoretical proposals. Here, we report an experimental quantum digital simulation of projective non-Abelian anyons and their braiding statistics with up to 68 programmable superconducting qubits arranged on a two-dimensional lattice. By implementing the ground states of the toric-code model with twists through quantum circuits, we demonstrate that twists exchange electric and magnetic charges and behave as a particular type of non-Abelian anyons, i.e., the Ising anyons. In particular, we show experimentally that these twists follow the fusion rules and non-Abelian braiding statistics of the Ising type, and can be explored to encode topological logical qubits. Furthermore, we demonstrate how to implement both single- and two-qubit logic gates through applying a sequence of elementary Pauli gates on the underlying physical qubits. Our results demonstrate a versatile quantum digital approach for simulating non-Abelian anyons, offering a new lens into the study of such peculiar quasiparticles.
Coexistence of Quasi-two-dimensional Superconductivity and Tunable Kondo Lattice in a van der Waals Superconductor
Shiwei Shen, Tian Qin, Jingjing Gao, Chenhaoping Wen, Jinghui Wang, Wei Wang, Jun Li, Xuan Luo, Wenjian Lu, Yuping Sun, and Shichao Yan
Chin. Phys. Lett.    2022, 39 (7): 077401 .   DOI: 10.1088/0256-307X/39/7/077401
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Realization of Kondo lattice in superconducting van der Waals materials not only provides a unique opportunity for tuning the Kondo lattice behavior by electrical gating or intercalation, but also is helpful for further understanding the heavy fermion superconductivity. Here we report a low-temperature and vector-magnetic-field scanning tunneling microscopy and spectroscopy study on a superconducting compound (4Hb-TaS$_{2})$ with alternate stacking of 1T-TaS$_{2}$ and 1H-TaS$_{2}$ layers. We observe the quasi-two-dimensional superconductivity in the 1H-TaS$_{2}$ layer with anisotropic response to the in-plane and out-of-plane magnetic fields. In the 1T-TaS$_{2}$ layer, we detect the Kondo resonance peak that results from the Kondo screening of the unpaired electrons in the Star-of-David clusters. We also find that the intensity of the Kondo resonance peak is sensitive to its relative position with the Fermi level, and it can be significantly enhanced when it is further shifted towards the Fermi level by evaporating Pb atoms onto the 1T-TaS$_{2}$ surface. Our results not only are important for fully understanding the electronic properties of 4Hb-TaS$_{2}$, but also pave the way for creating tunable Kondo lattice in the superconducting van der Waals materials.
Optically Detected Magnetic Resonance of Diamond Nitrogen-Vacancy Centers under Megabar Pressures
Jian-Hong Dai, Yan-Xing Shang, Yong-Hong Yu, Yue Xu, Hui Yu, Fang Hong, Xiao-Hui Yu, Xin-Yu Pan, and Gang-Qin Liu
Chin. Phys. Lett.    2022, 39 (11): 117601 .   DOI: 10.1088/0256-307X/39/11/117601
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Megabar pressures are of crucial importance for cutting-edge studies of condensed matter physics and geophysics. With the development of diamond anvil cell (DAC), laboratory studies of high pressure have entered the megabar era for decades. However, it is still challenging to implement in situ magnetic sensing under ultrahigh pressures. In this work, we demonstrate optically detected magnetic resonance and coherent quantum control of diamond nitrogen-vacancy (NV) center, a promising quantum sensor inside the DAC, up to 1.4 Mbar. The pressure dependence of optical and spin properties of NV centers in diamond are quantified, and the evolution of an external magnetic field has been successfully tracked at about 80 GPa. These results shed new light on our understanding of diamond NV centers and pave the way for quantum sensing under extreme conditions.
