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1.
Digital Simulation of Projective Non-Abelian Anyons with 68 Superconducting Qubits
Shibo Xu, Zheng-Zhi Sun, Ke Wang, Liang Xiang, Zehang Bao, Zitian Zhu, Fanhao Shen, Zixuan Song, Pengfei Zhang, Wenhui Ren, Xu Zhang, Hang Dong, Jinfeng Deng, Jiachen Chen, Yaozu Wu, Ziqi Tan, Yu Gao, Feitong Jin, Xuhao Zhu, Chuanyu Zhang, Ning Wang, Yiren Zou, Jiarun Zhong, Aosai Zhang, Weikang Li, Wenjie Jiang, Li-Wei Yu, Yunyan Yao, Zhen Wang, Hekang Li, Qiujiang Guo, Chao Song, H. Wang, and Dong-Ling Deng
中国物理快报 2023, 40 (
6
): 60301-060301. DOI: 10.1088/0256-307X/40/6/060301
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Non-Abelian anyons are exotic quasiparticle excitations hosted by certain topological phases of matter. They break the fermion-boson dichotomy and obey non-Abelian braiding statistics: their interchanges yield unitary operations, rather than merely a phase factor, in a space spanned by topologically degenerate wavefunctions. They are the building blocks of topological quantum computing. However, experimental observation of non-Abelian anyons and their characterizing braiding statistics is notoriously challenging and has remained elusive hitherto, in spite of various theoretical proposals. Here, we report an experimental quantum digital simulation of projective non-Abelian anyons and their braiding statistics with up to 68 programmable superconducting qubits arranged on a two-dimensional lattice. By implementing the ground states of the toric-code model with twists through quantum circuits, we demonstrate that twists exchange electric and magnetic charges and behave as a particular type of non-Abelian anyons, i.e., the Ising anyons. In particular, we show experimentally that these twists follow the fusion rules and non-Abelian braiding statistics of the Ising type, and can be explored to encode topological logical qubits. Furthermore, we demonstrate how to implement both single- and two-qubit logic gates through applying a sequence of elementary Pauli gates on the underlying physical qubits. Our results demonstrate a versatile quantum digital approach for simulating non-Abelian anyons, offering a new lens into the study of such peculiar quasiparticles.
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2.
A 700 W$\cdot$h$\cdot$kg$^{-1}$ Rechargeable Pouch Type Lithium Battery
Quan Li, Yang Yang, Xiqian Yu, and Hong Li
中国物理快报 2023, 40 (
4
): 48201-048201. DOI: 10.1088/0256-307X/40/4/048201
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High-energy-density rechargeable lithium batteries are being pursued by researchers because of their revolutionary potential nature. Current advanced practical lithium-ion batteries have an energy density of around 300 W$\cdot$h$\cdot$kg$^{-1}$. Continuing to increase the energy density of batteries to a higher level could lead to a major explosion development in some fields, such as electric aviation. Here, we have manufactured practical pouch-type rechargeable lithium batteries with both a gravimetric energy density of 711.3 W$\cdot$h$\cdot$kg$^{-1}$ and a volumetric energy density of 1653.65 W$\cdot$h$\cdot$L$^{-1}$. This is achieved through the use of high-performance battery materials including high-capacity lithium-rich manganese-based cathode and thin lithium metal anode with high specific energy, combined with extremely advanced process technologies such as high-loading electrode preparation and lean electrolyte injection. In this battery material system, the structural stability of cathode material in a widened charge/discharge voltage range and the deposition/dissolution behavior of interfacial modified thin lithium electrode are studied.
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3.
Giant Tunneling Magnetoresistance in Spin-Filter Magnetic Tunnel Junctions Based on van der Waals A-Type Antiferromagnet CrSBr
Guibin Lan, Hongjun Xu, Yu Zhang, Chen Cheng, Bin He, Jiahui Li, Congli He, Caihua Wan, Jiafeng Feng, Hongxiang Wei, Jia Zhang, Xiufeng Han, and Guoqiang Yu
中国物理快报 2023, 40 (
5
): 58501-058501. DOI: 10.1088/0256-307X/40/5/058501
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Two-dimensional van der Waals magnetic materials have demonstrated great potential for new-generation high-performance and versatile spintronic devices. Among them, magnetic tunnel junctions (MTJs) based on A-type antiferromagnets, such as CrI$_{3}$, possess record-high tunneling magnetoresistance (TMR) because of the spin filter effect of each insulating unit ferromagnetic layer. However, the relatively low working temperature and the instability of the chromium halides hinder applications of this system. Using a different technical scheme, we fabricated the MTJs based on an air-stable A-type antiferromagnet, CrSBr, and observed a giant TMR of up to 47000% at 5 K. Meanwhile, because of a relatively high Néel temperature of CrSBr, a sizable TMR of about 50% was observed at 130 K, which makes a big step towards spintronic devices at room temperature. Our results reveal the potential of realizing magnetic information storage in CrSBr-based spin-filter MTJs.
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4.
