Surface-Enhanced Third-Order Nonlinear Optical Response of C60 Films on Roughed Glass Plate
LI Shijie1, XU Xiaoping2, LI Wenzhu3, QIU Peihua, WANG Wenyao
1Department of Optics and Electronics, Zhejiang University, Hangzhou 310027
2The Center of Laboratory, Zhejiang University, Hangzhou 310027
3Department of Physics, Zhejiang University, Hangzhou 310027
Shanghai Institute of Optics and Fine Mechanics, Academia Sinica, Shanghai 201800
Surface-Enhanced Third-Order Nonlinear Optical Response of C60 Films on Roughed Glass Plate
LI Shijie1;XU Xiaoping2;LI Wenzhu3;QIU Peihua;WANG Wenyao
1Department of Optics and Electronics, Zhejiang University, Hangzhou 310027
2The Center of Laboratory, Zhejiang University, Hangzhou 310027
3Department of Physics, Zhejiang University, Hangzhou 310027
Shanghai Institute of Optics and Fine Mechanics, Academia Sinica, Shanghai 201800
Abstract： The nonlineat third order optical susceptibility of C60 films on roughed glass plate has been studied by using a mode locked Nd : YAG laser emitting 8ps pulsed at 1.064μm of 0.3 J energy. The large | x ( 3 ) ( - 3ω . ω, ω, ω)I = 2 x10-8 esu for C60 films of 15 μm thickness has been observed, which is 103 larger than the value in the bulk C60. This is due to surface enhanced effect.
1993, Vol. 10 
