Chin. Phys. Lett.  2007, Vol. 24 Issue (7): 1912-1914    DOI:
Original Articles |
An Effective Method of Producing Small Neutral Carbon Clusters
XIA Zhu-Hong1,2;CHEN Cheng-Chu2;HSU Yen-Chu2
1Department of Physics, Southeast University, Nanjing 2111892Institute of Atomic and Molecular Sciences, Academia Sinica, Taipei
Cite this article:   
XIA Zhu-Hong, CHEN Cheng-Chu, HSU Yen-Chu 2007 Chin. Phys. Lett. 24 1912-1914
Download: PDF(208KB)  
Export: BibTeX | EndNote | Reference Manager | ProCite | RefWorks
Abstract An effective method of producing small neutral carbon clusters Cn(n=1--6) is described. The small carbon clusters (positive or negative charge or neutral) are formed by plasma which are produced by a high power 532nm pulse laser ablating the surface of the metal Mn rod to react with small hydrocarbons supplied by a pulse valve, then the neutral carbon clusters are extracted and photo-ionized by another laser (266nm or 355nm) in the ionization region of a linear time-of-flight mass spectrometer. The distributions of the initial neutral carbon clusters are analysed with the ionic species appeared in mass spectra. It is observed that the yield of small carbon clusters with the present method is about 10 times than that of the traditional widely used technology of laser vaporization of graphite.
Keywords: 36.40.-c      39.90.+d      33.15.Ta     
Received: 04 April 2007      Published: 25 June 2007
PACS:  36.40.-c (Atomic and molecular clusters)  
  39.90.+d  
  33.15.Ta (Mass spectra)  
TRENDMD:   
URL:  
https://cpl.iphy.ac.cn/       OR      https://cpl.iphy.ac.cn/Y2007/V24/I7/01912
Service
E-mail this article
E-mail Alert
RSS
Articles by authors
XIA Zhu-Hong
CHEN Cheng-Chu
HSU Yen-Chu
[1] Weltner W Jr and Van Zee R J 1989 Chem. Rev. 89 1713 andreferences therein
[2] Van Orden A and Saykally R J 1998 Chem. Rev. 98 2313 andreferences therein
[3] Maier J P 1998 J. Phys. Chem. A 102 3462
[4] McCarthy M C and Thaddeus P 2001 Chem. Soc. Rev. 30 177
[5] Hinkle K W, Keady J J and Bernath P F 1988 Science 241 319
[6] Zhang G Q, Chen K S, Merer A J, Hsu Y C, Chen W J, Shaji S and LiaoY A 2005 J. Chem. Phys. 122 244308
[7] McCall B J, Casaes R N, Adamkovics M and Saykally R J 2003 Chem. Phys. Lett. 374 583
[8] Maier J P 1997 Chem. Soc. Rev. 26 21 andreferences therein
[9] Boguslavskiy A E and Maier J P 2006 J. Chem. Phys. 112 094308
[10] Linnartz H, Vaizert O, Motylewski T and Maier J P 2000 J. Chem. Phys. 112 9777
[11] Motylewski T, Vaizert O, Giesen T F, Linnartz H and Maier J P 1999 J. Chem. Phys. 111 6161
[12] Guo B C, Wei S, Purnell J, Buzza S and Castleman A W Jr 1992 Science 256 515
[13] Wei S, Guo B C, Purnell J, Buzza S and Castleman A W Jr 1992 Science 256 818
[14] Sumathi R and Hendrickx M 1998 Chem. Phys. Lett. 287 496
[15] Sumathi R and Hendrickx M 1998 J. Phys. Chem. A 102 4883
[16] Kalemos A and Dunning T H Jr 2005 J. Chem. Phys. 123 014301
[17] Redondo P, Barrientos and Largo A 2006 J. Chem. Theor.Comput. 2 885
