Original Articles |
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Large Third-Order Nonlinear Optical Susceptibility of Rh-Doped
BaTiO3 Thin Films Prepared by Pulsed Laser Deposition
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YANG Guang;WANG Huan-Hua;TAN Guo-Tai;JIANG An-Quan;ZHOU Yue-Liang;YANG Guo-Zhen;CHEN Zheng-Hao |
Laboratory of Optical Physics, Institute of Physics and Center for Condensed Matter Physics, Chinese Academy of Sciences, P. O. Box 603, Beijing 100080
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Cite this article: |
YANG Guang, WANG Huan-Hua, TAN Guo-Tai et al 2001 Chin. Phys. Lett. 18 1598-1600 |
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Abstract Rh-doped barium titanate (BaTiO3) epitaxial thin films have been fabricated on SrTiO3 (100) substrates by pulsed laser deposition. The nonlinear optical properties of the films were determined using z-scan method at a wavelength of 532nm with a laser duration of 10ns. The real and imaginary parts of the third-order nonlinear susceptibility x(3) were 5.71 x 10-7 esu and 9.59 x 10-8 esu, respectively. The real part value of x(3) of the Rh:BaTiO3 films is about one order larger than that of Ce-doped BaTiO3 thin films. The results show that Rh:BaTiO3 thin films have great potential applications for nonlinear optical devices.
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Keywords:
42.65.-k
61.10.-i
81.15.Fg
77.84.-s
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Published: 01 December 2001
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PACS: |
42.65.-k
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(Nonlinear optics)
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61.10.-i
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81.15.Fg
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(Pulsed laser ablation deposition)
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77.84.-s
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(Dielectric, piezoelectric, ferroelectric, and antiferroelectric materials)
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