Chin. Phys. Lett.  2024, Vol. 41 Issue (10): 107502    DOI: 10.1088/0256-307X/41/10/107502
CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES |
Centimeter-Scale Above-Room-Temperature Ferromagnetic Fe$_{3}$GaTe$_{2}$ Thin Films by Molecular Beam Epitaxy
Taikun Wang1,2†, Yongkang Xu1,2†, Yu Liu1,2, Xingze Dai1,2, Pengfei Yan1,2, Jin Wang1,2, Shuanghai Wang1,2, Yafeng Deng1,2, Kun He1,2, Caitao Li1,2, Ziang Wang1, Wenqin Zou3, Rongji Wen4, Yufeng Hao4, and Liang He1,2*
1School of Electronic Science and Engineering, Nanjing University, Nanjing 210000, China
2National Key Laboratory of Spintronics, Nanjing University, Suzhou 215163, China
3Department of Physics, Nanjing University, Nanjing 210000, China
4College of Engineering and Applied Science, Nanjing University, Nanjing 210000, China
Cite this article:   
Taikun Wang, Yongkang Xu, Yu Liu et al  2024 Chin. Phys. Lett. 41 107502
Download: PDF(2142KB)   PDF(mobile)(2162KB)   HTML
Export: BibTeX | EndNote | Reference Manager | ProCite | RefWorks
Abstract Fe$_{3}$GaTe$_{2}$, as a layered ferromagnetic material, has a Curie temperature ($T_{\rm c}$) higher than room temperature, making it the key material in next-generation spintronic devices. To be used in practical devices, large-sized high-quality Fe$_{3}$GaTe$_{2}$ thin films need to be prepared. Here, the centimeter-scale thin film samples with high crystal quality and above-room-temperature ferromagnetism with strong perpendicular magnetic anisotropy were prepared by molecular beam epitaxy technology. Furthermore, the $T_{\rm c}$ of the samples raises as the film thickness increases, and reaches 367 K when the film thickness is 60 nm. This study provides material foundations for the new generation of van der Waals spintronic devices and paves the way for the commercial application of Fe$_{3}$GaTe$_{2}$.
Received: 22 July 2024      Editors' Suggestion Published: 18 October 2024
PACS:  75.50.-y (Studies of specific magnetic materials)  
  75.50.Gg (Ferrimagnetics)  
  75.70.-i (Magnetic properties of thin films, surfaces, and interfaces)  
  75.47.-m (Magnetotransport phenomena; materials for magnetotransport)  
TRENDMD:   
URL:  
https://cpl.iphy.ac.cn/10.1088/0256-307X/41/10/107502       OR      https://cpl.iphy.ac.cn/Y2024/V41/I10/107502
Service
E-mail this article
E-mail Alert
RSS
Articles by authors
Taikun Wang
Yongkang Xu
Yu Liu
Xingze Dai
Pengfei Yan
Jin Wang
Shuanghai Wang
Yafeng Deng
Kun He
Caitao Li
Ziang Wang
Wenqin Zou
Rongji Wen
Yufeng Hao
and Liang He
[1] Guan M, Wang L, Zhao S, Zhou Z, Dong G, Su W, Min T, Ma J, Hu Z, Ren W, Ye Z G, Nan C W, and Liu M 2018 Adv. Mater. 30 1802902
[2] Jin W, Zhang G J, Wu H, Yang L, Zhang W F, and Chang H X 2023 Chin. Phys. Lett. 40 057301
[3] Kim S K, Beach G S D, Lee K J, Ono T, Rasing T, and Yang H 2022 Nat. Mater. 21 24
[4] Wu Y, Wang W, Pan L, and Wang K L 2022 Adv. Mater. 34 2105266
