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Theoretical Investigation of Femtosecond-Resolved Photoelectron Spectrum of Na2 Molecules |
MIAO Xiang-Yang1;WANG Lei1;YAO Li2;SONG He-Shan1 |
1School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 1160232Department of Physics, Dalian Maritime University, Dalian 116026 |
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Cite this article: |
MIAO Xiang-Yang, WANG Lei, YAO Li et al 2007 Chin. Phys. Lett. 24 2815-2818 |
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Abstract Effect of laser fields on Na2 interaction potentials is studied by calculating the time-resolved photoelectron spectrum (TRPES) with the time-dependent wave-packet method. It is shown that the photoelectron spectrum at different delay times reflects the population in different electronic states. We inspect the periodicity of vibrational motion in neutral states, and map the vibrational wave-packet propagation in corresponding internuclear coordinate.
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Keywords:
33.60.-q
33.80.Eh
42.50.Ct
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Received: 26 February 2007
Published: 20 September 2007
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PACS: |
33.60.-q
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33.80.Eh
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(Autoionization, photoionization, and photodetachment)
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42.50.Ct
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(Quantum description of interaction of light and matter; related experiments)
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[1] Reiss H R 1997 Laser Phys. 7 543 [2] Hu J, Han K L and He G Z 2005 Phys. Rev. Lett. 95 123001 [3] Kwak H, Chou K C, Guo J and Tom H W K 1999 Phys. Rev. Lett. 83 3745 [4] Zhang H, Han K L, Zhao Y, He G Z and Lou N Q 1997 Chem. Phys.Lett. 271 204 [5] Khundkar L R and Zewail A H 1990 Ann. Rev. Phys. Chem. 41 15 [6] Cong P, Mokhtari A and Zewail A H 1990 Chem. Phys. Lett. 172 109 [7] Frohnmeyer T, Hofmann M, Strehle M and Baumert T 1999 Chem. Phys. Lett. 312 447 [8] Baumert T, B\"uhler B, Grosser M, Weiss V, Wiedenmann E andGerber G 1991 J. Phys. Chem. 95 8103 [9] Baumert T, Engel V and Meier C 1992 Chem. Phys. Lett. 200 488 [10] Meier Ch and Engel V 1993 Chem. Phys. Lett. 212 691 [11] Feit M D, Fleck J J A and Steiger A 1982 J. Comput.Phys. 47 412 [12] Xie T X, Zhang Y, Zhao M Y and Han K L 2003 Phys. Chem.Chem. Phys. 5 2034 [13] Chu T S, Zhang Y and Han K L 2006 Int. Rev. Phys. Chem. 25 201 [14] Kosloff R and Kosloff D 1983 J. Chem. Phys. 79 1823 [15] Zhao M Y, Meng Q T, Xie T X, Han K L and He G Z 2005 Int. J.Quantum Chem. 101 153 [16] Hu J, Meng Q T and Han K L 2004 Chem. Phys. Lett. 393 393 [17] Meng Q T, Yang G H, Sun H L, Han K L and Lou N Q 2003 Phys. Rev. A 67 063202 [18] Miao X Y, Wang Lei and Song H S 2007 Phys. Rev. A 75 042512 [19] Miao X Y, Wang Lei, Yao Li and Song H S 2006 Chem. Phys.Lett. 433 28 |
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