Geometric Upper Critical Dimensions of the Ising Model
Sheng Fang, Zongzheng Zhou, and Youjin Deng
Chin. Phys. Lett.    2022, 39 (8): 080502 .   DOI: 10.1088/0256-307X/39/8/080502
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The upper critical dimension of the Ising model is known to be $d_{\rm c}=4$, above which critical behavior is regarded to be trivial. We hereby argue from extensive simulations that, in the random-cluster representation, the Ising model simultaneously exhibits two upper critical dimensions at $(d_{\rm c}=4,~d_{\rm p}=6)$, and critical clusters for $d \geq d_{\rm p}$, except the largest one, are governed by exponents from percolation universality. We predict a rich variety of geometric properties and then provide strong evidence in dimensions from 4 to 7 and on complete graphs. Our findings significantly advance the understanding of the Ising model, which is a fundamental system in many branches of physics.
Gatemon Qubit Based on a Thin InAs-Al Hybrid Nanowire
Jierong Huo, Zezhou Xia, Zonglin Li, Shan Zhang, Yuqing Wang, Dong Pan, Qichun Liu, Yulong Liu, Zhichuan Wang, Yichun Gao, Jianhua Zhao, Tiefu Li, Jianghua Ying, Runan Shang, and Hao Zhang
Chin. Phys. Lett.    2023, 40 (4): 047302 .   DOI: 10.1088/0256-307X/40/4/047302
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We study a gate-tunable superconducting qubit (gatemon) based on a thin InAs-Al hybrid nanowire. Using a gate voltage to control its Josephson energy, the gatemon can reach the strong coupling regime to a microwave cavity. In the dispersive regime, we extract the energy relaxation time $T_1\sim0.56$ µs and the dephasing time $T_2^* \sim0.38$ µs. Since thin InAs-Al nanowires can have fewer or single sub-band occupation and recent transport experiment shows the existence of nearly quantized zero-bias conductance peaks, our result holds relevancy for detecting Majorana zero modes in thin InAs-Al nanowires using circuit quantum electrodynamics.
Measuring Quantum Geometric Tensor of Non-Abelian System in Superconducting Circuits
Wen Zheng, Jianwen Xu, Zhuang Ma, Yong Li, Yuqian Dong, Yu Zhang, Xiaohan Wang, Guozhu Sun, Peiheng Wu, Jie Zhao, Shaoxiong Li, Dong Lan, Xinsheng Tan, and Yang Yu
Chin. Phys. Lett.    2022, 39 (10): 100202 .   DOI: 10.1088/0256-307X/39/10/100202
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Topology played an important role in physics research during the last few decades. In particular, the quantum geometric tensor that provides local information about topological properties has attracted much attention. It will reveal interesting topological properties but have not been measured in non-Abelian systems. Here, we use a four-qubit quantum system in superconducting circuits to construct a degenerate Hamiltonian with parametric modulation. By manipulating the Hamiltonian with periodic drivings, we simulate the Bernevig–Hughes–Zhang model and obtain the quantum geometric tensor from interference oscillation. In addition, we reveal its topological feature by extracting the topological invariant, demonstrating an effective protocol for quantum simulation of a non-Abelian system.
NMR Evidence for Universal Pseudogap Behavior in Quasi-Two-Dimensional FeSe-Based Superconductors
B. L. Kang, M. Z. Shi, D. Zhao, S. J. Li, J. Li, L. X. Zheng, D. W. Song, L. P. Nie, T. Wu, and X. H. Chen
Chin. Phys. Lett.    2022, 39 (12): 127401 .   DOI: 10.1088/0256-307X/39/12/127401
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Recently, by intercalating organic ions into bulk FeSe superconductors, two kinds of layered FeSe-based superconductors [(TBA)$_{x}$FeSe and (CTA)$_{x}$FeSe] with superconducting transition temperatures ($T_{\rm c}$) above 40 K have been discovered. Due to the large interlayer distance ($\sim $15 Å), these new layered superconductors have a large resistivity anisotropy analogous to bismuth-based cuprate superconductors. Moreover, remarkable pseudogap behavior well above $T_{\rm c}$ is revealed by nuclear magnetic resonance (NMR) measurements on $^{77}$Se nuclei, suggesting a preformed pairing scenario similar to that of cuprates. Here, we report another new kind of organic-ion-intercalated FeSe superconductor, (PY)$_{x}$FeSe, with a reduced interlayer distance ($\sim $10 Å) compared to (TBA)$_{x}$FeSe and (CTA)$_{x}$FeSe. By performing $^{77}$Se NMR and transport measurements, we observe a similar pseudogap behavior well above $T_{\rm c}$ of $\sim $40 K and a large resistivity anisotropy of $\sim$$10^{\boldsymbol{4}}$ in (PY)$_{x}$FeSe. All these facts strongly support a universal pseudogap behavior in these layered FeSe-based superconductors with quasi-two-dimensional electronic structures.
