Structural Deformation of CO22+ in Intense Femtosecond Laser Fields
ZHANG Sheng1,2, XIA Yuan-Qin1, WANG Yu-Quan1, LU Zhen-Zhong1, CHEN De-Ying1
1National Key Lab of Tunable Laser Technology, Harbin Institute of Technology, Harbin 1500012Department of Physics, Harbin Institute of Technology, Harbin 150001
Structural Deformation of CO22+ in Intense Femtosecond Laser Fields
ZHANG Sheng1,2, XIA Yuan-Qin1, WANG Yu-Quan1, LU Zhen-Zhong1, CHEN De-Ying1
1National Key Lab of Tunable Laser Technology, Harbin Institute of Technology, Harbin 1500012Department of Physics, Harbin Institute of Technology, Harbin 150001
摘要The angular distributions of CO+ from the dissociation of CO22+ and CO2+ in intense femtosecond laser fields (45fs, about 5×1015 W/cm2) are studied at a laser wavelength of 800nm based on the time-of-flight mass spectra of CO+ fragment ions. The experimental results show that structural deformation occurs in the charge state of CO22+ and the CO2+ maintains linear geometrical structure.
Abstract:The angular distributions of CO+ from the dissociation of CO22+ and CO2+ in intense femtosecond laser fields (45fs, about 5×1015 W/cm2) are studied at a laser wavelength of 800nm based on the time-of-flight mass spectra of CO+ fragment ions. The experimental results show that structural deformation occurs in the charge state of CO22+ and the CO2+ maintains linear geometrical structure.
[1] Yamanouchi K 2002 Science 295 1659 [2] Zhuo S M, Chen J X, Yu B Y, Jiang X S, Luo T, Liu Q G,Chen R and Xie S S 2008 J. Biomed. Opt. 13 054024 [3] Chen J X, Zhuo S M, Chen R, Jiang X S, Xie S S and Zou Q L2007 New. J. Phys. 9 212 [4] Posthumus J H 2004 Rep. Prog. Phys. 67 623 [5] Hasegawa H, Hishikawa A and Yamanouchi K 2001 Chem.Phys. Lett. 349 57 [6] Hishikawa A, Iwamae A, Hoshina K, Kono M and Yamanouchi K1998 Chem. Phys. Lett. 282 283 [7] Sanderson J H, El-Zein A, Bryan W A, Newell W R, Langley AJ and Taday P F 1999 Phys. Rev. A 59 2567 [8] Hishikawa A, Iwamae A and Yamanouchi K 1999 Phys.Rev. Lett. 83 1127 [9] Cornaggia C, Schmidt M and Normand D 1994 J. Phys. B 27 L123 [10] Bryan W A, Sanderson J H, El-Zein A, Newell W R, Taday PF and Langley A J 2000 J. Phys. B 33 745 [11] Zhao K, Zhang G and Hill W T 2003 Phys. Rev. A 68 063408 [12] Brichta J P, JWalker S, Helsten R and Sanderson J H 2007 J. Phys. B 40 117 [13] Minemoto S, Kanai T and Sakai H 2008 Phys. Rev. A 77 R041401 [14] Kono H, Koseki S, Shiota M and Fujimura Y 2001 J.Phys. Chem. A 105 5627 [15] Y. Sato, Kono H, Koseki S and Fujimura Y 2003 J. Am.Chem. Soc. 125 8019 [16] Wiley W C and Mclaren I H 1955 Rev. Sci. Instrum. 26 1150 [17] Cornaggia C 1996 Phys. Rev. A 54 R2555 [18] Alnaser A S, Maharjan C M, Tong X M, Ulrich B, RanitovicP, Shan B, Chang Z,. Lin C D, Cocke C L and. Litvinyuk I V 2005 Phys. Rev. A 71 R031403 [19] Voss S, Alnaser A S, Tong X M, Maharjan C M, Ranitovic P,Ulrich B, Shan B, Chang Z and Lin C D 2004 J. Phys. B 374239 [20] Huang J, Wu C Y, Xu N, Liang Q Q, Wu Z F, Yang H and GongQ H 2006 J. Phys. Chem. A 110 10179 [21] Cornaggia C and Hering Ph 2000 Phys. Rev. A 62 023403 [22] Liu J B and Chen W W, Hochlaf M, Qian X M, Chang C and NgC Y 2003 J. Chem. Phys. 118 149 [23] McKenna J, Suresh M, Srigengan B and Williams I D 2006 Phys. Rev. A 74 043409