| CONDENSED MATTER: STRUCTURE, MECHANICAL AND THERMAL PROPERTIES |
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Pressure Driven Structural Evolutions of 0.935(Na$_{0.5}$Bi$_{0.5}$)TiO$_{3}$-0.065BaTiO$_{3}$ Lead-Free Ferroelectric Single Crystal through Raman Spectroscopy |
| Qunfei Zheng1,2,4†, Qiang Li1,3†, Saidong Xue1, Yanhui Wu1, Lijuan Wang2, Qian Zhang3, Xiaomei Qin1*, Xiangyong Zhao1, Feifei Wang1, and Wenge Yang3 |
1Department of Physics, Mathematics & Science College, Shanghai Normal University, Shanghai 200234, China
2Center for High Pressure Science and Technology Advanced Research (HPSTAR), Beijing 100094, China
3Center for High Pressure Science and Technology Advanced Research (HPSTAR), Shanghai 201203, China
4Academy for Advanced Interdisciplinary Studies, Shenzhen Engineering Research Center for Frontier Materials Synthesis at High Pressures, Southern University of Science and Technology (SUSTech), Shenzhen 518055, China
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| Cite this article: |
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Qunfei Zheng, Qiang Li, Saidong Xue et al 2021 Chin. Phys. Lett. 38 026102 |
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Abstract Pressure evolution of local structure and vibrational dynamics of the perovskite-type relaxor ferroelectric single crystal of 0.935(Na$_{0.5}$Bi$_{0.5}$)TiO$_{3}$-0.065BaTiO$_{3}$ (NBT-6.5BT) is systematically investigated via in situ Raman spectroscopy. The pressure dependence of phonon modes up to 30 GPa reveals two characteristic pressures: one is at around 4.6 GPa which corresponds to the rhombohedral-to-tetragonal phase transition, showing that the pressure strongly suppresses the coupling between the off-centered A- and B-site cations; the other structural transition involving the oxygen octahedral tilt and vibration occurs at pressure $\sim $13–15 GPa with certain degree of order-disorder transition, evidenced by the abnormal changes of intensity and FWHM in Raman spectrum.
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Received: 16 November 2020
Published: 27 January 2021
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| PACS: |
61.50.Ks
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(Crystallographic aspects of phase transformations; pressure effects)
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77.84.-s
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(Dielectric, piezoelectric, ferroelectric, and antiferroelectric materials)
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78.30.-j
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(Infrared and Raman spectra)
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| Fund: Supported by the National Natural Science Foundation of China (Grant Nos. 11674231, 11974250, and 51772192), the Science and Technology Commission of Shanghai Municipality (Grant Nos. 17070502700 and 19070502800), and the Shenzhen Development and Reform Commission Foundation for Shenzhen Engineering Research Center for Frontier Materials Synthesis at High Pressures. |
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| [1] | Jaffe B, Cook W R and Jaffe H 1971 Piezoelectric Ceramics (London: Academic Press) |
| [2] | Saito Y, Takao H, Tani T, Nonoyama T, Takatori K, Homma T, Nagaya T and Nakamura M 2004 Nature 432 84 |
| [3] | Rodel J, Jo W, Seifert K T P, Anton E M, Granzow T and D 2009 J. Am. Ceram. Soc. 92 1153 |
| [4] | Li Y, Chen W, Zhou J, Xu Q, Sun H and Liao M 2005 Ceram. Int. 31 139 |
| [5] | Li Y, Chen W, Xu Q, Zhou J, Gu X and Fang S 2005 Mater. Chem. Phys. 94 328 |
| [6] | Takenaka T, Maruyama K and Sakata K 1991 Jpn. J. Appl. Phys. 30 2236 |
| [7] | Ma C, Guo H Z, Beckman S P and Tan X L 2012 Phys. Rev. Lett. 109 107602 |
| [8] | Li F, Zhang S J, Xu Z and Chen L Q 2017 Adv. Funct. Mater. 27 1700310 |
| [9] | Kang S J L, Park J H, Ko S Y and Lee H Y 2015 J. Am. Ceram. Soc. 98 347 |
| [10] | Chiang Y M, Farrey G W and Soukhojak A N 1998 Appl. Phys. Lett. 73 3683 |