Lithium Ion Batteries Operated at $-100\,^{\circ}\!$C
Jianli Gai, Jirong Yang, Wei Yang, Quan Li, Xiaodong Wu, and Hong Li
Chin. Phys. Lett.    2023, 40 (8): 086101 .   DOI: 10.1088/0256-307X/40/8/086101
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Enabling lithium-ion batteries (LIBs) to operate in a wider temperature range, e.g., as low or high as possible or capable of both, is an urgent need and shared goal. Here we report, for the first time, a low-temperature electrolyte consisting of traditional ethylene carbonate, methyl acetate, butyronitrile solvents, and 1 M LiPF$_{6}$ salt, attributed to its very low freezing point ($T_{\rm f} = -126.3\,^{\circ}\!$C) and high ion conductivity at extremely low temperatures (0.21 mS/cm at $-100\,^{\circ}\!$C), successfully extends the service temperature of a practical 9.6 Ah LIB down to $-100\,^{\circ}\!$C (49.6% capacity retention compared to that at room temperature), which is the lowest temperature reported for practical cells so far as we know, and is lower than the lowest natural temperature ($-89.2\,^{\circ}\!$C) recorded on earth. Meanwhile, the high-temperature performance of lithium-ion batteries is not affected. The capacity retention is 88.2% and 83.4% after 800 cycles at 25$\,^{\circ}\!$C and 45$\,^{\circ}\!$C, respectively. The progress also makes LIB a proper power supplier for space vehicles in astronautic explorations.
Giant Tunneling Magnetoresistance in Spin-Filter Magnetic Tunnel Junctions Based on van der Waals A-Type Antiferromagnet CrSBr
Guibin Lan, Hongjun Xu, Yu Zhang, Chen Cheng, Bin He, Jiahui Li, Congli He, Caihua Wan, Jiafeng Feng, Hongxiang Wei, Jia Zhang, Xiufeng Han, and Guoqiang Yu
Chin. Phys. Lett.    2023, 40 (5): 058501 .   DOI: 10.1088/0256-307X/40/5/058501
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Two-dimensional van der Waals magnetic materials have demonstrated great potential for new-generation high-performance and versatile spintronic devices. Among them, magnetic tunnel junctions (MTJs) based on A-type antiferromagnets, such as CrI$_{3}$, possess record-high tunneling magnetoresistance (TMR) because of the spin filter effect of each insulating unit ferromagnetic layer. However, the relatively low working temperature and the instability of the chromium halides hinder applications of this system. Using a different technical scheme, we fabricated the MTJs based on an air-stable A-type antiferromagnet, CrSBr, and observed a giant TMR of up to 47000% at 5 K. Meanwhile, because of a relatively high Néel temperature of CrSBr, a sizable TMR of about 50% was observed at 130 K, which makes a big step towards spintronic devices at room temperature. Our results reveal the potential of realizing magnetic information storage in CrSBr-based spin-filter MTJs.
Strongly Lensed Transient Sources: A Review
Kai Liao, Marek Biesiada, and Zong-Hong Zhu
Chin. Phys. Lett.    2022, 39 (11): 119801 .   DOI: 10.1088/0256-307X/39/11/119801
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The past decades have witnessed a lot of progress in gravitational lensing with two main targets: stars and galaxies (with active galactic nuclei). The success is partially attributed to the continuous luminescence of these sources making the detection and monitoring relatively easy. With the running of ongoing and upcoming large facilities/surveys in various electromagnetic and gravitational-wave bands, the era of time-domain surveys would guarantee constant detection of strongly lensed explosive transient events, for example, supernovae in all types, gamma ray bursts with afterglows in all bands, fast radio bursts, and even gravitational waves. Lensed transients have many advantages over the traditional targets in studying the Universe, and magnification effect helps to understand the transients themselves at high redshifts. In this review article, on base of the recent achievements in literature, we summarize the methods of searching for different kinds of lensed transient signals, the latest results on detection and their applications in fundamental physics, astrophysics, and cosmology. At the same time, we give supplementary comments as well as prospects of this emerging research direction that may help readers who are interested in entering this field.
