Intrinsic Electronic Properties of BN-Encapsulated, van der Waals Contacted MoSe$_{2}$ Field-Effect Transistors
Yinjiang Shao1, Jian Zhou1, Ning Xu1, Jian Chen1, Kenji Watanabe2, Takashi Taniguchi2, Yi Shi1, and Songlin Li1*
1School of Electronic Science and Engineering, National Laboratory of Solid-State Microstructures, and Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210023, China 2National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan
Abstract:Two-dimensional (2D) semiconductors have attracted considerable interest for their unique physical properties. Here, we report the intrinsic cryogenic electronic transport properties in few-layer MoSe$_{2}$ field-effect transistors (FETs) that are fully encapsulated in ultraclean hexagonal boron nitride dielectrics and are simultaneously van der Waals contacted with gold electrodes. The FETs exhibit electronically favorable channel/dielectric interfaces with low densities of interfacial traps ($ < $ $10^{10}$ cm$^{-2}$), which lead to outstanding device characteristics at room temperature, including near-Boltzmann-limit subthreshold swings (65 mV/dec), high carrier mobilities (53–68 cm$^{2}\cdot$V$^{-1}\cdot$s$^{-1}$), and negligible scanning hystereses ($ < $ $15$ mV). The dependence of various contact-related parameters with temperature and carrier density is also systematically characterized to understand the van der Waals contacts between gold and MoSe$_{2}$. The results provide insightful information about the device physics in van der Waals contacted and encapsulated 2D FETs.
Paik E Y, Zhang L, Burg G W, Gogna R, Tutuc E, and Deng H 2019 Nature576 80
[4]
Chen D X, Lian Z, Huang X, Su Y, Rashetnia M, Ma L, Yan L, Blei M, Xiang L, Taniguchi T, Watanabe K, Tongay S, Smirnov D, Wang Z, Zhang C, Cui Y T, and Shi S F 2022 Nat. Phys.18 1171
[5]
Ghiotto A, Shih E M, Pereira G S S G, Rhodes D A, Kim B, Zang J, Millis A J, Watanabe K, Taniguchi T, Hone J C, Wang L, Dean C R, and Pasupathy A N 2021 Nature597 345
[6]
Jin C H, Tao Z, Li T X, Xu Y, Tang Y, Zhu J C, Liu S, Watanabe K, Taniguchi T, Hone J C, Fu L, Shan J, and Mak K F 2021 Nat. Mater.20 940
[7]
Zhang Z M, Wang Y M, Watanabe K, Taniguchi T, Ueno K, Tutuc E, and LeRoy B J 2020 Nat. Phys.16 1093
[8]
Desai S B, Madhvapathy S R, Sachid A B, Llinas J P, Wang Q, Ahn G H, Pitner G, Kim M J, Bokor J, Hu C, Wong H S P, and Javey A 2016 Science354 99
[9]
Liu Y, Duan X, Shin H J, Park S, Huang Y, and Duan X 2021 Nature591 43
[10]
Wu F, Tian H, Shen Y, Hou Z, Ren J, Gou G, Sun Y, Yang Y, and Ren T L 2022 Nature603 259
Larentis S, Movva H C P, Fallahazad B, Kim K, Behroozi A, Taniguchi T, Watanabe K, Banerjee S K, and Tutuc E 2018 Phys. Rev. B97 201407
[13]
Tongay S, Zhou J, Ataca C, Lo K, Matthews T S, Li J, Grossman J C, and Wu J 2012 Nano Lett.12 5576
[14]
Zhang Y, Chang T R, Zhou B, Cui Y T, Yan H, Liu Z, Schmitt F, Lee J, Moore R, Chen Y, Lin H, Jeng H T, Mo S K, Hussain Z, Bansil A, and Shen Z X 2014 Nat. Nanotechnol.9 111
[15]
Chamlagain B, Li Q, Ghimire N J, Chuang H J, Perera M M, Tu H, Xu Y, Pan M, Xaio D, Yan J, Mandrus D, and Zhou Z 2014 ACS Nano8 5079
Chang Y H, Zhang W J, Zhu Y H, Han Y, Pu J, Chang J K, Hsu W T, Huang J K, Hsu C L, Chiu M H, Takenobu T, Li H, Wu C I, Chang W H, Wee A T S, and Li L J 2014 ACS Nano8 8582
[18]
Scuri G, Zhou Y, High A A, Wild D S, Shu C, De Greve K, Jauregui L A, Taniguchi T, Watanabe K, Kim P, Lukin M D, and Park H 2018 Phys. Rev. Lett.120 037402
Xu S Q, Wu Z F, Lu H H, Han Y, Long G, Chen X L, Han T, Ye W, Wu Y, Lin J, Shen J, Cai Y, He Y, Zhang F, Lortz R, Cheng C, and Wang N 2016 2D Mater.3 021007
Wang L, Meric I, Huang P Y, Gao Q, Gao Y, Tran H, Taniguchi T, Watanabe K, Campos L M, Muller D A, Guo J, Kim P, Hone J, Shepard K L, and Dean C R 2013 Science342 614
[23]
Tonndorf P, Schmidt R, Böttger P, Zhang X, Börner J, Liebig A, Albrecht M, Kloc C, Gordan O, Zahn D R T, de Vasconcellos S M, and Bratschitsch R 2013 Opt. Express21 4908
[24]
Yin J D, Chen H, Lu W, Liu M L, Li I L, Zhang M, Zhang W, Wang J, Xu Z, Yan P, Liu W, and Ruan S 2017 Nanotechnology28 484001
[25]
Illarionov Y Y, Rzepa G, Waltl M, Knobloch T, Grill A, Furchi M M, Mueller T, and Grasser T 2016 2D Mater.3 035004
[26]
Sze S M and Ng K K 2007 Physics of Semiconductor Devices 3rd edn (New Jersey: John Wiley & Sons)
[27]
Kim S, Konar A, Hwang W S, Lee J H, Lee J, Yang J, Jung C, Kim H, Yoo J B, Choi J Y, Jin Y W, Lee S Y, Jena D, Choi W, and Kim K 2012 Nat. Commun.3 1011
Li S L, Wakabayashi K, Xu Y, Nakaharai S, Komatsu K, Li W W, Lin Y F, Aparecido-Ferreira A, and Tsukagoshi K 2013 Nano Lett.13 3546
[38]
Cui X, Lee G H, Kim Y D, Arefe G, Huang P Y, Lee C H, Chenet D A, Zhang X, Wang L, Ye F, Pizzocchero F, Jessen B S, Watanabe K, Taniguchi T, Muller D A, Low T, Kim P, and Hone J 2015 Nat. Nanotechnol.10 534