| [11] | Jin C F, Zhang S Q, Shen Z Q and Li W L 2019 Chin. Phys. Lett. 36 107701 |
| [12] | Eerd B W, Damjanovic D, Klein N, Setter N and Trodahl J 2010 Phys. Rev. B 82 104112 |
| [13] | Huang T, Guo S, Xu L P, Chen C, Luo H S, Chu J H and Hu Z G 2015 J. Appl. Phys. 117 224103 |
| [14] | Kreisel J and Glazer A M 2000 J. Phys.: Condens. Matter 12 9689 |
| [15] | Datta K, Richter A, Göbbels M, Neder R B and Mihailova B 2014 Phys. Rev. B 90 064112 |
| [16] | Rout D, Moon K S, Rao V S and Kang S J L 2009 J. Ceram. Soc. Jpn 117 797 |
| [17] | Kreisel J, Bouvier P, Dkhil B, Thomas P A, Glazer A, Welberry T, Chaabane B and Mezouar M 2003 Phys. Rev. B 68 014113 |
| [18] | Thomas P A, Kreisel J, Glazer A M, Bouvier P, Jiang Q and Smith R 2005 Z. Kristallogr. 220 717 |
| [19] | Kreisel J, Glazer A, Bouvier P and Lucazeau G 2001 Phys. Rev. B 63 174106 |
| [20] | Glazer A M 1972 Acta Crystallogr. Sect. B: Struct. Crystallogr. Cryst. Chem. 28 3384 |
| [21] | Kreisel J, Glazer A M, Jones G, Thomas P A, Abello L and Lucazeau G 2000 J. Phys.: Condens. Matter 12 3267 |
| [22] | Ruiz-Fuertes J, Winkler B, Bernert T, Bayarjargal L, Morgenroth W, Koch-Müller M, Refson K, Milman V and Tamura N 2015 Phys. Rev. B 91 214110 |
| [23] | Venkateswaran U D, Naik V M and Naik R 1998 Phys. Rev. B 58 14256 |
| [24] | Zhang H W, Chen C, Deng H, Ren B, Zhao X Y, Lin D, Li X B and Luo H S 2014 J. Mater. Chem. C 2 10124 |
| [25] | Zheng Q, Zhao X, Sun R and Luo H 2011 Phys. Status Solidi A 208 1012 |
| [26] | Mao H K, Bell P M, Shaner J W and Steinberg D J 1978 J. Appl. Phys. 49 3276 |
| [27] | Zhang M S and Scott J F 1986 Ferroelectr. Lett. Sect. 6 147 |
| [28] | Trujillo S, Kreisel J, Jiang Q, Smith J H, Thomas P A, Bouvier P and Weiss F 2005 J. Phys.: Condens. Matter 17 6587 |
| [29] | Wang J, Zhou Z and Xue J 2006 Acta Mater. 54 1691 |
| [30] | Deluca M, Picht G, Hoffmann M J, Rechtenbach A, Töpfer J, Schader F H and Webber K G 2015 J. Appl. Phys. 117 134110 |
| [31] | Schütz D, Deluca M, Krauss W, Feteira A, Jackson T and Reichmann K 2012 Adv. Funct. Mater. 22 2285 |
| [32] | Cordero F, Craciun F, Trequattrini F, Mercadelli E and Galassi C 2010 Phys. Rev. B 81 144124 |
| [33] | Luo L, Ge J, Li J, Viehland D, Farley C, Bondnar R, Zheng Q and Luo H 2011 J. Appl. Phys. 109 113507 |
| [34] | Rout D, Moon K S, Park J and Kang S J L 2013 Curr. Appl. Phys. 13 1988 |
| [35] | Bismayer U 1990 Phase Transit. 27 211 |
| [36] | Welsch A M, Mihailova B, Gospodinov M, Stosch R, Güttler B and Bismayer U 2009 J. Phys.: Condens. Matter 21 235901 |
| [37] | Welsch A M, Maier B J, Mihailova B, Angel R J, Zhao J, Paulmann C, Engel J M, Gospodinov M, Marinova V and Bismayer U 2011 Z. Kristallogr. 226 126 |
| [38] | Waeselmann N, Mihailova B, Maier B J, Paulmann C, Gospodinov M, Marinova V and Bismayer U 2011 Phys. Rev. B 83 214104 |
| [39] | Salje E, Devarajan V, Bismayer U and Guimaraes D M C 1983 J. Phys. C 16 5233 |
| [40] | de la F G, Malcherek T, Gorfman S and Mihailova B 2017 Phys. Rev. B 96 214102 |
| [41] | Hill N A and Rabe K M 1999 Phys. Rev. B 59 8759 |
| [42] | Baettig P, Schelle C F, LeSar R, Waghmare U V and Spaldin N A 2005 Chem. Mater. 17 1376 |
| [43] | Maier B J, Angel R J, Marshall W G, Mihailova B, Paulmann C, Engel J M, Gospodinov M, Welsch A M, Petrova D and Bismayer U 2010 Acta Crystallogr. Sect. B: Struct. Crystallogr. Cryst. Chem. 66 280 |
| [44] | Jones G O and Thomas P A 2002 Acta Crystallogr. Sect. B: Struct. Crystallogr. Cryst. Chem. 58 168 |
| [45] | Fujii Y, Hoshino S, Yamada Y and Shirane G 1974 Phys. Rev. B 9 4549 |
| [46] | Zhu J L, Jin C Q, Cao W W and Wang X H 2008 Appl. Phys. Lett. 92 242901 |
| [47] | Han W, Zhu J L, Zhang S J, Zhang H, Wang X H, Wang Q L, Gao C X and Jin C Q 2013 J. Appl. Phys. 113 193513 |
| [48] | Zhu J L, Xiao C J, Chi Z H, Feng S M, Li F Y, Jin C Q, Deng X Y, Wang X H, Li L T, Dai Z H, W J and Xu Z 2006 Chin. Phys. Lett. 23 1631 |
| [49] | Li F Y, Jin C Q, You S J, Xiao C J, Yu R C, Wang X H, Liu J, Li X D, Li Y C and Chen C L 2006 Chin. Phys. Lett. 23 1249 |
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