Effect of Terraces at the Interface on the Structural and Physical Properties of La$_{0.8}$Sr$_{0.2}$MnO$_{3}$ Thin Films
Ya-Qing Feng1 , Kui-Juan Jin1,2** , Chen Ge1 , Xu He1 , Lin Gu1 , Zhen-Zhong Yang1 , Hai-Zhong Guo1 , Qian Wan1 , Meng He1 , Hui-Bin Lu1 , Guo-Zhen Yang1,2
1 Institute of Physics, Chinese Academy of Sciences, Beijing 1001902 Collaborative Innovation Center of Quantum Matter, Beijing 100190
Abstract :Employing atomic force microscopy, transmission electron microscopy and the second harmonic generation technique, we carefully explore the structural properties of 6-unit-cell-thick La$_{0.8}$Sr$_{0.2}$MnO$_{3}$ films grown on SrTiO$_{3}$ with atomically flat TiO$_{2}$-terminated terraces on the surface. The results clearly demonstrate that the terraces on the surface of TiO$_{2}$-terminated SrTiO$_{3}$ can improve the layer-by-layer epitaxial growth of the manganite films, which results in uniform film coverage at the beginning of growth and thus reduces the substrate-induced disorder at or near the interface. Comparing the magnetic and transport properties of La$_{0.8}$Sr$_{0.2}$MnO$_{3}$ films with the thicknesses varying from 6 unit cells to 80 unit cells grown respectively on as-received SrTiO$_{3}$ and TiO$_{2}$-terminated SrTiO$_{3}$, it is found that these atomically flat terraces on the surface of TiO$_{2}$-terminated SrTiO$_{3}$ can greatly enhance the Curie temperature and conductivities of the ultrathin La$_{0.8}$Sr$_{0.2}$MnO$_{3}$ films with thickness less than 50 unit cells, while no obvious difference is detected in the magnetic and transport properties of the 80 unit-cell thick films.
收稿日期: 2016-03-21
出版日期: 2016-08-01
:
68.35.Ct
(Interface structure and roughness)
75.75.-c
(Magnetic properties of nanostructures)
73.63.-b
(Electronic transport in nanoscale materials and structures)
68.37.Lp
(Transmission electron microscopy (TEM))
引用本文:
. [J]. 中国物理快报, 2016, 33(07): 76801-076801.
Ya-Qing Feng, Kui-Juan Jin, Chen Ge, Xu He, Lin Gu, Zhen-Zhong Yang, Hai-Zhong Guo, Qian Wan, Meng He, Hui-Bin Lu, Guo-Zhen Yang. Effect of Terraces at the Interface on the Structural and Physical Properties of La$_{0.8}$Sr$_{0.2}$MnO$_{3}$ Thin Films. Chin. Phys. Lett., 2016, 33(07): 76801-076801.
链接本文:
https://cpl.iphy.ac.cn/CN/10.1088/0256-307X/33/7/076801
或
https://cpl.iphy.ac.cn/CN/Y2016/V33/I07/76801
[1] Jiang Q D and Zegenhagen J 1995 Surf. Sci. 338 L882 [2] Silly F and Castell M R 2005 Appl. Phys. Lett. 87 213107 [3] Wang X, Fei Y Y, Lu H B, Jin K J, Zhu X D, Chen Z H, Zhou Y L and Yang G Z 2005 Sci. Chin. Ser. G 48 459 [4] Bibes M, Valencia S, Balcells L, Martínez B, Fontcuberta J, Wojcik M, Nadolski S and Jedryka E 2002 Phys. Rev. B 66 134416 [5] Seo S S A, Choi W S, Lee H N, Yu L, Kim K W, Bernhard C and Noh T W 2007 Phys. Rev. Lett. 99 266801 [6] Kim J S, Seo S S A, Chisholm M F, Kremer R K, Habermeier H U, Keimer B and Lee H N 2010 Phys. Rev. B 82 201407 [7] Ohtomo A and Hwang H Y 2004 Nature 427 423 [8] Dikin D A, Mehta M, Bark C W, Folkman C M, Eom C B and Chandrasekhar V 2011 Phys. Rev. Lett. 107 056802 [9] Ohtomo A, Muller D A, Grazul J L and Hwang H Y 2002 Nature 419 378 [10] Biscaras J, Bergeal N, Kushwaha A, Wolf T, Rastogi A, Budhani R C and Lesueur J 2010 Nat. Commun. 