Pressure Driven Structural Evolutions of 0.935(Na_0.5Bi_0.5)TiO_3-0.065BaTiO_3 Lead-Free Ferroelectric Single Crystal through Raman Spectroscopy

Qunfei Zheng; Qiang Li; Saidong Xue; Yanhui Wu; Lijuan Wang; Qian Zhang; Xiaomei Qin; Xiangyong Zhao; Feifei Wang; Wenge Yang

doi:10.1088/0256-307X/38/2/026102

Pressure Driven Structural Evolutions of 0.935(Na $_{0.5}$ Bi $_{0.5}$ )TiO $_{3}$ -0.065BaTiO $_{3}$ Lead-Free Ferroelectric Single Crystal through Raman Spectroscopy

¹Department of Physics, Mathematics & Science College, Shanghai Normal University, Shanghai 200234, China
²Center for High Pressure Science and Technology Advanced Research (HPSTAR), Beijing 100094, China
³Center for High Pressure Science and Technology Advanced Research (HPSTAR), Shanghai 201203, China
⁴Academy for Advanced Interdisciplinary Studies, Shenzhen Engineering Research Center for Frontier Materials Synthesis at High Pressures, Southern University of Science and Technology (SUSTech), Shenzhen 518055, China

Funds: Supported by the National Natural Science Foundation of China (Grant Nos. 11674231, 11974250, and 51772192), the Science and Technology Commission of Shanghai Municipality (Grant Nos. 17070502700 and 19070502800), and the Shenzhen Development and Reform Commission Foundation for Shenzhen Engineering Research Center for Frontier Materials Synthesis at High Pressures.

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Received Date: November 15, 2020

Published Date: January 31, 2021

Abstract

Abstract

Pressure evolution of local structure and vibrational dynamics of the perovskite-type relaxor ferroelectric single crystal of 0.935(Na $_{0.5}$ Bi $_{0.5}$ )TiO $_{3}$ -0.065BaTiO $_{3}$ (NBT-6.5BT) is systematically investigated via in situ Raman spectroscopy. The pressure dependence of phonon modes up to 30 GPa reveals two characteristic pressures: one is at around 4.6 GPa which corresponds to the rhombohedral-to-tetragonal phase transition, showing that the pressure strongly suppresses the coupling between the off-centered A- and B-site cations; the other structural transition involving the oxygen octahedral tilt and vibration occurs at pressure $\sim$ 13–15 GPa with certain degree of order-disorder transition, evidenced by the abnormal changes of intensity and FWHM in Raman spectrum.

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Pressure Driven Structural Evolutions of 0.935(Na $_{0.5}$ Bi $_{0.5}$ )TiO $_{3}$ -0.065BaTiO $_{3}$ Lead-Free Ferroelectric Single Crystal through Raman Spectroscopy

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Pressure Driven Structural Evolutions of 0.935(Na0.5_{0.5}Bi0.5_{0.5})TiO3_{3}-0.065BaTiO3_{3} Lead-Free Ferroelectric Single Crystal through Raman Spectroscopy

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Pressure Driven Structural Evolutions of 0.935(Na $_{0.5}$ Bi $_{0.5}$ )TiO $_{3}$ -0.065BaTiO $_{3}$ Lead-Free Ferroelectric Single Crystal through Raman Spectroscopy