Gatemon Qubit Based on a Thin InAs-Al Hybrid Nanowire
Jierong Huo, Zezhou Xia, Zonglin Li, Shan Zhang, Yuqing Wang, Dong Pan, Qichun Liu, Yulong Liu, Zhichuan Wang, Yichun Gao, Jianhua Zhao, Tiefu Li, Jianghua Ying, Runan Shang, and Hao Zhang
中国物理快报 2023, 40 (
4
): 47302-047302. DOI: 10.1088/0256-307X/40/4/047302
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We study a gate-tunable superconducting qubit (gatemon) based on a thin InAs-Al hybrid nanowire. Using a gate voltage to control its Josephson energy, the gatemon can reach the strong coupling regime to a microwave cavity. In the dispersive regime, we extract the energy relaxation time $T_1\sim0.56$ µs and the dephasing time $T_2^* \sim0.38$ µs. Since thin InAs-Al nanowires can have fewer or single sub-band occupation and recent transport experiment shows the existence of nearly quantized zero-bias conductance peaks, our result holds relevancy for detecting Majorana zero modes in thin InAs-Al nanowires using circuit quantum electrodynamics.
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5.
Lithium Ion Batteries Operated at $-100\,^{\circ}\!$C
Jianli Gai, Jirong Yang, Wei Yang, Quan Li, Xiaodong Wu, and Hong Li
中国物理快报 2023, 40 (
8
): 86101-086101. DOI: 10.1088/0256-307X/40/8/086101
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Enabling lithium-ion batteries (LIBs) to operate in a wider temperature range, e.g., as low or high as possible or capable of both, is an urgent need and shared goal. Here we report, for the first time, a low-temperature electrolyte consisting of traditional ethylene carbonate, methyl acetate, butyronitrile solvents, and 1 M LiPF$_{6}$ salt, attributed to its very low freezing point ($T_{\rm f} = -126.3\,^{\circ}\!$C) and high ion conductivity at extremely low temperatures (0.21 mS/cm at $-100\,^{\circ}\!$C), successfully extends the service temperature of a practical 9.6 Ah LIB down to $-100\,^{\circ}\!$C (49.6% capacity retention compared to that at room temperature), which is the lowest temperature reported for practical cells so far as we know, and is lower than the lowest natural temperature ($-89.2\,^{\circ}\!$C) recorded on earth. Meanwhile, the high-temperature performance of lithium-ion batteries is not affected. The capacity retention is 88.2% and 83.4% after 800 cycles at 25$\,^{\circ}\!$C and 45$\,^{\circ}\!$C, respectively. The progress also makes LIB a proper power supplier for space vehicles in astronautic explorations.
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6.
Chiral Dirac Fermion in a Collinear Antiferromagnet
Ao Zhang, Ke Deng, Jieming Sheng, Pengfei Liu, Shiv Kumar, Kenya Shimada, Zhicheng Jiang, Zhengtai Liu, Dawei Shen, Jiayu Li, Jun Ren, Le Wang, Liang Zhou, Yoshihisa Ishikawa, Takashi Ohhara, Qiang Zhang, Garry McIntyre, Dehong Yu, Enke Liu, Liusuo Wu, Chaoyu Chen, and Qihang Liu
中国物理快报 2023, 40 (
12
): 126101-126101. DOI: 10.1088/0256-307X/40/12/126101
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In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, it is predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral “Dirac-like” fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Such an unconventional chiral fermion, protected by a hidden $SU(2)$ symmetry in the hierarchy of an enhanced crystallographic group, namely spin space group, is not experimentally verified yet. Here, by angle-resolved photoemission spectroscopy measurements, we reveal the surface origin of the electron pocket at the Fermi surface in collinear antiferromagnet CoNb$_{3}$S$_{6}$. Combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions. Our work provides spectral evidence of the chiral Dirac-like fermion caused by particular spin symmetry in CoNb$_{3}$S$_{6}$, paving an avenue for exploring new emergent phenomena in antiferromagnets with unconventional quasiparticle excitations.
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7.
Ultrafast Condensed Matter Physics at Attoseconds
Shi-Qi Hu and Sheng Meng
中国物理快报 2023, 40 (
11
): 117801-. DOI: 10.1088/0256-307X/40/11/117801
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Our understanding of how photons couple to different degrees of freedom in solids forms the bedrock of ultrafast physics and materials sciences. In this review, the emergent ultrafast dynamics in condensed matter at the attosecond timescale have been intensively discussed. In particular, the focus is put on recent developments of attosecond dynamics of charge, exciton, and magnetism. New concepts and indispensable role of interactions among multiple degrees of freedom in solids are highlighted. Applications of attosecond electronic metrology and future prospects toward attosecond dynamics in condensed matter are further discussed. These pioneering studies promise future development of advanced attosecond science and technology such as attosecond lasers, laser medical engineering, and ultrafast electronic devices.
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8.
High-Temperature Superconductivity in La$_3$Ni$_2$O$_7$
Kun Jiang, Ziqiang Wang, and Fu-Chun Zhang
中国物理快报 2024, 41 (
1
): 17402-017402. DOI: 10.1088/0256-307X/41/1/017402
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Motivated by the recent discovery of high-temperature superconductivity in bilayer La$_3$Ni$_2$O$_7$ under pressure, we study its electronic properties and superconductivity due to strong electron correlation. Using the inversion symmetry, we decouple the low-energy electronic structure into block-diagonal symmetric and antisymmetric sectors. It is found that the antisymmetric sector can be reduced to a one-band system near half filling, while the symmetric bands occupied by about two electrons are heavily overdoped individually. Using the strong coupling mean field theory, we obtain strong superconducting pairing with $B_{\rm 1g}$ symmetry in the antisymmetric sector. We propose that due to the spin-orbital exchange coupling between the two sectors, $B_{\rm 1g}$ pairing is induced in the symmetric bands, which in turn boosts the pairing gap in the antisymmetric band and enhances the high-temperature superconductivity with a congruent d-wave symmetry in pressurized La$_3$Ni$_2$O$_7$.
