Double Resonance Raman Scattering in Single-Layer MoSe_2 under Moderate Pressure

Jian-mei Li; Yi-kun Yao; Li-huan Sun; Xin-yan Shan; Cong Wang; Xing-hua Lu

doi:10.1088/0256-307X/36/4/048201

Double Resonance Raman Scattering in Single-Layer MoSe $_{2}$ under Moderate Pressure

¹Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190
²School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100190
³Center for Excellence in Topological Quantum Computation, Beijing 100190
⁴Songshan Lake Materials Laboratory, Dongguan 523808
⁵School of Physics & Mathematical Sciences, Nanyang Technological University, Singapore 639798, Singapore

Funds: Supported by the Strategic Priority Research Program (B) of the Chinese Academy of Sciences under Grant Nos XDB30000000, XDB28000000 and XDB07030100, the National Natural Science Foundation of China under Grant Nos 11774395, 11727902 and 91753136, and the Beijing Natural Science Foundation under Grant No 4181003.

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Received Date: December 03, 2018

Published Date: March 31, 2019

Abstract

Abstract

Pressure-dependent properties in layered transition-dichalcogenides are important for our understanding of their basic structures and applications. We investigate the electronic structure in MoSe $_{2}$ monolayer under external pressure up to 5.73 GPa by Raman spectroscopy and photoluminescence (PL) spectroscopy. The double resonance out-of-plane acoustic mode ( $2ZA$ ) phonon is observed in Raman spectroscopy near 250 cm $^{-1}$ , which presents pronounced intensity and pressure dependence. Significant variation in $2ZA$ peak intensity under different pressures reflects the change in electronic band structure as pressure varies, which is consistent with the blue shift in PL spectroscopy. The high sensitivity in both Raman and PL spectroscopy under moderate pressure in such a two-dimensional material may have many advantages for optoelectronic applications.

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Double Resonance Raman Scattering in Single-Layer MoSe $_{2}$ under Moderate Pressure

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Double Resonance Raman Scattering in Single-Layer MoSe $_{2}$ under Moderate Pressure