Improvement of Cyclic Stability of Na$_{0.67}$Mn$_{0.8}$Ni$_{0.1}$Co$_{0.1}$O$_{2}$ via Suppressing Lattice Variation
Zhongmin Ren1 , Muqin Wang1,3* , Shuaishuai Chen2 , Lei Ding2 , Hua Li1 , Jian Liu1 , Jieyun Zheng4* , Zhihong Liu1 , Deyu Wang1,2* , and Mingkui Wang3
1 Key Laboratory of Optoelectronic Chemical Materials and Devices, School of Chemical and Environmental Engineering, Jianghan University, Wuhan 430056, China2 Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China3 Wuhan National Laboratory for Optoelectronics, Huazhong University of Science & Technology, Wuhan 430074, China4 Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China
Abstract ：Strategies to prolong operational life are highly pursued to strengthen the advantage of cost-effectiveness on sodium-ion batteries (SIBs). We demonstrate the crucial influence of particles' internal mechanical strains on durability of cathode, which does not attract enough attentions from the community. Among the investigated samples, 2% Ti-modified-Na$_{0.67}$Ni$_{0.1}$Co$_{0.1}$Mn$_{0.8}$O$_{2}$ suppresses the $c$-axis lattice variation by 38%, attains the reversible capacity 86% higher after 200 cycles, and still keeps intact morphology. This approach indicates that the mechanical properties could tailor cyclic stability of cathode, which is particular important to further improve competitiveness for SIBs.
收稿日期: 2021-03-08
出版日期: 2021-07-05
引用本文:
. [J]. 中国物理快报, 2021, 38(7): 76102-.
链接本文:
https://cpl.iphy.ac.cn/CN/10.1088/0256-307X/38/7/076102
或
https://cpl.iphy.ac.cn/CN/Y2021/V38/I7/76102
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2021, Vol. 38 