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9.
Optical Neural Network Architecture for Deep Learning with Temporal Synthetic Dimension
Bo Peng, Shuo Yan, Dali Cheng, Danying Yu, Zhanwei Liu, Vladislav V. Yakovlev, Luqi Yuan, and Xianfeng Chen
中国物理快报 2023, 40 (
3
): 34201-034201. DOI: 10.1088/0256-307X/40/3/034201
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The physical concept of synthetic dimensions has recently been introduced into optics. The fundamental physics and applications are not yet fully understood, and this report explores an approach to optical neural networks using synthetic dimension in time domain, by theoretically proposing to utilize a single resonator network, where the arrival times of optical pulses are interconnected to construct a temporal synthetic dimension. The set of pulses in each roundtrip therefore provides the sites in each layer in the optical neural network, and can be linearly transformed with splitters and delay lines, including the phase modulators, when pulses circulate inside the network. Such linear transformation can be arbitrarily controlled by applied modulation phases, which serve as the building block of the neural network together with a nonlinear component for pulses. We validate the functionality of the proposed optical neural network for the deep learning purpose with examples handwritten digit recognition and optical pulse train distribution classification problems. This proof of principle computational work explores the new concept of developing a photonics-based machine learning in a single ring network using synthetic dimensions, which allows flexibility and easiness of reconfiguration with complex functionality in achieving desired optical tasks.
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10.
Lu–H–N Phase Diagram from First-Principles Calculations
Fankai Xie, Tenglong Lu, Ze Yu, Yaxian Wang, Zongguo Wang, Sheng Meng, and Miao Liu
中国物理快报 2023, 40 (
5
): 57401-057401. DOI: 10.1088/0256-307X/40/5/057401
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Employing a comprehensive structure search and high-throughput first-principles calculation method on 1561 compounds, the present study reveals the phase diagram of Lu–H–N. In detail, the formation energy landscape of Lu–H–N is derived and utilized to assess the thermodynamic stability of each compound that is created via element substitution. The result indicates that there is no stable ternary structure in the Lu–H–N chemical system, however, metastable ternary structures, such as Lu$_{20}$H$_{2}$N$_{17}$ $(C2/m)$ and Lu$_{2}$H$_{2}$N ($P\bar{3}m1$), are observed to have small $E_{\rm hull}$ ($ < 100$ meV/atom). It is also found that the energy convex hull of the Lu–H–N system shifts its shape when applying hydrostatic pressure up to 10 GPa, and the external pressure stabilizes a couple of binary phases such as LuN$_{9}$ and Lu$_{10}$H$_{21}$. Additionally, interstitial voids in LuH$_{2}$ are observed, which may explain the formation of Lu$_{10}$H$_{21}$ and LuH$_{3-\delta}$N$_{\epsilon}$. To provide a basis for comparison, x-ray diffraction patterns and electronic structures of some compounds are also presented.
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11.
Electron-Exciton Coupling in 1T-TiSe$_{2}$ Bilayer
Li Zhu, Wei-Min Zhao, Zhen-Yu Jia, Huiping Li, Xuedong Xie, Qi-Yuan Li, Qi-Wei Wang, Li-Guo Dou, Ju-Gang Hu, Yi Zhang, Wenguang Zhu, Shun-Li Yu, Jian-Xin Li, and Shao-Chun Li
中国物理快报 2023, 40 (
5
): 57101-057101. DOI: 10.1088/0256-307X/40/5/057101
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Excitons in solid state are bosons generated by electron-hole pairs as the Coulomb screening is sufficiently reduced. The exciton condensation can result in exotic physics such as super-fluidity and insulating state. In charge density wave (CDW) state, 1T-TiSe$_{2}$ is one of the candidates that may host the exciton condensation. However, to envision its excitonic effect is still challenging, particularly at the two-dimensional limit, which is applicable to future devices. Here, we realize the epitaxial 1T-TiSe$_{2}$ bilayer, the two-dimensional limit for its $2 \times 2\times 2$ CDW order, to explore the exciton-associated effect. By means of high-resolution scanning tunneling spectroscopy and quasiparticle interference, we discover an unexpected state residing below the conduction band and right within the CDW gap region. As corroborated by our theoretical analysis, this mysterious phenomenon is in good agreement with the electron-exciton coupling. Our study provides a material platform to explore exciton-based electronics and opto-electronics.
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12.
