Lower Exciton Number Strong Light Matter Interaction in Plasmonic Tweezers

The plasmonic nanocavity is an excellent platform for the study of light matter interaction within a sub-diffraction volume under ambient conditions. We design a structure of plasmonic tweezers, which can trap molecular J-aggregates and also serve as a plasmonic cavity with which to investigate strong light matter interaction. The optical response of the cavity is calculated via finite-difference time-domain methods, and the optical force is evaluated based on the Maxwell stress tensor method. With the help of the coupled oscillator model and virtual exciton theory, we investigate the strong coupling progress at the lower level of excitons, finding that a Rabi splitting of 230 meV can be obtained in a single exciton system. We further analyze the relationship between optical force and model volume in the coupling system. The proposed method offers a way to locate molecular J-aggregates in plasmonic tweezers for investigating optical force performance and strong light matter interaction.