Observation of Rydberg Series in Sodium Vapor by Two-Photon Resonant Nondegenerate Four-Wave Mixing

  • Published Date: August 31, 2001
  • We apply two-photon resonant nondegenerate four-wave mixing
    with a resonant intermediate state for the observation of Rydberg states in sodium vapor. The broadening and shift of the sodium 3S -11D transition perturbed by argon are investigated. This technique can achieve Doppler-free resolution of narrow spectral structures of Rydberg levels if lasers with narrow bandwidths are employed.
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