Chin. Phys. Lett.  1999, Vol. 16 Issue (9): 641-642    DOI:
Original Articles |
Quantum Beat Spectroscopy of SO2 in the 235-224nm Range
CHEN Yang;PEI Lin-sen;JIN Jin;CHEN Cong-xiang;MA Xing-xiao
Department of Chemical Physics, University of Science and Technology of China, Hefei 230026 Open Laboratory of Bond Selective Chemistry, Chinese Academy of Sciences, Hefei 230026
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CHEN Yang, PEI Lin-sen, JIN Jin et al  1999 Chin. Phys. Lett. 16 641-642
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Abstract Using time-resolved laser-induced fluorescence(L1F) spectroscopy, the fluorescence quantum beat decay was observed in C ( 1B2 ) ← X(1A1) transition of SO2 molecule. The experimental results show that only the v3 mode and its combination band v1 + v2 + v3 excitation exist the beat decay. Analyzing the result, we attribute the quantum beat states to the coupling of the v3 vibration mode of C state with the high vibrational levels of the electronic ground state.



Keywords: 33.20.Vq      33.50.Dq      33.80.Be     
Published: 01 September 1999
PACS:  33.20.Vq (Vibration-rotation analysis)  
  33.50.Dq (Fluorescence and phosphorescence spectra)  
  33.80.Be (Level crossing and optical pumping)  
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https://cpl.iphy.ac.cn/       OR      https://cpl.iphy.ac.cn/Y1999/V16/I9/0641
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CHEN Yang
PEI Lin-sen
JIN Jin
CHEN Cong-xiang
MA Xing-xiao
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