| CONDENSED MATTER: STRUCTURE, MECHANICAL AND THERMAL PROPERTIES |
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Unlocking the Potential of Two-Dimensional Janus Superlattices: Directly Visualizing Phonon Transitions |
| Yingzhou Liu, Jincheng Yue, Yinong Liu, Lei-Lei Nian*, and Shiqian Hu* |
| School of Physics and Astronomy, Yunnan University, Kunming 650091, China |
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| Cite this article: |
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Yingzhou Liu, Jincheng Yue, Yinong Liu et al 2023 Chin. Phys. Lett. 40 086301 |
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Abstract Recent research has focused on using Anderson's localization concept to modulate coherent phonon transport by introducing disorder into periodic structures. However, designing and identifying the disorder's strength remain challenging, and visual evidence characterizing phonon localization is lacking. Here, we investigate the effect of disorder on coherent phonon transport in a two-dimensional Janus MoSSe/WSSe superlattice with a defined disorder strength. Using non-equilibrium molecular dynamics, we demonstrate that strong disorder can lead to strong phonon localization, as evidenced by smaller thermal conductivity and significantly different dependence on defect ratio in strongly disordered structures. Furthermore, we propose a novel defect engineering method to determine whether phonon localization occurs. Our work provides a unique platform for modulating coherent phonon transport and presents visual evidence of the phonon transition from localization to nonlocalization. These findings will contribute to development of phonon transport and even phononics, which are essential for thermoelectric and phononic applications.
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Received: 13 July 2023
Published: 07 August 2023
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| PACS: |
63.22.-m
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(Phonons or vibrational states in low-dimensional structures and nanoscale materials)
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63.50.-x65.80.-g
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71.23.-k
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(Electronic structure of disordered solids)
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71.55.Jv
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(Disordered structures; amorphous and glassy solids)
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31.15.xv
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(Molecular dynamics and other numerical methods)
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