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Rotational and Vibrational Temperatures of Atmospheric Double rc Argon--Nitrogen Plasma |
YAN Jian-Hua1;TU Xin1;MA Zeng-Yi1;CEN Ke-Fa1;B. G. Cheron2 |
1State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 3100272UMR 6614 CNRS CORIA, Saint Etienne du Rouvray 76801, France |
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Cite this article: |
YAN Jian-Hua, TU Xin, MA Zeng-Yi et al 2007 Chin. Phys. Lett. 24 1317-1321 |
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Abstract The spectroscopic technique is employed to study the emission of atmospheric argon--nitrogen plasma jet generated by an original dc double anode plasma torch. The molecular bands of the N2+ first negative system are observed at the torch exit and chosen to evaluate the rotational and vibrational temperatures in comparison with the simulated spectra. The excitation temperature (Texc ≈9600K) is determined from the Boltzmann plot method. The results show that the rotational, vibrational, electron and kinetic temperatures are in good agreement with one another, which indicates that the core region of atmospheric double arc argon--nitrogen plasma jet at the torch exit is close to the local thermodynamic equilibrium state under our experimental conditions.
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Keywords:
52.70.Kz
52.75.Hn
33.20.Vq
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Received: 09 November 2006
Published: 23 April 2007
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PACS: |
52.70.Kz
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(Optical (ultraviolet, visible, infrared) measurements)
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52.75.Hn
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(Plasma torches)
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33.20.Vq
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(Vibration-rotation analysis)
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[1] Pfender E 1999 Plasma Chem. Plasma Process 19 1 [2] Gao K L, Zhan R J, Wang C L, Cao J X and Xiang Z L 1992 Chin.Phys. Lett. 9 144 [3] Lofthus A and Krupenie P H 1977 J. Phys. Chem.Ref. Data 6 133 [4] Czernichowski A 1987 J. Phys. D: Appl. Phys. 20 559 [5] Rajabian M 2001 Ph.D. Thesis (Uniersity of Sherbrooke) chap4 p 66 [6] Laux C O, Gressman R J, Kruger C H, Roux F, Michaud F and Dais S P2001 J. Quant. Spectrosc. Radiat. Transfer 68 473 [7] Kang Z D and Pu Y K 2002 Chin. Phys. Lett. 19 211 [8] Zhang J L, Liu L Y, Ma T C and Den X L 2002 SpectrochimicaActa A 58 1915 [9] Nagy O 2003 Chem. Phys. 286 109 [10] Beletse A A, Kukushkin A M, Fedoro A et al 2004 HighTemperature 42 342 [11] Rajabian M, Graelle D and acquie S 2004 Plasma Chem.Plasma Process 24 285 [12] Herzberg G 1950 Molecular Spectra and MolecularStructure: Spectra of Diatomic molecules, olume I (Princeton: anNostrand Reinhold) chap 4 p 151 [13] Gilmore F R, Laher R R and Espy P J 1992 J. Phys.Chem. Ref. Data 21 1005 [14] Kovacs I 1969 Rotational Structure in the Spectra of DiatomicMolecule (London: Adam Hilger) chap 3 p 66 |
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