Chin. Phys. Lett.  2009, Vol. 26 Issue (7): 073301    DOI: 10.1088/0256-307X/26/7/073301
ATOMIC AND MOLECULAR PHYSICS |
Theoretical Investigation of Femtosecond-Resolved Photoelectron Spectra of the Li2 Molecule
LIU Yu-Fang, LIU Rui-Qiong, DING Jun-Xia
Department of Physics, Henan Normal University, Xinxiang 453007
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LIU Yu-Fang, LIU Rui-Qiong, DING Jun-Xia 2009 Chin. Phys. Lett. 26 073301
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Abstract The time-dependent quantum wave packet method is used to investigate the dynamics for the Li2 molecule, and the time-resolved photoelectron spectra (TRPES) of the Li2 molecule are calculated. At the short delay time, the particular phenomenon of TRPES with four peaks is qualitatively interpreted in a dressed state picture by analyzing wave packet motion on light-induced potential (LIP). The significant difference in the electronic structure of E1g+ between the inner and outer turning points has an impact on the TRPES. The control for the first excited state A1u+ of the initial wave packet is discussed.
Keywords: 33.60.+q      33.80.Eh      42.50.Ct     
Received: 03 December 2008      Published: 02 July 2009
PACS:  33.60.+q (Photoelectron spectra )  
  33.80.Eh (Autoionization, photoionization, and photodetachment)  
  42.50.Ct (Quantum description of interaction of light and matter; related experiments)  
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https://cpl.iphy.ac.cn/10.1088/0256-307X/26/7/073301       OR      https://cpl.iphy.ac.cn/Y2009/V26/I7/073301
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LIU Yu-Fang
LIU Rui-Qiong
DING Jun-Xia
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