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Nonresonant Optical Nonlinearities of Surface Chemically Modified ZnO Composite Nanoparticles |
WANG Rong-yao;WU Xiao-chun;ZOU Bing-suo;WANG Li;WU Peng-fei;LIU Shao-mei;WANG Jin-guo;XU Ji-ren |
Optical Physics Laboratory, Institute of Physics, Chinese Academy of Sciences, Beijing 100080 |
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Cite this article: |
WANG Rong-yao, WU Xiao-chun, ZOU Bing-suo et al 1998 Chin. Phys. Lett. 15 27-29 |
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Abstract With surface chemical modification, we have obtained core-shell structure ZnO nanoparticles. The nonresonant third-order nonlinear optical refraction of this new composite material was found to be -3.8 x 10-l0 esu by Z-scan measurements with a femtosecond pulsed laser. The ultrafast nonlinear response time ~250 fs measured by time-resolved pump-probe techniques suggests that the nonlinearity of this new material originates mainly from a rapid electronic polarization process or virtual process such as the optical Stark effect.
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Keywords:
42.65.An
42.70.Nq
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Published: 01 January 1998
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PACS: |
42.65.An
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(Optical susceptibility, hyperpolarizability)
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42.70.Nq
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(Other nonlinear optical materials; photorefractive and semiconductor materials)
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