| ATOMIC AND MOLECULAR PHYSICS |
|
|
|
|
Manipulation of Resonance-Enhanced Multiphoton-Ionization Photoelectron Spectroscopy by Two Time-Delayed Femtosecond Laser Pulses |
| LU Chen-Hui, ZHANG Shi-An**, SUN Zhen-Rong |
State Key Laboratory of Precision Spectroscopy, and Department of Physics, East China Normal University, Shanghai 200062
|
|
| Cite this article: |
|
LU Chen-Hui, ZHANG Shi-An, SUN Zhen-Rong 2013 Chin. Phys. Lett. 30 113302 |
|
|
|
|
Abstract We theoretically demonstrate that the (2+1) resonance-enhanced multiphoton-ionization (REMPI) photoelectron spectrum in a cesium (Cs) atom can be effectively manipulated by two time-delayed femtosecond laser pulses, involving its photoelectron spectral structure and photoelectron energy. We show that the photoelectron spectrum exhibits interference fringes and the fringe spacing is determined by the time delay of the two laser pulses, and the photoelectron energy is periodically modulated and the modulation period is determined by the two-photon transition frequency of the excited state. Finally, we utilize the power spectrum of the two time-delayed laser pulses and the two-photon transition probability of the excited state to respectively explain the modulations of the photoelectron spectrum and photoelectron energy.
|
|
|
Received: 09 September 2013
Published: 30 November 2013
|
|
| PACS: |
33.60.+q
|
(Photoelectron spectra )
|
| |
32.80.Qk
|
(Coherent control of atomic interactions with photons)
|
| |
32.80.Rm
|
(Multiphoton ionization and excitation to highly excited states)
|
|
|
|
|
|
[1] Goswami D 2003 Phys. Rep. 374 385
[2] Silberberg Y 2009 Annu. Rev. Phys. Chem. 60 277
[3] Nuernberger P, Vogt G, Brixner T and Gerber G 2007 Phys. Chem. Chem. Phys. 9 2470
[4] Dantus M and Lozovoy V V 2004 Chem. Rev. 104 1813
[5] Zhang S, Zhang H, Jia T, Wang Z and Sun Z 2009 Phys. Rev. A 80 043402
[6] Bruner B D, Suchowski H, Vitanov N V and Silberberg Y 2010 Phys. Rev. A 81 063410
[7] Lozovoy V V, Pastirk L, Walowicz K A and Dantus M 2003 J. Chem. Phys. 118 3187
[8] Amitay Z, Gandman A, Chuntonov L and Rybak L 2008 Phys. Rev. Lett. 100 193002
[9] Bartels R, Backus S, Zeek E, Misoguti L, Vdovin G, Chris-tov I P, Murnane M and Kapteyn H C 2000 Nature 406 164
[10] Van Rhijn A C W, Jurna M, Jafarpour A, Herek J L and Offerhaus H L 2011 J. Raman Spectrosc. 42 1859
[11] Zhang S, Zhang H, Jia T, Wang Z and Sun Z 2010 J. Chem. Phys. 132 044505
[12] Katz O, Levitt J M, Grinvald E and Silberberg Y 2010 Opt. Express 18 22693
[13] Patel V, Malinovsky V S and Malinovskaya S 2010 Phys. Rev. A 81 063404
[14] Konradi J, Singh A K and Materny A 2006 J. Photochem. Photobiol. A 180 289
[15] Wollenhaupt M, Bayer T, Vitanov N V and Baumert T 2010 Phys. Rev. A 81 053422
[16] Krug M, Bayer T, Wollenhaupt M, Sarpe-Tudoran C, Baumert T, Ivanov S S and Vitanov N V 2009 New J. Phys. 11 105051
[17] Prabhudesai V S, Lev U, Natan A, Bruner B D, Diner A, Heber O, Strasser D, Schwalm D, Ben-Itzhak I, Hua J J, Esry B D, Silberberg Y and Zajfman D 2010 Phys. Rev. A 81 023401
[18] Plenge J, Wirsing A, Wagner-Drebenstedt I, Halfpap I, Kieling B, Wassermann B and Ruehl E 2011 Phys. Chem. Chem. Phys. 13 8705
[19] Zhang J, Harthcock C and Kong W 2012 J. Phys. Chem. A 116 1551
[20] Zhang J, Harthcock C, Han F Y and Kong W 2011 J. Chem. Phys. 135 244306
[21] Shen L, Zhang B L and Suits A G 2010 J. Phys. Chem. A 114 3114
[22] Liu Y F, Liu R Q and Ding J X 2009 Chin. Phys. Lett. 26 073301
[23] Ding J X, Liu Y F and Liu R Q 2010 Chin. Phys. B 19 033301
[24] Blanchet V, Boye S, Zamith S, Campos A, Girard B, Lievin J and Gauyacq D 2003 J. Chem. Phys. 119 3751
[25] Liu J, Kim H T and Anderson S L 2001 J. Chem. Phys. 114 9797
[26] Morre N P and Levis R J 2000 J. Chem. Phys. 112 1316
[27] Scherper C R, Kuijt J, Buma W J and de Lange C A 1998 J. Chem. Phys. 109 7844
[28] Xu H G, Zhang Z G, Zheng W J, Wu M M and Sun Q 2011 Chin. Phys. B 20 043102
[29] Wollenhaupt M, Bayer T, Vitanov N V and Baumert T 2010 Phys. Rev. A 81 053422
[30] Wollenhaupt M, Pr?kelt A, Sarpe-Tudoran C, Liese D, Bayer T and Baumert T 2006 Phys. Rev. A 73
[31] Wollenhaupt M, Pr?kelt A, Sarpe-Tudoran C, Liese D, Bayer T and Baumert T 2006 Appl. Phys. B 82 183
[32] Wollenhaupt M, Pr?kelt A, Sarpe-Tudoran C, Liese D, Bayer T and Baumert T 2005 J. Opt. B 7 S270
[33] Wollenhaupt M, Engle V and Baumert T 2005 Annu. Rev. Phys. Chem. 56 25
[34] Zhang S, Zhang H, Jia T, Wang Z and Sun Z 2010 J. Phys. B 43 135401
[35] Zhang S, Lu C, Jia T, Qiu J and Sun Z 2012 J. Chem. Phys. 137 174301
[36] Zhang S, Lu C, Jia T and Sun Z 2012 Phys. Rev. A 86 012513
[37] Zhang S, Lu C, Jia T, Qiu J and Sun Z 2012 Phys. Rev. A 86 043433
[38] Bouchene M A et al 1998 Eur. Phys. J. D 2 131
[39] Zhang S et al 2013 Phys. Rev. A 87 035403
[40] Meshulach D and Silberberg Y 1999 Phys. Rev. A 60 1287
[41] Wollenhaupt M et al 2002 Phys. Rev. Lett. 89 173001 |
|
Viewed |
|
|
|
Full text
|
|
|
|
|
Abstract
|
|
|
|
|
