| CONDENSED MATTER: STRUCTURE, MECHANICAL AND THERMAL PROPERTIES |
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Improvement of Cyclic Stability of Na$_{0.67}$Mn$_{0.8}$Ni$_{0.1}$Co$_{0.1}$O$_{2}$ via Suppressing Lattice Variation |
| Zhongmin Ren1, Muqin Wang1,3*, Shuaishuai Chen2, Lei Ding2, Hua Li1, Jian Liu1, Jieyun Zheng4*, Zhihong Liu1, Deyu Wang1,2*, and Mingkui Wang3 |
1Key Laboratory of Optoelectronic Chemical Materials and Devices, School of Chemical and Environmental Engineering, Jianghan University, Wuhan 430056, China
2Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China
3Wuhan National Laboratory for Optoelectronics, Huazhong University of Science & Technology, Wuhan 430074, China
4Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China
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| Cite this article: |
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Zhongmin Ren, Muqin Wang, Shuaishuai Chen et al 2021 Chin. Phys. Lett. 38 076102 |
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Abstract Strategies to prolong operational life are highly pursued to strengthen the advantage of cost-effectiveness on sodium-ion batteries (SIBs). We demonstrate the crucial influence of particles' internal mechanical strains on durability of cathode, which does not attract enough attentions from the community. Among the investigated samples, 2% Ti-modified-Na$_{0.67}$Ni$_{0.1}$Co$_{0.1}$Mn$_{0.8}$O$_{2}$ suppresses the $c$-axis lattice variation by 38%, attains the reversible capacity 86% higher after 200 cycles, and still keeps intact morphology. This approach indicates that the mechanical properties could tailor cyclic stability of cathode, which is particular important to further improve competitiveness for SIBs.
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Received: 08 March 2021
Published: 05 July 2021
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| PACS: |
61.05.-a
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(Techniques for structure determination)
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61.05.C-
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(X-ray diffraction and scattering)
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62.20.mt
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(Cracks)
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62.20.-x
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(Mechanical properties of solids)
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| Fund: Supported by the China Postdoctoral Science Foundation (Grant No. 2020M682391), Beijing Municipal Science and Technology Commission (Grant No. Z191100004719001), the Start-Up Funding of Jianghan University, and the “Chutian Scholar Program” of Hubei Province. |
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