[5] Zhang Y Y, Ren X L, Liu R Z, Chen Z H, Wu X Z, Pang J, Wang W, Lan G B, Watanabe K, Taniguchi T, Shi Y G, Yu G Q, and Shao Q M 2024 arXiv:2405.06250 [cond-mat.mes-hall]
[6] Guo Y, Liu N S, Zhao Y Y, Jiang X, Zhou S, and Zhao J J 2020 Chin. Phys. Lett. 37 107506
[7] Sivadas N, Okamoto S, Xu X D, Fennie C J, and Xiao D 2018 Nano Lett. 18 7658
[8] Zhang P Y, Chung T F, Li Q W, Wang S Q, Wang Q J, Huey W L B, Yang S, Goldberger J E, Yao J, and Zhang X 2022 Nat. Mater. 21 1373
[9] Gupta V, Cham T M, Stiehl G M, Bose A, Mittelstaedt J A, Kang K F, Jiang S W, Mak K F, Shan J, Buhrman R A, and Ralph D C 2020 Nano Lett. 20 7482
[10] Hao Z Q, Li H W, Zhang S H, Li X T, Lin G T, Luo X, Sun Y P, Liu Z, and Wang Y Y 2018 Sci. Bull. 63 825
[11] Zhu W X, Song C, Han L, Guo T W, Bai H, and Pan F 2022 Nat. Commun. 13 6428
[12] Chen X H, Wang H T, Liu H J, Wang C, Wei G S, Fang C, Wang H C, Geng C Y, Liu S J, Li P Y, Yu H M, Zhao W S, Miao J G, Li Y T, Wang L, Nie T X, Zhao J M, and Wu X J 2022 Adv. Mater. 34 2106172
[13] Deng Y J, Yu Y J, Song Y C, Zhang J Z, Wang N Z, Sun Z Y, Yi Y F, Wu Y Z, Wu S W, Zhu J Y, Wang J, Chen X H, and Zhang Y B 2018 Nature 563 94
[14] Feng H L, Li Y, Shi Y G, Xie H Y, Li Y Q, and Xu Y 2022 Chin. Phys. Lett. 39 077501
[15] Liu X Q, Huang P Y, Xia Y, Gao L, Liao L Y, Cui B S, Backes D, van der Laan G, Hesjedal T, Ji Y C, Chen P, Zhang Y F, Wu F, Wang M X, Zhang J W, Yu G Q, Song C, Chen Y L, Liu Z K, Yang Y M, Peng Y, Li G, Yao Q, and Kou X F 2023 Adv. Funct. Mater. 33 2304454
[16] Xian J J, Wang C, Nie J H, Li R, Han M J, Lin J H, Zhang W H, Liu Z Y, Zhang Z M, Miao M P, Yi Y F, Wu S W, Chen X D, Han J B, Xia Z C, Ji W, and Fu Y S 2022 Nat. Commun. 13 257
[17] Zhang X Q, Lu Q S, Liu W Q, Niu W, Sun J B, Cook J, Vaninger M, Miceli P F, Singh D J, Lian S W, Chang T R, He X Q, Du J, He L, Zhang R, Bian G, and Xu Y B 2021 Nat. Commun. 12 2492
[18] Zhang G J, Guo F, Wu H, Wen X K, Yang L, Jin W, Zhang W F, and Chang H X 2022 Nat. Commun. 13 5067
[19] Kajale S N, Nguyen T, Chao C A, Bono D C, Boonkird A, Li M D, and Sarkar D 2024 Nat. Commun. 15 1485
[20] Pan Z C, Li D, Ye X G, Chen Z, Chen Z H, Wang A Q, Tian M L, Yao G J, Liu K H, and Liao Z M 2023 Sci. Bull. 68 2743
[21] Zha H M, Li W, Zhang G J, Liu W J, Deng L W, Jiang Q, Ye M, Wu H, Chang H X, and Qiao S 2023 Chin. Phys. Lett. 40 087501
[22] Zhu W K, Xie S H, Lin H L, Zhang G J, Wu H, Hu T G, Wang Z A, Zhang X M, Xu J H, Wang Y J, Zheng Y H, Yan F G, Zhang J, Zhao L X, Patané A, Zhang J, Chang H X, and Wang K Y 2022 Chin. Phys. Lett. 39 128501
Related articles from Frontiers Journals
[1] Ming-Shuang Li, Hui-Min Li, and Song Liu. Synthesis Methods and Property Control of Two-Dimensional Magnetic Materials[J]. Chin. Phys. Lett., 2024, 41(2): 107502
[2] Jia Luo, Jia-Hao Guo, Yun-He Hou, Jun-Lin Wang, Yong-Bing Xu, Yan Zhou, Philip Wing Tat Pong, and Guo-Ping Zhao. Manipulating Skyrmion Motion on a Nanotrack with Varied Material Parameters and Tilted Spin Currents[J]. Chin. Phys. Lett., 2023, 40(9): 107502
