Chin. Phys. Lett.  2023, Vol. 40 Issue (11): 117501    DOI: 10.1088/0256-307X/40/11/117501
CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES |
Giant 2D Skyrmion Topological Hall Effect with Ultrawide Temperature Window and Low-Current Manipulation in 2D Room-Temperature Ferromagnetic Crystals
Gaojie Zhang1,2, Qingyuan Luo3, Xiaokun Wen1,2, Hao Wu1,2*, Li Yang1,2, Wen Jin1,2, Luji Li1,2, Jia Zhang4, Wenfeng Zhang1,2,5, Haibo Shu3*, and Haixin Chang1,2,5*
1State Key Laboratory of Material Processing and Die & Mold Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China
2Wuhan National High Magnetic Field Center and Institute for Quantum Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China
3College of Optical and Electronic Technology, China Jiliang University, Hangzhou 310018, China
4School of Physics and Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074, China
5Shenzhen R&D Center of Huazhong University of Science and Technology, Shenzhen 518000, China
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Gaojie Zhang, Qingyuan Luo, Xiaokun Wen et al  2023 Chin. Phys. Lett. 40 117501
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Abstract The discovery and manipulation of topological Hall effect (THE), an abnormal magnetoelectric response mostly related to the Dzyaloshinskii–Moriya interaction (DMI), are promising for next-generation spintronic devices based on topological spin textures such as magnetic skyrmions. However, most skyrmions and THE are stabilized in a narrow temperature window either below or over room temperature with high critical current manipulation. It is still elusive and challenging to achieve large THE with both wide temperature window till room temperature and low critical current manipulation. Here, using controllable, naturally oxidized sub-20 and sub-10 nm 2D van der Waals room-temperature ferromagnetic Fe$_{3}$GaTe$_{2-x}$ crystals, we report robust 2D skyrmion THE with ultrawide temperature window ranging in three orders of magnitude from 2 to 300 K, in combination with giant THE of $\sim$ 5.4 $µ \Omega\cdot$cm at 10 K and $\sim$ 0.15 $µ \Omega\cdot$cm at 300 K, which is 1–3 orders of magnitude larger than that of all known room-temperature 2D skyrmion systems. Moreover, room-temperature current-controlled THE is also realized with a low critical current density of $\sim$ $6.2\times10^{5}$ A$\cdot$cm$^{-2}$. First-principles calculations unveil natural oxidation-induced highly enhanced 2D interfacial DMI reasonable for robust giant THE. This work paves the way to room-temperature electrically controlled 2D THE-based practical spintronic devices.
Received: 17 October 2023      Express Letter Published: 01 November 2023
PACS:  75.70.Cn (Magnetic properties of interfaces (multilayers, superlattices, heterostructures))  
  12.39.Dc (Skyrmions)  
  75.50.Gg.  
  85.75.-d (Magnetoelectronics; spintronics: devices exploiting spin polarized transport or integrated magnetic fields)  
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https://cpl.iphy.ac.cn/10.1088/0256-307X/40/11/117501       OR      https://cpl.iphy.ac.cn/Y2023/V40/I11/117501
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Gaojie Zhang
Qingyuan Luo
Xiaokun Wen
Hao Wu
Li Yang
Wen Jin
Luji Li
Jia Zhang
Wenfeng Zhang
Haibo Shu
and Haixin Chang
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