A High-Randomness and High-Stability Electronic Quantum Random Number Generator without Post Processing
Yu-Xuan Liu, Ke-Xin Huang, Yu-Ming Bai, Zhe Yang, and Jun-Lin Li
中国物理快报 2023, 40 (
7
): 70303-070303. DOI: 10.1088/0256-307X/40/7/070303
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Random numbers are one of the key foundations of cryptography. This work implements a discrete quantum random number generator (QRNG) based on the tunneling effect of electrons in an avalanche photo diode. Without any post-processing and conditioning, this QRNG can output raw sequences at a rate of 100 Mbps. Remarkably, the statistical min-entropy of the 8,000,000 bits sequence reaches 0.9944 bits/bit, and the min-entropy validated by NIST SP 800-90B reaches 0.9872 bits/bit. This metric is currently the highest value we have investigated for QRNG raw sequences. Moreover, this QRNG can continuously and stably output raw sequences with high randomness over extended periods. The system produced a continuous output of 1,174 Gbits raw sequence for a duration of 11,744 s, with every 8 Mbits forming a unit to obtain a statistical min-entropy distribution with an average value of 0.9892 bits/bit. The statistical min-entropy of all data (1,174 Gbits) achieves the value of 0.9951 bits/bit. This QRNG can produce high-quality raw sequences with good randomness and stability. It has the potential to meet the high demand in cryptography for random numbers with high quality.
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13.
Pressure-Induced Color Change in the Lutetium Dihydride LuH$_{2}$
Pengfei Shan, Ningning Wang, Xiquan Zheng, Qingzheng Qiu, Yingying Peng, and Jinguang Cheng
中国物理快报 2023, 40 (
4
): 46101-046101. DOI: 10.1088/0256-307X/40/4/046101
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The lutetium dihydride LuH$_{2}$ is stable at ambient conditions. Here we show that its color undergoes sequential changes from dark blue at ambient pressure to pink at $\sim$ $2.2$ GPa and then to bright red at $\sim$ $4$ GPa upon compression in a diamond anvil cell. Such a pressure-induced color change in LuH$_{2}$ is reversible and it is very similar to that recently reported in the N-doped lutetium hydride [
Nature
615
, 244 (2023)
]. However, our preliminary resistance measurements on LuH$_{2}$ under pressures up to $\sim$ $7$ GPa evidenced no superconductivity down to 1.5 K.
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14.
Flat Band and $\mathbb{Z}_2$ Topology of Kagome Metal
CsTi$_{3}$Bi$_{5}$
Yuan Wang, Yixuan Liu, Zhanyang Hao, Wenjing Cheng, Junze Deng, Yuxin Wang, Yuhao Gu, Xiao-Ming Ma, Hongtao Rong, Fayuan Zhang, Shu Guo, Chengcheng Zhang, Zhicheng Jiang, Yichen Yang, Wanling Liu, Qi Jiang, Zhengtai Liu, Mao Ye, Dawei Shen, Yi Liu, Shengtao Cui, Le Wang, Cai Liu, Junhao Lin, Ying Liu, Yongqing Cai, Jinlong Zhu, Chaoyu Chen, and Jia-Wei Mei
中国物理快报 2023, 40 (
3
): 37102-. DOI: 10.1088/0256-307X/40/3/037102
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The simple kagome-lattice band structure possesses Dirac cones, flat band, and saddle point with van Hove singularities in the electronic density of states, facilitating the emergence of various electronic orders. Here we report a titanium-based kagome metal CsTi$_{3}$Bi$_{5}$ where titanium atoms form a kagome network, resembling its isostructural compound CsV$_{3}$Sb$_{5}$. Thermodynamic properties including the magnetization, resistance, and heat capacity reveal the conventional Fermi liquid behavior in the kagome metal CsTi$_{3}$Bi$_{5}$ and no signature of superconducting or charge density wave (CDW) transition anomaly down to 85 mK. Systematic angle-resolved photoemission spectroscopy measurements reveal multiple bands crossing the Fermi level, consistent with the first-principles calculations. The flat band formed by the destructive interference of hopping in the kagome lattice is observed directly. Compared to CsV$_{3}$Sb$_{5}$, the van Hove singularities are pushed far away above the Fermi level in CsTi$_{3}$Bi$_{5}$, in line with the absence of CDW. Furthermore, the first-principles calculations identify the nontrivial $\mathbb{Z}_2$ topological properties for those bands crossing the Fermi level, accompanied by several local band inversions. Our results suppose CsTi$_{3}$Bi$_{5}$ as a complementary platform to explore the superconductivity and nontrivial band topology.
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15.
Dark Korteweg–De Vrise System and Its Higher-Dimensional Deformations
Si-Yu Zhu, De-Xing Kong, and Sen-Yue Lou
中国物理快报 2023, 40 (
8
): 80201-. DOI: 10.1088/0256-307X/40/8/080201
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The new dimensional deformation approach is proposed to generate higher-dimensional analogues of integrable systems. An arbitrary ($K$+1)-dimensional integrable Korteweg–de Vries (KdV) system, as an example, exhibiting symmetry, is illustrated to arise from a reconstructed deformation procedure, starting with a general symmetry integrable (1+1)-dimensional dark KdV system and its conservation laws. Physically, the dark equation systems may be related to dark matter physics. To describe nonlinear physics, both linear and nonlinear dispersions should be considered. In the original lower-dimensional integrable systems, only liner or nonlinear dispersion is included. The deformation algorithm naturally makes the model also include the linear dispersion and nonlinear dispersion.
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16.
