Chin. Phys. Lett.  2024, Vol. 41 Issue (11): 117505    DOI: 10.1088/0256-307X/41/11/117505
CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES |
Rare-Earth Chalcogenides: An Inspiring Playground for Exploring Frustrated Magnetism
Mingtai Xie1,2, Weizhen Zhuo1,2, Yanzhen Cai1,2, Zheng Zhang2*, and Qingming Zhang1,2*
1School of Physical Science and Technology, Lanzhou University, Lanzhou 730000, China
2Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China
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Mingtai Xie, Weizhen Zhuo, Yanzhen Cai et al  2024 Chin. Phys. Lett. 41 117505
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Abstract The rare-earth chalcogenide $ARECh_{2}$ family ($A$ = alkali metal or monovalent ions, $RE$ = rare earth, $Ch$ = chalcogen) has emerged as a paradigmatic platform for studying frustrated magnetism on a triangular lattice. The family members exhibit a variety of ground states, from quantum spin liquid to exotic ordered phases, providing fascinating insight into quantum magnetism. Their simple crystal structure and chemical tunability enable systematic exploration of competing interactions in quantum magnets. Recent neutron scattering and thermodynamic studies have revealed rich phase diagrams and unusual excitations, refining theoretical models of frustrated systems. This review provides a succinct introduction to $ARECh_{2}$ research. It summarizes key findings on crystal structures, single-ion physics, magnetic Hamiltonians, ground states, and low-energy excitations. By highlighting current developments and open questions, we aim to catalyze further exploration and deeper physical understanding on this frontier of quantum magnetism.
Received: 26 September 2024      Review Published: 25 November 2024
PACS:  75.10.Jm (Quantized spin models, including quantum spin frustration)  
  75.10.Kt (Quantum spin liquids, valence bond phases and related phenomena)  
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Mingtai Xie
Weizhen Zhuo
Yanzhen Cai
Zheng Zhang
and Qingming Zhang
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