[3] Heming Zha, Wei Li, Gaojie Zhang, Wenjing Liu, Liwei Deng, Qi Jiang, Mao Ye, Hao Wu, Haixin Chang, and Shan Qiao. Enhanced Magnetic Interaction between Ga and Fe in Two-Dimensional van der Waals Ferromagnetic Crystal Fe$_{3}$GaTe$_{2}$[J]. Chin. Phys. Lett., 2023, 40(8): 107502
[4] Jing-Yang You, Xue-Juan Dong, Bo Gu, and Gang Su. Possible Room-Temperature Ferromagnetic Semiconductors[J]. Chin. Phys. Lett., 2023, 40(6): 107502
[5] Xiao-Yan Wang, Jun-Fa Lin, Xiang-Yu Zeng, Huan Wang, Xiao-Ping Ma, Yi-Ting Wang, Kun Han, and Tian-Long Xia. Multiple Magnetic Phase Transitions and Critical Behavior in Single-Crystal SmMn$_{2}$Ge$_{2}$[J]. Chin. Phys. Lett., 2023, 40(6): 107502
[6] Wenkai Zhu, Shihong Xie, Hailong Lin, Gaojie Zhang, Hao Wu, Tiangui Hu, Ziao Wang, Xiaomin Zhang, Jiahan Xu, Yujing Wang, Yuanhui Zheng, Faguang Yan, Jing Zhang, Lixia Zhao, Amalia Patanè, Jia Zhang, Haixin Chang, and Kaiyou Wang. Large Room-Temperature Magnetoresistance in van der Waals Ferromagnet/Semiconductor Junctions[J]. Chin. Phys. Lett., 2022, 39(12): 107502
[7] Lin Feng, Chen-Chen Guo, Xue-Ying Zhang, Hai-Cheng Xuan, Wen-Hong Wang, En-Ke Liu, Guang-Heng Wu. Possible Martensitic Transformation in Heusler Alloy Pt$_{2}$MnSn from First Principles[J]. Chin. Phys. Lett., 2018, 35(3): 107502
[8] KUMAR V., SINHA Anita, SINGH B. P., SINHA A. P., JHA V.. Refractive Index and Electronic Polarizability of Ternary Chalcopyrite Semiconductors[J]. Chin. Phys. Lett., 2015, 32(12): 107502
[9] SI Ping-Zhan, XIAO Xiao-Fei, FENG He, YU Sen-Jiang, GE Hong-Liang . Overcoming Decomposition with Order-Reversed Quenching Obtained by Flash Melting[J]. Chin. Phys. Lett., 2013, 30(7): 107502
[10] Osman Murat Ozkendir**. Chromium Substitution Effect on the Magnetic Structure of Iron Oxides[J]. Chin. Phys. Lett., 2012, 29(5): 107502
[11] ZHOU Tie-Ge,LIU Zhi-Qiang**,ZUO Xu. First-Principles Study of Doped Half-Metallic Spinels: Cu0.5Zn0.5Cr2S4, Cu0.5Cd0.5Cr2S4, Li0.5Zn0.5Cr2O4 and Li0.5Zn0.5Cr2S4[J]. Chin. Phys. Lett., 2012, 29(4): 107502
[12] LIU Chun-Ming**, XIANG Xia, ZHANG Yan, JIANG Yong, ZU Xiao-Tao . Magnetism of a Nitrogen-Implanted TiO2 Single Crystal[J]. Chin. Phys. Lett., 2011, 28(12): 107502
[13] CHEN Hai-Ying, ZHANG Yan, YANG Yun-Bo, CHEN Xue-Gang, LIU Shun-Quan, WANG Chang-Sheng, YANG Ying-Chang, YANG Jin-Bo, ** . Magnetostrictions and Magnetic Properties of Nd-Fe-B and SrFe12O19[J]. Chin. Phys. Lett., 2011, 28(7): 107502
[14] LI Yong-Feng, LIU Gui-Bin, SHI Li-Jie, LIU Bang-Gui. Fe-Vacancy-Induced Ferromagnetism in Tetragonal FeSe Thin Films[J]. Chin. Phys. Lett., 2009, 26(12): 107502
[15] ZHOU Guang-Hong, WANG Yin-Gang, QI Xian-Jin. Thermal Stability of CoFe/Cu/CoFe/IrMn Top Spin Valve[J]. Chin. Phys. Lett., 2009, 26(3): 107502
Viewed
Full text


Abstract