Spectroscopic Evidence for Electron Correlations in Epitaxial Bilayer Graphene with Interface-Reconstructed Superlattice Potentials
Chaofei Liu and Jian Wang
Chin. Phys. Lett.    2022, 39 (7): 077301 .   DOI: 10.1088/0256-307X/39/7/077301
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Superlattice potentials are theoretically predicted to modify the single-particle electronic structures. The resulting Coulomb-interaction-dominated low-energy physics would generate highly novel many-body phenomena. Here, by in situ tunneling spectroscopy, we show the signatures of superstructure-modulated correlated electron states in epitaxial bilayer graphene (BLG) on 6H-SiC(0001). As the carrier density is locally quasi-‘tuned’ by the superlattice potentials of a $6 \times 6$ interface reconstruction phase, the spectral-weight transfer occurs between the two broad peaks flanking the charge-neutral point. Such a detected non-rigid band shift beyond the single-particle band description implies the existence of correlation effects, probably attributed to the modified interlayer coupling in epitaxial BLG by the $6 \times 6$ reconstruction as in magic-angle BLG by the moiré potentials. Quantitative analysis suggests that the intrinsic interface reconstruction shows a high carrier tunability of $\sim $1/2 filling range, equivalent to the back gating by a voltage of $\sim $70 V in a typical gated BLG/SiO$_{2}$/Si device. The finding in interface-modulated epitaxial BLG with reconstruction phase extends the BLG platform with electron correlations beyond the magic-angle situation, and may stimulate further investigations on correlated states in graphene systems and other van der Waals materials.
Ferroelectricity in Charge-Ordering Crystals with Centrosymmetric Lattices
Yali Yang, Laurent Bellaiche, and Hongjun Xiang
Chin. Phys. Lett.    2022, 39 (9): 097701 .   DOI: 10.1088/0256-307X/39/9/097701
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The switchability between the two ferroelectric (FE) states of an FE material makes FEs widely used in memories and other electronic devices. However, for conventional FEs, its FE switching only occurs between the two FE states whose spatial inversion symmetry is broken. The search for FE materials is therefore subject to certain limitations. We propose a new type of FEs whose FE states still contain spatial inversion centers. The change in polarization of this new type of FEs originates from electronic transfer between two centrosymmetric FE states under an external electric field. Taking BaBiO$_{3}$ as an example, we show that charge-ordering systems can be a typical representative of this new type of FEs. Moreover, unlike traditional ferroelectrics, the change in polarization in this new type of FEs is quantum in nature with the direction dependent on the specific FE transition path. Our work therefore not only extends the concept of FEs but may also open up a new way to find multiferroics.
Dark Korteweg–De Vrise System and Its Higher-Dimensional Deformations
Si-Yu Zhu, De-Xing Kong, and Sen-Yue Lou
Chin. Phys. Lett.    2023, 40 (8): 080201 .   DOI: 10.1088/0256-307X/40/8/080201
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The new dimensional deformation approach is proposed to generate higher-dimensional analogues of integrable systems. An arbitrary ($K$+1)-dimensional integrable Korteweg–de Vries (KdV) system, as an example, exhibiting symmetry, is illustrated to arise from a reconstructed deformation procedure, starting with a general symmetry integrable (1+1)-dimensional dark KdV system and its conservation laws. Physically, the dark equation systems may be related to dark matter physics. To describe nonlinear physics, both linear and nonlinear dispersions should be considered. In the original lower-dimensional integrable systems, only liner or nonlinear dispersion is included. The deformation algorithm naturally makes the model also include the linear dispersion and nonlinear dispersion.
