Chin. Phys. Lett.  2020, Vol. 37 Issue (1): 017401    DOI: 10.1088/0256-307X/37/1/017401
CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES |
Physical Properties of [$A_{6}$Cl][Fe$_{24}$Se$_{26}$]($A$=K, Rb) with Self-Similar Structure
Shaohua Wang, Qiangwei Yin, Hechang Lei**
Department of Physics and Beijing Key Laboratory of Opto-electronic Functional Materials $&$ Micro-nano Devices, Renmin University of China, Beijing 100872
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Shaohua Wang, Qiangwei Yin, Hechang Lei 2020 Chin. Phys. Lett. 37 017401
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Abstract We have successfully synthesized two novel compounds [$A_{6}$Cl][Fe$_{24}$Se$_{26}$] ($A$ = K, Rb). The key structural units of them are FeSe octamers, consisting of edge-shared FeSe$_{4}$ tetrahedra. Two kinds of FeSe octamer layers with different connection configurations stack along the $c$ axis, forming a three-dimensional (3D) TiAl$_{3}$-type structure. Interestingly, the 3D structural topology of these ocatmers in one unit cell is similar to the local atomic arrangement of themselves, i.e., self-similarity in structure. Physical property characterizations indicate that both the compounds exhibit insulating antiferromagnetism with Neel temperatures $T_{\rm N}\sim 110$ K and 75 K for [K$_{6}$Cl][Fe$_{24}$Se$_{26}$] and [Rb$_{6}$Cl][Fe$_{24}$Se$_{26}$].
Received: 13 September 2019      Published: 23 December 2019
PACS:  74.50.+r (Tunneling phenomena; Josephson effects)  
  75.20.Ck (Nonmetals)  
  75.30.-m (Intrinsic properties of magnetically ordered materials)  
  75.30.Cr (Saturation moments and magnetic susceptibilities)  
Fund: Supported by the National Key R&D Program of China under Grant No. 2016YFA0300504, the National Natural Science Foundation of China (Nos. 11574394, 11774423, 11822412), the Fundamental Research Funds for the Central Universities, and the Research Funds of Renmin University of China (RUC) (15XNLQ07, 18XNLG14, 19XNLG17).
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https://cpl.iphy.ac.cn/10.1088/0256-307X/37/1/017401       OR      https://cpl.iphy.ac.cn/Y2020/V37/I1/017401
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Shaohua Wang
Qiangwei Yin
Hechang Lei
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