Ultrafast Electron Diffraction with Spatiotemporal Resolution of Atomic Motion
LIANG Wen-Xi1, ZHU Peng-Fei1, WANG Xuan2, NIE Shou-Hua2, ZHANG Zhong-Chao3, Clinite Rick2, CAO Jian-Ming2, SHENG Zheng-Ming1,3, ZHANG Jie1,3
1Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 1001902Physics Department and National High Magnetic Field Laboratory, Florida State University, Tallahassee, Florida 32310, USA3Department of Physics, Shanghai Jiao Tong University, Shanghai 200240
Ultrafast Electron Diffraction with Spatiotemporal Resolution of Atomic Motion
LIANG Wen-Xi1, ZHU Peng-Fei1, WANG Xuan2, NIE Shou-Hua2, ZHANG Zhong-Chao3, Clinite Rick2, CAO Jian-Ming2, SHENG Zheng-Ming1,3, ZHANG Jie1,3
1Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 1001902Physics Department and National High Magnetic Field Laboratory, Florida State University, Tallahassee, Florida 32310, USA3Department of Physics, Shanghai Jiao Tong University, Shanghai 200240
摘要Ultrafast electron diffraction (UED) is a rapidly advancing technique capable of recording the atomic-detail structural dynamics in real time. We report the establishment of the first UED system in China. Employing this UED apparatus, both the coherent and the concurrent thermal lattice motions in an aluminium thin-film, trigged by ultrafast laser heating, have been observed. These results demonstrate its ability to directly measure a sub-milli-angstrom lattice spacing change on a sub-picosecond time scale.
Abstract:Ultrafast electron diffraction (UED) is a rapidly advancing technique capable of recording the atomic-detail structural dynamics in real time. We report the establishment of the first UED system in China. Employing this UED apparatus, both the coherent and the concurrent thermal lattice motions in an aluminium thin-film, trigged by ultrafast laser heating, have been observed. These results demonstrate its ability to directly measure a sub-milli-angstrom lattice spacing change on a sub-picosecond time scale.
[1] Sundstr\"{om V 1996 Femtochemistry and Femtobiology:Ultrafast Reaction Dynamics at Atomic-Scale Resolution (River Edge,NJ: World Scientific) [2] Zewail A H 2000 Angew. Chem. Int. Ed. 39 2587 [3] Helliwell J R and Rentzepis P M 1997 Time-ResolvedDiffraction (New York: Oxford University Press) [4] Perman B, \v{Srajer V, Ren Z, Teng T, Pradervand C, UrsbyT, Bourgeois D, Schotte F, Wulff M, Kort R, Hellingwerf K and MoffatK 1998 Science 279 1946 [5] Chin A H, Schoenlein R W, Glover T E, Balling P, Leemans WP and Shank C V 1999 Phys. Rev. Lett. 83 336 [6] Schoenlein R W, Chattopadhyay S, Chong H H W, Glover T E,Heimann P A, Shank C V, Zholents A A and Zolotorev M S 2000 Science 287 2237 [7] Cavalleri A, Toth C, Siders C W, Squier J A, Raksi F,Forget P and Kieffer J C 2001 Phys. Rev. Lett. 8723237401 [8] Mourou G and Williamson S 1982 Appl. Phys. Lett. 41 44 [9] Williamson J C, Cao J, Ihee H, Frey H and Zewail A H 1997 Nature 386 159 [10] Cao J, Hao Z, Park H, Tao C, Kau D and Blaszczyk L 2003 Appl. Phys. Lett. 83 1044 [11] King W E, Campbell G H, Frank A, Reed B, Schmerge J F,Siwick B J, Stuart B C and Weber P M 2005 J. Appl. Phys. 97 111101 [12] Dwyer J R, Hebeisen C T, Ernstorfer R, Harb M,Deyirmenjian V B, Jordan E J and Miller R J D 2006 Phil. Trans.R. Soc. A 364 741 [13] Baum P, Yang D S and Zewail A H 2007 Science 318 788 [14] Hubbell J H and Overbo I 1979 J. Phys. Chem. Ref.Data 8 69 [15] Wang X, Nie S H, Park H, Li J J, Clinite R, Li R K, WangX J and Cao J M 2008 Rev. Sci. Instrum. (to be published) [16] Thomsen C, Strait J, Vardeny Z, Maris H J, Tauc J andHauser J J 1984 Phys. Rev. Lett. 53 989 [17] Kuznetsov A V and Stanton C J, 1994 Phys. Rev.Lett. 73 3243 [18] Lide D R 2002 CRC Handbook of Chemistry and Physics (RocaRaton, FL: Chemical Rubber Company) [19] Rousse A, Rischel C and Gauthier J C 2001 Rev. Mod.Phys. 73 17 [20] Nie S H, Wang X, Li J J, Clinite R and Cao J M 2008 Microscopy Research and Technique (in press) [21] Park H, Wang X, Nie S, Clinite R and Cao J 2005 Solid State Commun. 136 559