Exploration of High-Harmonic Generation from the CS$_2$ Molecule by the Lewenstein Method in Two-Color Circularly Polarized Laser Field

doi:10.1088/0256-307X/34/1/014206

Chin. Phys. Lett.

2017, Vol. 34

Issue (1): 014206 DOI: 10.1088/0256-307X/34/1/014206

FUNDAMENTAL AREAS OF PHENOMENOLOGY(INCLUDING APPLICATIONS)

Exploration of High-Harmonic Generation from the CS$_2$ Molecule by the Lewenstein Method in Two-Color Circularly Polarized Laser Field

Hong-Dan Zhang¹, Jing Guo^1,2**, Yan Shi^1,3, Hui Du¹, Hai-Feng Liu¹, Xu-Ri Huang², Xue-Shen Liu^1**, Jun Jing¹

¹Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012
²Institute of Theoretical Chemistry, Jilin University, Changchun 130012
³National Center of Quality Supervision and Inspection of Automobile Spare Parts, Changchun 130012

Cite this article:

Hong-Dan Zhang, Jing Guo, Yan Shi et al 2017 Chin. Phys. Lett. 34 014206

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Abstract The high harmonic generation (HHG) from the CS$_2$ molecule in intense laser fields is investigated using the extended Lewenstein method. The initial state is the highest-occupied molecular orbital of the CS$_2$ molecule, which can be well described by Gaussian wave packet using GAMESS-UK package. Compared with the case of the elliptical laser, the HHG can be extended in two-color circularly polarized laser field. The time-frequency analysis and classical electron trajectory as well as the ionization yield curve are also presented to further explain the underlying mechanism. After adding a static electric field on the $z$-direction, the single quantum path control is realized and the supercontinuum spectra are obtained. Moreover, an isolated 110 as pulse can be obtained by superposing the harmonics from 130th to 180th order.

Received: 06 September 2016 Published: 29 December 2016

PACS:	42.65.Ky	(Frequency conversion; harmonic generation, including higher-order harmonic generation)
	42.65.Re	(Ultrafast processes; optical pulse generation and pulse compression)
	32.80.Rm	(Multiphoton ionization and excitation to highly excited states)

Fund: Supported by the National Natural Science Foundation of China under Grant Nos 11574117, 11271158, 61575077 and 11575071.

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https://cpl.iphy.ac.cn/10.1088/0256-307X/34/1/014206 OR https://cpl.iphy.ac.cn/Y2017/V34/I1/014206

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	Hong-Dan Zhang
	Jing Guo
	Yan Shi
	Hui Du
	Hai-Feng Liu
	Xu-Ri Huang
	Xue-Shen Liu
	Jun Jing

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