High-Temperature Superconductivity in Doped Boron Clathrates
Liang Ma, Lingrui Wang, Yifang Yuan, Haizhong Guo, and Hongbo Wang
中国物理快报 2023, 40 (
8
): 86201-086201. DOI: 10.1088/0256-307X/40/8/086201
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The recent discoveries of near-room-temperature superconductivity in clathrate hydrides present compelling evidence for the reliability of theory-orientated conventional superconductivity. Nevertheless, the harsh pressure conditions required to maintain such high $T_{\rm c}$ limit their practical applications. To address this challenge, we conducted extensive first-principles calculations to investigate the doping effect of the recently synthesized LaB$_{8}$ clathrate, intending to design high-temperature superconductors at ambient pressure. Our results demonstrate that these clathrates are highly promising for high-temperature superconductivity owing to the coexistence of rigid boron covalent networks and the tunable density of states at the Fermi level. Remarkably, the predicted $T_{\rm c}$ of BaB$_{8}$ could reach 62 K at ambient pressure, suggesting a significant improvement over the calculated $T_{\rm c}$ of 14 K in LaB$_{8}$. Moreover, further calculations of the formation enthalpies suggest that BaB$_{8}$ could be potentially synthesized under high-temperature and high-pressure conditions. These findings highlight the potential of doped boron clathrates as promising superconductors and provide valuable insights into the design of light-element clathrate superconductors.
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17.
Superconductivity Observed in Tantalum Polyhydride at High Pressure
X. He, C. L. Zhang, Z. W. Li, S. J. Zhang, B. S. Min, J. Zhang, K. Lu, J. F. Zhao, L. C. Shi, Y. Peng, X. C. Wang, S. M. Feng, J. Song, L. H. Wang, V. B. Prakapenka, S. Chariton, H. Z. Liu, and C. Q. Jin
中国物理快报 2023, 40 (
5
): 57404-057404. DOI: 10.1088/0256-307X/40/5/057404
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We report experimental discovery of tantalum polyhydride superconductor. It was synthesized under high-pressure and high-temperature conditions using diamond anvil cell combined with
in situ
high-pressure laser heating techniques. The superconductivity was investigated via resistance measurements at pressures. The highest superconducting transition temperature $T_{\rm c}$ was found to be $\sim$ $30$ K at 197 GPa in the sample that was synthesized at the same pressure with $\sim$ $2000$ K heating. The transitions are shifted to low temperature upon applying magnetic fields that support the superconductivity nature. The upper critical field at zero temperature $\mu_{0}H_{\rm c2}$(0) of the superconducting phase is estimated to be $\sim$ $20$ T that corresponds to Ginzburg–Landau coherent length $\sim$ $40$ Å. Our results suggest that the superconductivity may arise from $I\bar{4}3d$ phase of TaH$_{3}$. It is, for the first time to our best knowledge, experimental realization of superconducting hydrides for the VB group of transition metals.
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18.
Light-Induced Phonon-Mediated Magnetization in Monolayer MoS$_{2}$
Shengjie Zhang, Yufei Pei, Shiqi Hu, Na Wu, Da-Qiang Chen, Chao Lian, and Sheng Meng
中国物理快报 2023, 40 (
7
): 77502-077502. DOI: 10.1088/0256-307X/40/7/077502
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Light-induced ultrafast spin dynamics in materials is of great importance for developments of spintronics and magnetic storage technology. Recent progresses include ultrafast demagnetization, magnetic switching, and magnetic phase transitions, while the ultrafast generation of magnetism is hardly achieved. Here, a strong light-induced magnetization (up to $0.86\mu_{\scriptscriptstyle{\rm B}}$ per formula unit) is identified in non-magnetic monolayer molybdenum disulfide (MoS$_{2}$). With the state-of-the-art time-dependent density functional theory simulations, we demonstrate that the out-of-plane magnetization can be induced by circularly polarized laser, where chiral phonons play a vital role. The phonons strongly modulate spin-orbital interactions and promote electronic transitions between the two conduction band states, achieving an effective magnetic field $\sim$ $380$ T. Our study provides important insights into the ultrafast magnetization and spin-phonon coupling dynamics, facilitating effective light-controlled valleytronics and magnetism.
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19.