[18] Majumdar D, Roszak S and Balasubramanian K 2003 J. Chem.Phys. 118 130
[19] Balfour W J, Cao J Y, Prasad C V V and Qian C X W 1994 J. Chem. Phys. 101 10343
Related articles from Frontiers Journals
[1] GAO Xing-Xin, JIA Yan-Hui, LI Gong-Ping**, CHO Seong-Jin, KIM Hee . Diffusion and Interface Reaction of Cu/Si (100) Films Prepared by Cluster Beam Deposition[J]. Chin. Phys. Lett., 2011, 28(3): 1912-1914
[2] CHEN Liang, , SHE Lei, LI Jiao-Mei, GAO Ke-Lin,. Kinetic Energy of Trapped Ions Cooled by Buffer Gas[J]. Chin. Phys. Lett., 2010, 27(6): 1912-1914
[3] HAN Ji-Feng, YANG Chao-Wen, MIAO Jing-Wei, LU Jian-Feng, LIU Meng, LUO Xiao-Bing, SHI Mian-Gong. An Experimental Observation of Axial Variation of Average Size of Methane Clusters in a Gas Jet[J]. Chin. Phys. Lett., 2010, 27(4): 1912-1914
[4] YAN Hui, , YANG Guo-Qing, , WANG Jin, ZHAN Ming-Sheng,. Directly Trapping Atoms in a U-Shaped Magneto-Optical Trap Using a Mini Atom Chip[J]. Chin. Phys. Lett., 2008, 25(9): 1912-1914
[5] XIE Zun, MA Qing-Min, LIU Ying, LI You-Cheng. Stability and Growth Modes of Ni--C Clusters: A Study based on All-Electron Density Function Theory[J]. Chin. Phys. Lett., 2008, 25(4): 1912-1914
[6] KE Min, YAN Bo, LI Xiao-Lin, WANG Yu-Zhu. Guiding Neutral Atoms with Two Current-Carrying Wires and a Vertical Bias Field on the Atom Chip[J]. Chin. Phys. Lett., 2008, 25(3): 1912-1914
[7] GONG Xiu-Fang, WANG Yin, NING Xi-Jing. Growth of C30 and C31 Clusters: Structures, Energetics and Dynamics[J]. Chin. Phys. Lett., 2008, 25(2): 1912-1914
[8] ZHU Jing-Yi, WANG Bing-Xing, GUO Wei, WANG Yan-Qiu, WANG Li. Simplified Model for Analysing Ion/Photoelectron Images[J]. Chin. Phys. Lett., 2007, 24(7): 1912-1914
[9] MA Qing-Min, XIE Zun, LIU Ying, LI You-Cheng. Configurations, Electronic Structure and Magnetic Ordering of Small Manganese Clusters[J]. Chin. Phys. Lett., 2007, 24(7): 1912-1914
[10] WANG Wen-Min0g, SHE Lei, LI Jiao-Mei, GAO Ke-Lin. Detection of Isotopes of Mercury Ions by Resonant Ejection in Paul Trap[J]. Chin. Phys. Lett., 2007, 24(7): 1912-1914
[11] WAN Hai-Qing, ZHOU Yan-Hong, XU Ying. Transport Properties of Binary Clusters[J]. Chin. Phys. Lett., 2007, 24(12): 1912-1914
[12] ZHOU Yan-Hong, ZHENG Xiao-Hong, XU Ying, ZENG Zhao-Yang, ZENG Zhi. Effects of Relative Orientation of Molecules on Electron Transport in Molecular Devices[J]. Chin. Phys. Lett., 2006, 23(9): 1912-1914
[13] BAI Yu-Lin, CHEN Xiang-Rong, ZHOU Xiao-Lin, CHENG Xiao-Hong, YANG Xiang-Dong,. First-Principles Calculations for Structures and Melting Temperature of Si6 Clusters[J]. Chin. Phys. Lett., 2006, 23(8): 1912-1914
[14] XU Ya-Ge, JI Dong, SHEN Xu-Yang, WANG Xiao-Lu, LI Jia-Ming,. A Theoretical Study of Clusters: Realizing Differences between the Second-Row and the Third-Row Elements[J]. Chin. Phys. Lett., 2006, 23(7): 1912-1914
[15] LIU Fu-Chun, JIN Ming-Xing, DING Da-Jun. Hexapole State-Selection and Beam Focus of Linear Triatomic Molecules[J]. Chin. Phys. Lett., 2006, 23(5): 1912-1914
Viewed
Full text


Abstract