A Theoretical Distinction Between Time-Resolved Resonance Raman and Resonance Fluorescence
LU Jing1, DU Si-De2, FAN Kang-Nian1, Lee Soo-Ying3
1Department of Chemistry, 2Department of Physics, Fudan University, Shanghai 200433
3Department of Chemistry, National University of Singapore, Singapore 119260, Singapore
A Theoretical Distinction Between Time-Resolved Resonance Raman and Resonance Fluorescence
LU Jing1;DU Si-De2;FAN Kang-Nian1;Lee Soo-Ying3
1Department of Chemistry, 2Department of Physics, Fudan University, Shanghai 200433
3Department of Chemistry, National University of Singapore, Singapore 119260, Singapore
Abstract： Based on the time-dependent theory, an analysis of the distinction between resonance Raman (RR) and resonance fluorescence (RF) with pulse excitation was presented. The real population of the intermediate state gives two optical components-the independent time evolution of intermediate ket and bra states generates RR while RF originates from the phase coherent between ket and bra states. In cw limit, the transition probability of spontaneous emission with pulse excitation can be reduced to the classical theory.
(Dynamics of nonlinear optical systems; optical instabilities, optical chaos and complexity, and optical spatio-temporal dynamics)
引用本文:
LU Jing;DU Si-De;FAN Kang-Nian;Lee Soo-Ying. A Theoretical Distinction Between Time-Resolved Resonance Raman and Resonance Fluorescence[J]. 中国物理快报, 2000, 17(4): 272-274.
LU Jing, DU Si-De, FAN Kang-Nian, Lee Soo-Ying. A Theoretical Distinction Between Time-Resolved Resonance Raman and Resonance Fluorescence. Chin. Phys. Lett., 2000, 17(4): 272-274.
2000, Vol. 17 