Optical Neural Network Architecture for Deep Learning with Temporal Synthetic Dimension
Bo Peng, Shuo Yan, Dali Cheng, Danying Yu, Zhanwei Liu, Vladislav V. Yakovlev, Luqi Yuan, and Xianfeng Chen
Chin. Phys. Lett.    2023, 40 (3): 034201 .   DOI: 10.1088/0256-307X/40/3/034201
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The physical concept of synthetic dimensions has recently been introduced into optics. The fundamental physics and applications are not yet fully understood, and this report explores an approach to optical neural networks using synthetic dimension in time domain, by theoretically proposing to utilize a single resonator network, where the arrival times of optical pulses are interconnected to construct a temporal synthetic dimension. The set of pulses in each roundtrip therefore provides the sites in each layer in the optical neural network, and can be linearly transformed with splitters and delay lines, including the phase modulators, when pulses circulate inside the network. Such linear transformation can be arbitrarily controlled by applied modulation phases, which serve as the building block of the neural network together with a nonlinear component for pulses. We validate the functionality of the proposed optical neural network for the deep learning purpose with examples handwritten digit recognition and optical pulse train distribution classification problems. This proof of principle computational work explores the new concept of developing a photonics-based machine learning in a single ring network using synthetic dimensions, which allows flexibility and easiness of reconfiguration with complex functionality in achieving desired optical tasks.
Pressure-Induced Color Change in the Lutetium Dihydride LuH$_{2}$
Pengfei Shan, Ningning Wang, Xiquan Zheng, Qingzheng Qiu, Yingying Peng, and Jinguang Cheng
Chin. Phys. Lett.    2023, 40 (4): 046101 .   DOI: 10.1088/0256-307X/40/4/046101
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The lutetium dihydride LuH$_{2}$ is stable at ambient conditions. Here we show that its color undergoes sequential changes from dark blue at ambient pressure to pink at $\sim$ $2.2$ GPa and then to bright red at $\sim$ $4$ GPa upon compression in a diamond anvil cell. Such a pressure-induced color change in LuH$_{2}$ is reversible and it is very similar to that recently reported in the N-doped lutetium hydride [Nature 615, 244 (2023)]. However, our preliminary resistance measurements on LuH$_{2}$ under pressures up to $\sim$ $7$ GPa evidenced no superconductivity down to 1.5 K.
Electron-Exciton Coupling in 1T-TiSe$_{2}$ Bilayer
Li Zhu, Wei-Min Zhao, Zhen-Yu Jia, Huiping Li, Xuedong Xie, Qi-Yuan Li, Qi-Wei Wang, Li-Guo Dou, Ju-Gang Hu, Yi Zhang, Wenguang Zhu, Shun-Li Yu, Jian-Xin Li, and Shao-Chun Li
Chin. Phys. Lett.    2023, 40 (5): 057101 .   DOI: 10.1088/0256-307X/40/5/057101
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Excitons in solid state are bosons generated by electron-hole pairs as the Coulomb screening is sufficiently reduced. The exciton condensation can result in exotic physics such as super-fluidity and insulating state. In charge density wave (CDW) state, 1T-TiSe$_{2}$ is one of the candidates that may host the exciton condensation. However, to envision its excitonic effect is still challenging, particularly at the two-dimensional limit, which is applicable to future devices. Here, we realize the epitaxial 1T-TiSe$_{2}$ bilayer, the two-dimensional limit for its $2 \times 2\times 2$ CDW order, to explore the exciton-associated effect. By means of high-resolution scanning tunneling spectroscopy and quasiparticle interference, we discover an unexpected state residing below the conduction band and right within the CDW gap region. As corroborated by our theoretical analysis, this mysterious phenomenon is in good agreement with the electron-exciton coupling. Our study provides a material platform to explore exciton-based electronics and opto-electronics.
