Charge imprinting biases topology of correlated insulator in hBN-aligned rhombohedral multilayer graphene

  • Rhombohedral multilayer graphene aligned with hexagonal boron nitride (RMG-hBN) hosts correlated Chern phases, but the microscopic role of hBN stacking remains unclear, especially when the active carriers are displaced away from the moiré interface. Using Hartree-Fock calculations over layer numbers, twist angles, displacement fields, fillings, and hBN alignments, we show that correlated insulators are most robust at small twist angles and intermediate layer number (N ≃ 6), where bandwidth suppression is balanced by layer delocalization of the wavefunctions of the active carriers. Under moiré-distant conditions at filling ν = 1, the topology of the insulating state is strongly biased by charge imprinting: the hBN alignment shapes the occupied valence-band charge texture near the interface via moiré potential, which acts through long-range Coulomb interactions as a remote electrostatic template for doped conduction electrons. Depending on the alignment, this template favors either triangular charge localization associated with trivial insulators or honeycomb-like charge networks compatible with Chern insulators. Our results identify valence-band charge textures as a microscopic route by which a remote moiré interface controls correlated topology in multilayer graphene.
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