Emergence of High-Temperature Superconducting Phase in Pressurized La$_{3}$Ni$_{2}$O$_7$ Crystals
Jun Hou, Peng-Tao Yang, Zi-Yi Liu, Jing-Yuan Li, Peng-Fei Shan, Liang Ma, Gang Wang, Ning-Ning Wang, Hai-Zhong Guo, Jian-Ping Sun, Yoshiya Uwatoko, Meng Wang, Guang-Ming Zhang, Bo-Sen Wang, and Jin-Guang Cheng
中国物理快报 2023, 40 (
11
): 117302-. DOI: 10.1088/0256-307X/40/11/117302
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The recent report of pressure-induced structural transition and signature of superconductivity with $T_{\rm c}\approx80$ K above 14 GPa in La$_{3}$Ni$_{2}$O$_{7}$ crystals has garnered considerable attention. To further elaborate this discovery, we carried out comprehensive resistance measurements on La$_{3}$Ni$_{2}$O$_{7}$ crystals grown in an optical-image floating zone furnace under oxygen pressure (15 bar) using a diamond anvil cell (DAC) and cubic anvil cell (CAC), which employ a solid (KBr) and liquid (glycerol) pressure-transmitting medium, respectively. Sample 1 measured in the DAC exhibits a semiconducting-like behavior with large resistance at low pressures and gradually becomes metallic upon compression. At pressures $P \geqslant13.7$ GPa we observed the appearance of a resistance drop of as much as $\sim$ 50% around 70 K, which evolves into a kink-like anomaly at pressures above 40 GPa and shifts to lower temperatures gradually with increasing magnetic field. These observations are consistent with the recent report mentioned above. On the other hand, sample 2 measured in the CAC retains metallic behavior in the investigated pressure range up to 15 GPa. The hump-like anomaly in resistance around $\sim$ 130 K at ambient pressure disappears at $P\geqslant2$ GPa. In the pressure range of 11–15 GPa we observed the gradual development of a shoulder-like anomaly in resistance at low temperatures, which evolves into a pronounced drop of resistance of 98% below 62 K at 15 GPa, reaching a temperature-independent resistance of 20 $µ \Omega$ below 20 K. Similarly, this resistance anomaly can be progressively shifted to lower temperatures by applying external magnetic fields, resembling a typical superconducting transition. Measurements on sample 3 in the CAC reproduce the resistance drop at pressures above 10 GPa and realize zero resistance below 10 K at 15 GPa even though an unusual semiconducting-like behavior is retained in the normal state. Based on these results, we constructed a dome-shaped superconducting phase diagram and discuss some issues regarding the sample-dependent behaviors on pressure-induced high-temperature superconductivity in the La$_{3}$Ni$_{2}$O$_{7}$ crystals.
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20.
Hydrothermally Obtaining Superconductor Single Crystal of FeSe$_{0.2}$Te$_{0.8}$ without Interstitial Fe
Sheng Ma, Shanshan Yan, Jiali Liu, Yizhe Wang, Yuhang Zhang, Zhen Zhao, Zouyouwei Lu, Dong Li, Yue Liu, Jihu Lu, Hua Zhang, Haitao Yang, Fang Zhou, Zian, Li, Xiaoli Dong, and Zhongxian Zhao
中国物理快报 2023, 40 (
6
): 67402-. DOI: 10.1088/0256-307X/40/6/067402
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We report a hydrothermal route to remove interstitial excess Fe in non-superconducting iron chalcogenide Fe$_{1+\delta}$Se$_{1-x}$Te$_{x}$ single crystals. The extra-Fe-free ($\delta \sim 0$) FeSe$_{0.2}$Te$_{0.8}$ single crystal thus obtained shows bulk superconductivity at $T_{\rm c} \sim 13.8$ K, which is about 2 K higher than the FeSe$_{0.2}$Te$_{0.8}$ sample obtained by usual post-annealing process. The upper critical field $\mu_{0}H_{\rm c2}$ is estimated to be $\sim$ $42.5$ T, similar to the annealed FeSe$_{0.2}$Te$_{0.8}$. It is surprising to find that the hydrothermal FeSe$_{0.2}$Te$_{0.8}$ exhibits a remarkably small isothermal magnetization hysteresis loop at $T = 3$ K. This yields an extremely low critical current density $J_{\rm c} \sim 1.1\times 10^{2}$ A$\cdot$cm$^{-2}$ (over 100 times smaller than the annealed FeSe$_{0.2}$Te$_{0.8}$) and indicates more free vortices in the hydrothermal FeSe$_{0.2}$Te$_{0.8}$.
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21.
Quantum Anomalous Hall Effects Controlled by Chiral Domain Walls
Qirui Cui, Jinghua Liang, Yingmei Zhu, Xiong Yao, and Hongxin Yang
中国物理快报 2023, 40 (
3
): 37502-. DOI: 10.1088/0256-307X/40/3/037502
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We report the interplay between two different topological phases in condensed matter physics, the magnetic chiral domain wall (DW), and the quantum anomalous Hall (QAH) effect. It is shown that the chiral DW driven by Dzyaloshinskii–Moriya interaction can divide the uniform domain into several zones where the neighboring zone possesses opposite quantized Hall conductance. The separated domain with a chiral edge state (CES) can be continuously modified by external magnetic field-induced domain expansion and thermal fluctuation, which gives rise to the reconfigurable QAH effect. More interestingly, we show that the position of CES can be tuned by spin current driven chiral DW motion. Several two-dimensional magnets with high Curie temperature and large topological band gaps are proposed for realizing these phenomena. The present work thus reveals the possibility of chiral DW controllable QAH effects.
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22.
Empirical Determination of the Pion Mass Distribution
Y.-Z. Xu, K. Raya, Z.-F. Cui, C. D. Roberts, and J. Rodríguez-Quintero
中国物理快报 2023, 40 (
4
): 41201-041201. DOI: 10.1088/0256-307X/40/4/041201
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Existing pion+nucleus Drell-Yan and electron+pion scattering data are used to develop ensembles of model-independent representations of the pion generalized parton distribution (GPD). Therewith, one arrives at a data-driven prediction for the pion mass distribution form factor, $\theta_2^\pi $. Compared with the pion elastic electromagnetic form factor, $\theta_2^\pi$ is harder: the ratio of the radii derived from these two form factors is $r_\pi^{\theta_2}/r_\pi = 0.79(3)$. Our data-driven predictions for the pion GPD, related form factors and distributions should serve as valuable constraints on theories of pion structure.
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23.
