Two-Dimensional Nonlinear Laser Spectra Calculations with Numerical Path Integral
LIANG Xian-Ting**
Department of Physics and Institute of Modern Physics, Ningbo University, Ningbo 315211
Abstract ：Two-dimensional three-order nonlinear response functions and the laser spectra of the two-level Frenkel-exciton model, interacting with three short laser pulses in direction ?k 1 +k 2 +k 3 , are calculated using the numerical path integral. The method is non-Markovian and the results show that the numerical simulation scheme provides a new pathway for theoretically investigating the multidimensional ultrafast laser spectra including the non-Markovian effects.
收稿日期: 2012-03-05
出版日期: 2012-07-31
[1] Mukamel S and Abramavicius D 2004 Chem. Rev. 104 2073 2008 Chem. Rev. 108 1331 2003 Annu. Rev. Phys. Chem. 54 425 1990 Annu. Rev. Phys. Chem. 41 647 2009 Annu. Rev. Phys. Chem. 60 21 2006 Adv. Chem. Phys. 132 1 2004 Opt. Lett. 29 884 1980 J. Chem. Phys. 73 648 1974 Opt. Commun. 12 191 1991 J. Chem. Phys. 94 2413 1989 Adv. Chem. Phys. 75 1 2005 Nature 434 625 2005 Science 309 1338 2005 Proc. Natl. Acad. Sci. USA 102 11185 2010 J. Chem. Phys. 132 134506 Principles of Nonlinear Optical Spectroscopy (New York: Oxford Unversity Press)2006 J. Phys. Chem. B 110 3362 1991 J. Chem. Phys. 94 179 2007 J. Chem. Phys. 127 075101 2007 Europhys. Lett. 80 17005 2008 Chem. Phys. 347 185 2010 J. Chem. Phys. 132 024505 1994 Chem. Phys. Lett. 221 482 1995 J. Chem. Phys. 102 4600 1995 J. Chem. Phys. 102 4611 1996 Proc. Natl. Acad. Sci. USA 93 3926 2000 Phys. Rev. E 62 5808 2004 Chem. Phys. 296 333 2007 Chem. Phys. Lett. 449 296 2008 Chem. Phys. 352 106 2005 Phys. Rev. B 72 245328 2010 Phys. Rev. E 81 011906 1997 Comput. Phys. Commun. 99 335 2010 Phys. Rev. E 82 051918 2006 J. Phys. Chem. B 110 3362 2011 J. Phys. Chem. A 115 3787
[1]
.
[2]
.
[3]
.
[4]
.
[5]
.
[6]
.
[7]
.
[8]
.
[9]
.
[10]
.
[11]
.
[12]
.
[13]
.
[14]
.
[15]
.
2012, Vol. 29 
