Original Articles |
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Autler--Townes Splitting in Photoelectron Spectrum of Three-Level Li2 Molecule in Ultrashort Pulse Laser Fields |
HU Wen-Hui;YUAN Kai-Jun;HAN Yong-Chang; SHU Chuan-Cun;CONG Shu-Lin |
Department of Physics, Dalian University of Technology, Dalian, 116024 |
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Cite this article: |
HU Wen-Hui, YUAN Kai-Jun, HAN Yong-Chang et al 2007 Chin. Phys. Lett. 24 1556-1559 |
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Abstract The Autler--Townes (AT) splitting in femtosecond photoelectron spectrum of three-level Li2 molecules is theoretically investigated using time-dependent quantum wave packet method. With proper femtosecond laser pulses, three peaks of the AT splitting can be observed in the photoelectron spectrum. The AT splitting stems from rapid Rabi oscillation caused by intense ultrashort laser pluses. The effects of laser parameters on the molecular ionization dynamics are also discussed.
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Keywords:
33.80.Eh
42.50.Hz
82.53.Kp
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Received: 07 November 2006
Published: 17 May 2007
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PACS: |
33.80.Eh
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(Autoionization, photoionization, and photodetachment)
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42.50.Hz
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(Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift)
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82.53.Kp
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(Coherent spectroscopy of atoms and molecules)
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