Lu–H–N Phase Diagram from First-Principles Calculations
Fankai Xie, Tenglong Lu, Ze Yu, Yaxian Wang, Zongguo Wang, Sheng Meng, and Miao Liu
Chin. Phys. Lett.    2023, 40 (5): 057401 .   DOI: 10.1088/0256-307X/40/5/057401
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Employing a comprehensive structure search and high-throughput first-principles calculation method on 1561 compounds, the present study reveals the phase diagram of Lu–H–N. In detail, the formation energy landscape of Lu–H–N is derived and utilized to assess the thermodynamic stability of each compound that is created via element substitution. The result indicates that there is no stable ternary structure in the Lu–H–N chemical system, however, metastable ternary structures, such as Lu$_{20}$H$_{2}$N$_{17}$ $(C2/m)$ and Lu$_{2}$H$_{2}$N ($P\bar{3}m1$), are observed to have small $E_{\rm hull}$ ($ < 100$ meV/atom). It is also found that the energy convex hull of the Lu–H–N system shifts its shape when applying hydrostatic pressure up to 10 GPa, and the external pressure stabilizes a couple of binary phases such as LuN$_{9}$ and Lu$_{10}$H$_{21}$. Additionally, interstitial voids in LuH$_{2}$ are observed, which may explain the formation of Lu$_{10}$H$_{21}$ and LuH$_{3-\delta}$N$_{\epsilon}$. To provide a basis for comparison, x-ray diffraction patterns and electronic structures of some compounds are also presented.
Renormalization Group Theory of Eigen Microstates
Teng Liu, Gao-Ke Hu, Jia-Qi Dong, Jing-Fang Fan, Mao-Xin Liu, and Xiao-Song Chen
Chin. Phys. Lett.    2022, 39 (8): 080503 .   DOI: 10.1088/0256-307X/39/8/080503
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We propose a renormalization group (RG) theory of eigen microstates, which are introduced in the statistical ensemble composed of microstates obtained from experiments or computer simulations. A microstate in the ensemble can be considered as a linear superposition of eigen microstates with probability amplitudes equal to their eigenvalues. Under the renormalization of a factor $b$, the largest eigenvalue $\sigma_1$ has two trivial fixed points at low and high temperature limits and a critical fixed point with the RG relation $\sigma_1^b = b^{\beta/\nu} \sigma_1$, where $\beta$ and $\nu$ are the critical exponents of order parameter and correlation length, respectively. With the Ising model in different dimensions, it has been demonstrated that the RG theory of eigen microstates is able to identify the critical point and to predict critical exponents and the universality class. Our theory can be used in research of critical phenomena both in equilibrium and non-equilibrium systems without considering the Hamiltonian, which is the foundation of Wilson's RG theory and is absent for most complex systems.
Ultrafast Condensed Matter Physics at Attoseconds
Shi-Qi Hu and Sheng Meng
Chin. Phys. Lett.    2023, 40 (11): 117801 .   DOI: 10.1088/0256-307X/40/11/117801
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Our understanding of how photons couple to different degrees of freedom in solids forms the bedrock of ultrafast physics and materials sciences. In this review, the emergent ultrafast dynamics in condensed matter at the attosecond timescale have been intensively discussed. In particular, the focus is put on recent developments of attosecond dynamics of charge, exciton, and magnetism. New concepts and indispensable role of interactions among multiple degrees of freedom in solids are highlighted. Applications of attosecond electronic metrology and future prospects toward attosecond dynamics in condensed matter are further discussed. These pioneering studies promise future development of advanced attosecond science and technology such as attosecond lasers, laser medical engineering, and ultrafast electronic devices.
