| CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES |
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Tunable Thermal Conductivity of Ferroelectric P(VDF-TrFE) Nanofibers via Molecular Bond Modulation |
| Lan Dong1,2, Bohai Liu3, Yuanyuan Wang1,2*, and Xiangfan Xu3* |
1School of Energy and Materials, Shanghai Polytechnic University, Shanghai 201209, China
2Shanghai Engineering Research Center of Advanced Thermal Functional Materials, Shanghai Polytechnic University, Shanghai 201209, China
3Center for Phononics and Thermal Energy Science, China-EU Joint Center for Nanophononics, School of Physics Science and Engineering, Tongji University, Shanghai 200092, China
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| Cite this article: |
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Lan Dong, Bohai Liu, Yuanyuan Wang et al 2022 Chin. Phys. Lett. 39 127201 |
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Abstract Dipoles in ferroelectric copolymer P(VDF-TrFE) can be driven by electric field, introducing phonon transport modulations via polarizing molecular chains. The thermal conductivity in single 75/25 P(VDF-TrFE) nanofibers is found to increase with electric field related phonon renormalization, resulted from change in vibrational assignment excited by polarization process. This is evidenced by a direct change of bond energy and bond length in 75/25 P(VDF-TrFE) nanofibers from Raman characterization under polarization electric field. The experimental results provide further intuitive evidences that the size of ferroelectric polymers could directly affect the ferroelectricity from the size-dependent thermal transport measurement.
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Received: 27 September 2022
Published: 04 December 2022
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| PACS: |
65.60.+a
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(Thermal properties of amorphous solids and glasses: heat capacity, thermal expansion, etc.)
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44.10.+i
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(Heat conduction)
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66.30.hk
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(Polymers)
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74.25.Kc
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(Phonons)
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