1 89 [11] Wang M, Ou Y B, Li F S, Zhang W H, Tang C J, Wang L L, Xue Q K and Ma X C 2014 Acta Phys. Sin. 63 027401 [12] Padhan P, Pandey N K, Srivastava S, Rakshit R K, Kulkarni V N and Budhani R C 2000 Solid State Commun. 117 27 [13] Zhao R Q, Jin K J, Guo H Z, Lu H B and Yang G Z 2013 Sci. Chin. Phys. Mech. Astron. 56 2370 [14] Fontcuberta J, Skumryev V, Laukhin V, Granados X and Salje E K H 2015 Sci. Rep. 5 13784 [15] Salje E K H, Aktas O, Carpenter M A, Laguta V V and Scott J F 2013 Phys. Rev. Lett. 111 247603 [16] Rondinelli J M, May S J and Freeland J M 2012 MRS Bull. 37 261 [17] Feng Y Q, Jin K J, Gu L, He X, Ge C, Zhang Q H, He M, Guo Q L, Wan Q, He M, Lu H B and Yang G Z 2016 Sci. Rep. 6 22382 [18] Pesquera D, Skumryev V, Sanchez F, Herranz G and Fontcuberta J 2011 Phys. Rev. B 84 184412 [19] Wang C, Jin K J, Gu L, Lu H B, Li S M, Zhou W J, Zhao R Q, Guo H Z, He M and Yang G Z 2013 Appl. Phys. Lett. 102 252401 [20] Urushibara A, Moritomo Y, Arima T, Asamitsu A, Kido G and Tokura Y 1995 Phys. Rev. B 51 14103 [21] Luo Z Y, Tang J, Ma B, Zhang Z Z, Jin Q Y and Wang J P 2012 Chin. Phys. Lett. 29 127501 [22] Ge C, Jin K J, Gu L, Peng L C, Hu Y S, Guo H Z, Shi H F, Li J K, Wang J O, Guo X X, Wang C and He M 2015 Adv. Mater. Interfaces 2 1500407 [23] Moreo A, Mayr M, Feiguin A, Yunoki S and Dagotto E 2000 Phys. Rev. Lett. 84 5568
[1]
. [J]. 中国物理快报, 2019, 36(6): 67301-.
[2]
. [J]. 中国物理快报, 2018, 35(5): 56802-.
[3]
. [J]. 中国物理快报, 2018, 35(4): 46802-.
[4]
. [J]. 中国物理快报, 2017, 34(4): 48201-048201.
[5]
. [J]. 中国物理快报, 2016, 33(12): 126801-126801.
[6]
. [J]. 中国物理快报, 2015, 32(4): 45202-045202.
[7]
. [J]. Chin. Phys. Lett., 2012, 29(12): 127303-127303.
[8]
. [J]. Chin. Phys. Lett., 2012, 29(12): 127501-127501.
[9]
XUE Bai-Qing,CHANG Hu-Dong,SUN Bing,WANG Sheng-Kai,LIU Hong-Gang**. The Impact of HCl Precleaning and Sulfur Passivation on the Al2 O3 /Ge Interface in Ge Metal-Oxide-Semiconductor Capacitors [J]. 中国物理快报, 2012, 29(4): 46801-046801.
[10]
LU Li,CHANG Hu-Dong,SUN Bing,WANG Hong,XUE Bai-Qing,ZHAO Wei,LIU Hong-Gang**. Solid Phase Reactions of Ni-GaAs Alloys for High Mobility III–V MOSFET Applications [J]. 中国物理快报, 2012, 29(4): 46802-046802.
[11]
YU Yang1** , WU Qun1 , WANG Xue-Wei1 , YANG Xiao-Bin2 . Wetting Behavior between Droplets and Dust [J]. 中国物理快报, 2012, 29(2): 26802-026802.
[12]
TAN Ting-Ting**;LIU Zheng-Tang;LI Yan-Yan
. Electrical, Structural and Interfacial Characterization of HfO2 Films on Si Substrates [J]. 中国物理快报, 2011, 28(8): 86803-086803.
[13]
XU Run**;TANG Min-Yan;ZHU Yan-Yan;WANG Lin-Jun
. Epitaxial Growth of Si(111)/Er2 O3 (111) Structure on Si(111) by Molecular Beam Epitaxy [J]. 中国物理快报, 2011, 28(3): 36801-036801.
[14]
MEI Mao-Fei;YU Bo-Ming;LUO Liang;CAI Jian-Chao. A Model for the Contact Angle of Liquid Droplets on Rough Surfaces [J]. 中国物理快报, 2010, 27(7): 76802-076802.
[15]
ZHANG Ning-Yu;TENG Shu-Yun;SONG Hong-Sheng;LIU Gui-Yuan;CHENG Chuan-Fu. Extraction of Parameters of Random Self-Affine Fractal Surfaces from Light Scattered Intensity by Levenberg-Marquardt Algorithm [J]. 中国物理快报, 2009, 26(3): 34209-034209.