Continuously Doping Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+\delta}$ into Electron-Doped Superconductor by CaH$_{2}$ Annealing Method
Jin Zhao, Yu-Lin Gan, Guang Yang, Yi-Gui Zhong, Cen-Yao Tang, Fa-Zhi Yang, Giao Ngoc Phan, Qiang-Tao Sui, Zhong Liu, Gang Li, Xiang-Gang Qiu, Qing-Hua Zhang, Jie Shen, Tian Qian, Li Lu, Lei Yan, Gen-Da Gu, and Hong Ding
Chin. Phys. Lett.    2022, 39 (7): 077403 .   DOI: 10.1088/0256-307X/39/7/077403
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As a typical hole-doped cuprate superconductor, Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+\delta}$(Bi2212) carrier doping is mostly determined by its oxygen content. Traditional doping methods can regulate its doping level within the range of hole doping. Here we report the first application of CaH$_{2}$ annealing method in regulating the doping level of Bi2212. By continuously controlling the anneal time, a series of differently doped samples can be obtained. The combined experimental results of x-ray diffraction, scanning transmission electron microscopy, resistance and Hall measurements demonstrate that the CaH$_{2}$ induced topochemical reaction can effectively change the oxygen content of Bi2212 within a very wide range, even switching from hole doping to electron doping. We also found evidence of a low-$T_{\rm c}$ superconducting phase in the electron doping side.
Flat Band and $\mathbb{Z}_2$ Topology of Kagome Metal CsTi$_{3}$Bi$_{5}$
Yuan Wang, Yixuan Liu, Zhanyang Hao, Wenjing Cheng, Junze Deng, Yuxin Wang, Yuhao Gu, Xiao-Ming Ma, Hongtao Rong, Fayuan Zhang, Shu Guo, Chengcheng Zhang, Zhicheng Jiang, Yichen Yang, Wanling Liu, Qi Jiang, Zhengtai Liu, Mao Ye, Dawei Shen, Yi Liu, Shengtao Cui, Le Wang, Cai Liu, Junhao Lin, Ying Liu, Yongqing Cai, Jinlong Zhu, Chaoyu Chen, and Jia-Wei Mei
Chin. Phys. Lett.    2023, 40 (3): 037102 .   DOI: 10.1088/0256-307X/40/3/037102
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The simple kagome-lattice band structure possesses Dirac cones, flat band, and saddle point with van Hove singularities in the electronic density of states, facilitating the emergence of various electronic orders. Here we report a titanium-based kagome metal CsTi$_{3}$Bi$_{5}$ where titanium atoms form a kagome network, resembling its isostructural compound CsV$_{3}$Sb$_{5}$. Thermodynamic properties including the magnetization, resistance, and heat capacity reveal the conventional Fermi liquid behavior in the kagome metal CsTi$_{3}$Bi$_{5}$ and no signature of superconducting or charge density wave (CDW) transition anomaly down to 85 mK. Systematic angle-resolved photoemission spectroscopy measurements reveal multiple bands crossing the Fermi level, consistent with the first-principles calculations. The flat band formed by the destructive interference of hopping in the kagome lattice is observed directly. Compared to CsV$_{3}$Sb$_{5}$, the van Hove singularities are pushed far away above the Fermi level in CsTi$_{3}$Bi$_{5}$, in line with the absence of CDW. Furthermore, the first-principles calculations identify the nontrivial $\mathbb{Z}_2$ topological properties for those bands crossing the Fermi level, accompanied by several local band inversions. Our results suppose CsTi$_{3}$Bi$_{5}$ as a complementary platform to explore the superconductivity and nontrivial band topology.
Theory of Critical Phenomena with Memory
Shaolong Zeng, Sue Ping Szeto, and Fan Zhong
Chin. Phys. Lett.    2022, 39 (12): 120501 .   DOI: 10.1088/0256-307X/39/12/120501
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Memory is a ubiquitous characteristic of complex systems, and critical phenomena are one of the most intriguing phenomena in nature. Here, we propose an Ising model with memory, develop a corresponding theory of critical phenomena with memory for complex systems, and discover a series of surprising novel results. We show that a naive theory of a usual Hamiltonian with a direct inclusion of a power-law decaying long-range temporal interaction violates radically a hyperscaling law for all spatial dimensions even at and below the upper critical dimension. This entails both indispensable consideration of the Hamiltonian for dynamics, rather than the usual practice of just focusing on the corresponding dynamic Lagrangian alone, and transformations that result in a correct theory in which space and time are inextricably interwoven, leading to an effective spatial dimension that repairs the hyperscaling law. The theory gives rise to a set of novel mean-field critical exponents, which are different from the usual Landau ones, as well as new universality classes. These exponents are verified by numerical simulations of the Ising model with memory in two and three spatial dimensions.