Correlation Renormalized and Induced Spin-Orbit Coupling
Kun Jiang
中国物理快报 2023, 40 (
1
): 17102-. DOI: 10.1088/0256-307X/40/1/017102
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Interplay of spin-orbit coupling (SOC) and electron correlation generates a bunch of emergent quantum phases and transitions, especially topological insulators and topological transitions. We find that electron correlation will induce extra large SOC in multi-orbital systems under atomic SOC and change ground state topological properties. Using the Hartree–Fock mean field theory, phase diagrams of $p_{x}/p_{y}$ orbital ionic Hubbard model on honeycomb lattice are well studied. In general, correction of strength of SOC $\delta \lambda \propto (U'-J)$. Due to breaking down of rotation symmetry, form of SOC on multi-orbital materials is also changed under correlation. If a non-interacting system is close to fermionic instability, spontaneous generalized SOC can also be found. Using renormalization group, SOC is leading instability close to quadratic band-crossing point. Mean fields at quadratic band-crossing point are also studied.
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24.
Higher Dimensional Camassa–Holm Equations
S. Y. Lou, Man Jia, and Xia-Zhi Hao
中国物理快报 2023, 40 (
2
): 20201-. DOI: 10.1088/0256-307X/40/2/020201
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Utilizing some conservation laws of the (1+1)-dimensional Camassa–Holm (CH) equation and/or its reciprocal forms, some (n+1)-dimensional CH equations for $n\geq 1$ are constructed by a modified deformation algorithm. The Lax integrability can be proven by applying the same deformation algorithm to the Lax pair of the (1+1)-dimensional CH equation. A novel type of peakon solution is implicitly given and expressed by the LambertW function.
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25.
Low-Temperature Aqueous Na-Ion Batteries: Strategies and Challenges of Electrolyte Design
Qiubo Guo, Shuai Han, Yaxiang Lu, Liquan Chen, and Yong-Sheng Hu
中国物理快报 2023, 40 (
2
): 28801-. DOI: 10.1088/0256-307X/40/2/028801
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Aqueous Na-ion batteries (ANIBs) are considered to be promising secondary battery systems for grid-scale energy storage applications and have attracted widespread attention due to their unique merits of rich resources of Na, as well as the inherent safety and low cost of aqueous electrolytes. However, the narrow electrochemical stability widow and high freezing point of traditional dilute aqueous electrolytes restrict their multi-scenario applications. Considering the charge-storage mechanism of ANIBs, the optimization and design of aqueous Na-based electrolytes dominate their low-temperature performance, which is also hot off the press in this field. In this review, we first systematically comb the research progress of the novel electrolytes and point out their remaining challenges in ANIBs. Then our perspectives on how to further improve the low-temperature performance of ANIBs will also be discussed. Finally, this review briefly sheds light on the potential direction of low-temperature ANIBs, which would guide the future design of high-performance aqueous rechargeable batteries.
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26.
Engineering Interlayer Hybridization in Energy Space via Dipolar Overlayers
Bin Shao, Xiao Jiang, Jan Berges, Sheng Meng, and Bing Huang
中国物理快报 2023, 40 (
8
): 87303-087303. DOI: 10.1088/0256-307X/40/8/087303
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The interlayer hybridization (IH) of van der Waals (vdW) materials is thought to be mostly associated with the unignorable interlayer overlaps of wavefunctions ($t$) in real space. Here, we develop a more fundamental understanding of IH by introducing a new physical quantity, the IH admixture ratio $\alpha$. Consequently, an exotic strategy of IH engineering in energy space can be proposed, i.e., instead of changing $t$ as commonly used, $\alpha$ can be effectively tuned in energy space by changing the on-site energy difference (${2\varDelta}$) between neighboring-layer states. In practice, this is feasible via reshaping the electrostatic potential of the surface by deposing a dipolar overlayer, e.g., crystalline ice. Our first-principles calculations unveil that IH engineering via adjusting ${2\varDelta}$ can greatly tune interlayer optical transitions in transition-metal dichalcogenide bilayers, switch different types of Dirac surface states in Bi$_{2}$Se$_{3}$ thin films, and control magnetic phase transition of charge density waves in 1H/1T-TaS$_{2}$ bilayers, opening new opportunities to govern the fundamental optoelectronic, topological, and magnetic properties of vdW systems beyond the traditional interlayer distance or twisting engineering.
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27.
Signature of Superconductivity in Pressurized La$_{4}$Ni$_{3}$O$_{10}$
Qing Li, Ying-Jie Zhang, Zhe-Ning Xiang, Yuhang Zhang, Xiyu Zhu, and Hai-Hu Wen
中国物理快报 2024, 41 (
1
): 17401-. DOI: 10.1088/0256-307X/41/1/017401
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The discovery of high-temperature superconductivity near 80 K in bilayer nickelate La$_{3}$Ni$_{2}$O$_{7}$ under high pressures has renewed the exploration of superconducting nickelate in bulk materials. The extension of superconductivity in other nickelates in a broader family is also essential. Here, we report the experimental observation of superconducting signature in trilayer nickelate La$_{4}$Ni$_{3}$O$_{10}$ under high pressures. By using a modified sol-gel method and post-annealing treatment under high oxygen pressure, we successfully obtained polycrystalline La$_{4}$Ni$_{3}$O$_{10}$ samples with different transport behaviors at ambient pressure. Then we performed high-pressure electrical resistance measurements on these samples in a diamond-anvil-cell apparatus. Surprisingly, the signature of possible superconducting transition with a maximum transition temperature ($T_{\rm c}$) of about 20 K under high pressures is observed, as evidenced by a clear drop of resistance and the suppression of resistance drops under magnetic fields. Although the resistance drop is sample-dependent and relatively small, it appears in all of our measured samples. We argue that the observed superconducting signal is most likely to originate from the main phase of La$_{4}$Ni$_{3}$O$_{10}$. Our findings will motivate the exploration of superconductivity in a broader family of nickelates and shed light on the understanding of the underlying mechanisms of high-$T_{\rm c}$ superconductivity in nickelates.
