| CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES |
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Magnetism Measurements of Two-Dimensional van der Waals Antiferromagnet CrPS$_{4}$ Using Dynamic Cantilever Magnetometry |
| Qi Li1,2, Weili Zhen1, Ning Wang1, Meng Shi1,2, Yang Yu3, Senyang Pan1,2, Lin Deng1,2, Jiaqiang Cai1,2, Kang Wang1*, Lvkuan Zou4*, Zhongming Zeng4, Zhaosheng Wang1, and Jinglei Zhang1* |
1Anhui Province Key Laboratory of Condensed Matter Physics at Extreme Conditions, High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences, Hefei 230031, China
2Science Island Branch of Graduate School, University of Science and Technology of China, Hefei 230026, China
3School of Advanced Manufacturing Engineering, Hefei University, Hefei 230601, China
4Suzhou Institute of Nano-tech and Nano-bionics, Chinese Academy of Sciences, Suzhou 215123, China
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| Cite this article: |
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Qi Li, Weili Zhen, Ning Wang et al 2024 Chin. Phys. Lett. 41 107503 |
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Abstract Recent experimental and theoretical work has focused on two-dimensional van der Waals (2D vdW) magnets due to their potential applications in sensing and spintronics devises. In measurements of these emerging materials, conventional magnetometry often encounters challenges in characterizing the magnetic properties of small-sized vdW materials, especially for antiferromagnets with nearly compensated magnetic moments. Here, we investigate the magnetism of 2D antiferromagnet CrPS$_{4}$ with a thickness of 8 nm by using dynamic cantilever magnetometry (DCM). Through a combination of DCM experiment and the calculation based on a Stoner–Wohlfarth-type model, we unravel the magnetization states in 2D CrPS$_{4}$ antiferromagnet. In the case of $H\parallel c$, a two-stage phase transition is observed. For $H\perp c$, a hump in the effective magnetic restoring force is noted, which implies the presence of spin reorientation as temperature increases. These results demonstrate the benefits of DCM for studying magnetism of 2D magnets.
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Received: 02 September 2024
Published: 29 September 2024
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| PACS: |
75.70.Ak
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(Magnetic properties of monolayers and thin films)
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07.10.Cm
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(Micromechanical devices and systems)
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75.30.Kz
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(Magnetic phase boundaries (including classical and quantum magnetic transitions, metamagnetism, etc.))
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75.50.Ee
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(Antiferromagnetics)
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