A High-Randomness and High-Stability Electronic Quantum Random Number Generator without Post Processing
Yu-Xuan Liu, Ke-Xin Huang, Yu-Ming Bai, Zhe Yang, and Jun-Lin Li
Chin. Phys. Lett.    2023, 40 (7): 070303 .   DOI: 10.1088/0256-307X/40/7/070303
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Random numbers are one of the key foundations of cryptography. This work implements a discrete quantum random number generator (QRNG) based on the tunneling effect of electrons in an avalanche photo diode. Without any post-processing and conditioning, this QRNG can output raw sequences at a rate of 100 Mbps. Remarkably, the statistical min-entropy of the 8,000,000 bits sequence reaches 0.9944 bits/bit, and the min-entropy validated by NIST SP 800-90B reaches 0.9872 bits/bit. This metric is currently the highest value we have investigated for QRNG raw sequences. Moreover, this QRNG can continuously and stably output raw sequences with high randomness over extended periods. The system produced a continuous output of 1,174 Gbits raw sequence for a duration of 11,744 s, with every 8 Mbits forming a unit to obtain a statistical min-entropy distribution with an average value of 0.9892 bits/bit. The statistical min-entropy of all data (1,174 Gbits) achieves the value of 0.9951 bits/bit. This QRNG can produce high-quality raw sequences with good randomness and stability. It has the potential to meet the high demand in cryptography for random numbers with high quality.
Chiral Dirac Fermion in a Collinear Antiferromagnet
Ao Zhang, Ke Deng, Jieming Sheng, Pengfei Liu, Shiv Kumar, Kenya Shimada, Zhicheng Jiang, Zhengtai Liu, Dawei Shen, Jiayu Li, Jun Ren, Le Wang, Liang Zhou, Yoshihisa Ishikawa, Takashi Ohhara, Qiang Zhang, Garry McIntyre, Dehong Yu, Enke Liu, Liusuo Wu, Chaoyu Chen, and Qihang Liu
Chin. Phys. Lett.    2023, 40 (12): 126101 .   DOI: 10.1088/0256-307X/40/12/126101
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In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, it is predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral “Dirac-like” fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Such an unconventional chiral fermion, protected by a hidden $SU(2)$ symmetry in the hierarchy of an enhanced crystallographic group, namely spin space group, is not experimentally verified yet. Here, by angle-resolved photoemission spectroscopy measurements, we reveal the surface origin of the electron pocket at the Fermi surface in collinear antiferromagnet CoNb$_{3}$S$_{6}$. Combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions. Our work provides spectral evidence of the chiral Dirac-like fermion caused by particular spin symmetry in CoNb$_{3}$S$_{6}$, paving an avenue for exploring new emergent phenomena in antiferromagnets with unconventional quasiparticle excitations.
Dynamic Nonreciprocity with a Kerr Nonlinear Resonator
Rui-Kai Pan, Lei Tang, Keyu Xia, and Franco Nori
Chin. Phys. Lett.    2022, 39 (12): 124201 .   DOI: 10.1088/0256-307X/39/12/124201
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On-chip optical nonreciprocal devices are vital components for integrated photonic systems and scalable quantum information processing. Nonlinear optical isolators and circulators have attracted considerable attention because of their fundamental interest and their important advantages in integrated photonic circuits. However, optical nonreciprocal devices based on Kerr or Kerr-like nonlinearity are subject to dynamical reciprocity when the forward and backward signals coexist simultaneously in a nonlinear system. Here, we theoretically propose a method for realizing on-chip nonlinear isolators and circulators with dynamic nonreciprocity. Dynamic nonreciprocity is achieved via the chiral modulation on the resonance frequency due to coexisting self- and cross-Kerr nonlinearities in an optical ring resonator. This work showing dynamic nonreciprocity with a Kerr nonlinear resonator can be an essential step toward integrated optical isolation.