Original Articles |
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Density Distributions of H and H2 in Pulsed Microwave Hydrogen Plasmas |
DUAN Xu-Ru1;H. Lange2;QIAN Shang-Jie1;N. Lang2 |
1Southwestern Institute of Physics, PO Box 432, Chengdu 610041
2Institute of Low Temperature Plasma Physics, Greifswald 17489, Germany |
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Cite this article: |
DUAN Xu-Ru, H. Lange, QIAN Shang-Jie et al 2003 Chin. Phys. Lett. 20 489-492 |
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Abstract Temporal distribution of the H atom and H2 densities in a pulsed microwave hydrogen plasmas has been measured simultaneously by two-photon absorption laser-induced fluorescence (TALIF). The measurement of the H-atom absolute density obtained by NO2 titration in a flow tube reactor shows that the density of H2 could be determined by the measured effective lifetime of the TALIF signal via the quenching equation. The H-atom density of about 1.5 x 1015cm-3 in both pulsed and stationary phases does not obviously change. It is found that the gas temperature volume effect plays an important role in governing the distributions of the H-atom density and it is mole fraction. The calculated gas temperature is in good consistent with the rotational temperature of H2 measured by optical emission spectroscopy in pulsed phase.
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Keywords:
52.70.-m
52.20.-j
31.70.Hq
32.50.+d
33.50.Dq
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Published: 01 April 2003
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PACS: |
52.70.-m
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(Plasma diagnostic techniques and instrumentation)
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52.20.-j
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(Elementary processes in plasmas)
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31.70.Hq
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(Time-dependent phenomena: excitation and relaxation processes, and reaction rates)
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32.50.+d
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(Fluorescence, phosphorescence (including quenching))
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33.50.Dq
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(Fluorescence and phosphorescence spectra)
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