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28.
Electron-Correlation-Induced Charge Density Wave in FeGe
Lin Wu, Yating Hu, Dongze Fan, Di Wang, and Xiangang Wan
中国物理快报 2023, 40 (
11
): 117103-117103. DOI: 10.1088/0256-307X/40/11/117103
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As the first magnetic kagome material to exhibit the charge density wave (CDW) order, FeGe has attracted much attention in recent research. Similar to $A$V$_{3}$Sb$_{5}$ ($A$ = K, Cs, Rb), FeGe exhibits the CDW pattern with an in-plane 2$\times$2 structure and the existence of van Hove singularities near the Fermi level. However, sharply different from $A$V$_{3}$Sb$_{5}$ which has phonon instability at $M$ point, all the theoretically calculated phonon frequencies in FeGe remain positive. Based on first-principles calculations, we surprisingly find that the maximum of nesting function is at $K$ point instead of $M$ point. Two Fermi pockets with Fe-$d_{xz}$ and Fe-$d_{x^{2}-y^{2}}$/$d_{xy}$ orbital characters have large contribution to the Fermi nesting, which evolve significantly with $k_{z}$, indicating the highly three-dimensional (3D) feature of FeGe in contrast to $A$V$_{3}$Sb$_{5}$. Considering the effect of local Coulomb interaction, we reveal that the instability at $K$ point is significantly suppressed due to the sublattice interference mechanism. Meanwhile, the wave functions nested by vector $M$ have many ingredients located at the same Fe site, thus the instability at $M$ point is enhanced. This indicates that the electron correlation, rather than electron-phonon interaction, plays a key role in the CDW transition at $M$ point.
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29.
Magnetic-Field-Induced Sign Changes of Thermal Expansion in DyCrO$_{4}$
Jin-Cheng He, Zhao Pan, Dan Su, Xu-Dong Shen, Jie Zhang, Da-Biao Lu, Hao-Ting Zhao, Jun-Zhuang Cong, En-Ke Liu, You-Wen Long, and Young Sun
中国物理快报 2023, 40 (
6
): 66501-066501. DOI: 10.1088/0256-307X/40/6/066501
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The anharmonicity of lattice vibration is mainly responsible for the coefficient of thermal expansion (CTE) of materials. External stimuli, such as magnetic and electric fields, thus cannot effectively change the CTE, much less the sign variation from positive to negative or vice versa. In this study, we report significant magnetic field effects on the CTE of zircon- and scheelite-type DyCrO$_{4}$ prepared at ambient and high pressures, respectively. At zero field, the zircon-type DyCrO$_{4}$ exhibits a negative CTE below the ferromagnetic-order temperature of 23 K. With increasing field up to $\ge $1.0 T, however, the sign of the CTE changes from negative to positive. In the scheelite phase, magnetic field can change the initially positive CTE to be negative with a field up to 2.0 T, and then a reentrant positive CTE is induced by enhanced fields $\ge $3.5 T. Both zircon and scheelite phases exhibit considerable magnetostrictive effects with the absolute values as high as $\sim$ $800$ ppm at 2 K and 10 T. The strong spin–lattice coupling is discussed to understand the unprecedented sign changes of the CTE caused by applying magnetic fields. The current DyCrO$_{4}$ provides the first example of field-induced sign change of thermal expansion, opening up a way to readily control the thermal expansion beyond the conventional chemical substitution.
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30.
Augmenting Density Matrix Renormalization Group with Disentanglers
Xiangjian Qian and Mingpu Qin
中国物理快报 2023, 40 (
5
): 57102-057102. DOI: 10.1088/0256-307X/40/5/057102
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Density matrix renormalization group (DMRG) and its extensions in the form of matrix product states are arguably the choice for the study of one-dimensional quantum systems in the last three decades. However, due to the limited entanglement encoded in the wave-function ansatz, to maintain the accuracy of DMRG with the increase of the system size in the study of two-dimensional systems, exponentially increased resources are required, which limits the applicability of DMRG to only narrow systems. We introduce a new ansatz in which DMRG is augmented with disentanglers to encode area-law-like entanglement entropy (entanglement entropy supported in the new ansatz scales as $l$ for an $l \times l$ system). In the new method, the $O(D^3)$ low computational cost of DMRG is kept (with an overhead of $O(d^4)$ and $d$ the dimension of the physical degrees of freedom). We perform benchmark calculations with this approach on the two-dimensional transverse Ising and Heisenberg models. This new ansatz extends the power of DMRG in the study of two-dimensional quantum systems.
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