FUNDAMENTAL AREAS OF PHENOMENOLOGY(INCLUDING APPLICATIONS) |
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Two-Dimensional Nonlinear Laser Spectra Calculations with Numerical Path Integral |
LIANG Xian-Ting** |
Department of Physics and Institute of Modern Physics, Ningbo University, Ningbo 315211 |
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Cite this article: |
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Abstract Two-dimensional three-order nonlinear response functions and the laser spectra of the two-level Frenkel-exciton model, interacting with three short laser pulses in direction ?k1+k2+k3, are calculated using the numerical path integral. The method is non-Markovian and the results show that the numerical simulation scheme provides a new pathway for theoretically investigating the multidimensional ultrafast laser spectra including the non-Markovian effects.
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Received: 05 March 2012
Published: 31 July 2012
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