%A Chenqiang Hua, Hua Bai, Yi Zheng, Zhu-An Xu, Shengyuan A. Yang, Yunhao Lu, and Su-Huai Wei %T Strong Coupled Magnetic and Electric Ordering in Monolayer of Metal Thio(seleno)phosphates %0 Journal Article %D 2021 %J Chin. Phys. Lett. %R 10.1088/0256-307X/38/7/077501 %P 077501%V 38 %N 7 %U {https://cpl.iphy.ac.cn/CN/abstract/article_105948.shtml} %8 2021-06-04 %X The coupling between electric ordering and magnetic ordering in two-dimensional (2D) materials is important for both fundamental research of 2D multiferroics and future development of magnetism-based information storage and operation. Here, we introduce a scheme for realizing a magnetic phase transition through the transition of electric ordering. We take CuMoP$_{2}$S$_{6}$ monolayer as an example, which is a member of the large 2D transition-metal chalcogen-phosphates family. Based on first-principles calculations, we find that it is a multiferroic with unprecedented characters, namely, it exhibits two different phases: an antiferroelectric-antiferromagnetic phase and a ferroelectric-ferromagnetic phase, in which the electric and magnetic orderings are strongly coupled. Importantly, the electric polarization is out-of-plane, so the magnetism can be readily switched by using the gate electric field. Our finding reveals a series of 2D multiferroics with special magnetoelectric coupling, which hold great promise for experimental realization and practical applications.