Identification of Above-Threshold Ionization by Imaging Photoelectrons from Ammonia Molecules in an Intense Femtosecond Laser Field
Qin Yang1,4 , Jing Leng1,4 , Yan-Hui Wang2 , Ya-Nan Sun1,3 , Hai-Bin Du5 , Dong-Dong Zhang1,4 , Le-Le Song1,6 , Lan-Hai He1,4* , and Fu-Chun Liu1,4*
1 Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China2 College of Electronic Science and Engineering, State Key Laboratory on Integrated Optoelectronics, Jilin University, Changchun 130012, China3 Department of Physics, No. 151 Middle School of Changchun, Changchun 130000, China4 Jilin Provincial Key Laboratory of Applied Atomic and Molecular Spectroscopy, Jilin University, Changchun 130012, China5 Department of Comprehensive, Harbin City Vocational College, Harbin 150000, China6 Jilin Institute of Chemical Technology, Jilin 132022, China
Abstract ：The above-threshold ionization process of ammonia molecules induced by a femtosecond laser field at 800 nm is studied in the intensity range from $1.6 \times 10^{13}$ to $5.7 \times 10^{13}$ W/cm$^{2}$. Channel switching under different laser intensities is observed and identified in the photoelectron kinetic energy spectra of ammonia. Based on the photoelectron kinetic energy distributions and the photoelectron angular distributions, the characteristic peaks observed are exclusively assigned to the multiphoton resonance through certain intermediate states, followed by multiphoton above-threshold ionization.
收稿日期: 2021-12-01
出版日期: 2022-01-29
:
33.80.Wz
(Other multiphoton processes)
33.60.+q
(Photoelectron spectra )
42.50.Hz
(Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift)
33.80.Rv
(Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states))
引用本文:
. [J]. 中国物理快报, 2022, 39(2): 23301-.
链接本文:
https://cpl.iphy.ac.cn/CN/10.1088/0256-307X/39/2/023301
或
https://cpl.iphy.ac.cn/CN/Y2022/V39/I2/23301
[1] Aseyev S A, Ni Y, Frasinski L J, Muller H G, and Vrakking M J J 2003 Phys. Rev. Lett. 91 223902 [2] Tsubouchi M, Whitaker B J, Wang L, Kohguchi H, and Suzuki T 2001 Phys. Rev. Lett. 86 4500 [3] Mauritsson J, Johnsson P, Mansten E, Swoboda M, Ruchon T, L'Huillier A, and Schafer K J 2008 Phys. Rev. Lett. 100 073003 [4] Irimia D, Petsalakis I D, Theodorakopoulos G, and Janssen M H M 2010 J. Phys. Chem. A 114 3157 [5] Lehmann C S, Ram N B, Powis I, and Janssen M H M 2013 J. Phys. Chem. 139 234307 [6] Boll R, Anielski D, Bostedt C, Bozek J D, Christensen L, Coffee R, De S, Decleva P, Epp S W, Erk B, Foucar L, Krasniqi F, Kuepper J, Rouzee A, Rudek B, Rudenko A, Schorb S, Stapelfeldt H, Stener M, Stern S, Techert S, Trippel S, Vrakking M J J, Ullrich J, and Rolles D 2013 Phys. Rev. A 88 061402 [7] Ramasesha K, Leone S R, and Neumark D M 2016 Annu. Rev. Phys. Chem. 67 41 [8] Ahmed M and Kostko O 2020 Phys. Chem. Chem. Phys. 22 2713 [9] Xiong Y, Wilkin K J, and Centurion M 2020 Phys. Rev. Res. 2 043064 [10] Banks H I B, Hadjipittas A, and Emmanouilidou A 2020 J. Phys. B 53 225602 [11] Thoman J W, Chandler D W, Parker D H, and Janssen M 1988 Laser Chem. 9 27 [12] Eppink A T J B and Parker D H 1998 Rev. Sci. Instrum. 68 3477 [13] Wang B, Liu B, Wang Y, and Wang L 2010 Phys. Rev. A 81 043421 [14] Li M, Zhang P, Luo S, Zhou Y, Zhang Q, Lan P, and Lu P 2015 Phys. Rev. A 92 063404 [15] Corkum P B 1993 Phys. Rev. Lett. 71 1994 [16] Vampa G, McDonald C R, Orlando G, Klug D D, Corkum P B, and Brabec T 2014 Phys. Rev. Lett. 113 073901 [17] Shao J, Zhang C P, Jia J C, Ma J L, and Miao X Y 2019 Chin. Phys. Lett. 36 054203 [18] Zhang H, Liu X, Jin F, Zhu M, Yang S, Dong W, Song X, and Yang W 2021 Chin. Phys. Lett. 38 063201 [19] Meckel M, Comtois D, Zeidler D, Staudte A, Pavicic D, Bandulet H C, Pepin H, Kieffer J C, Doerner R, Villeneuve D M, and Corkum P B 2008 Science 320 1478 [20] Blaga C I, Xu J, DiChiara A D, Sistrunk E, Zhang K, Agostini P, Miller T A, DiMauro L F, and Lin C D 2012 Nature 483 194 [21] Bian X B, Huismans Y, Smirnova O, Yuan K J, Vrakking M J J, and Bandrauk A D 2011 Phys. Rev. A 84 043420 [22] Wang S, Zhu Z, Zhang Y, Yan T M, and Jiang Y 2021 Chin. Phys. Lett. 38 013401 [23] van der Zwan E V, Chirila C C, and Lein M 2008 Phys. Rev. A 78 033410 [24] Smeenk C, Arissian L, Staudte A, Villeneuve D M, and Corkum P B 2009 J. Phys. B 42 185402 [25] Holmegaard L, Hansen J L, Kalhoj L, Kragh S L, Stapelfeldt H, Filsinger F, Kuepper J, Meijer G, Dimitrovski D, Abu-samha M, Martiny C P J, and Madsen L B 2010 Nat. Phys. 6 428 [26] Allendorf S W, Leahy D J, Jacobs D C, and Zare R N 1989 J. Chem. Phys. 91 2216 [27] Townsend D and Reid K L 2000 J. Chem. Phys. 112 9783 [28] Stapelfeldt H and Seideman T 2003 Rev. Mod. Phys. 75 543 [29] Yin Y Y, Chen C, Elliott D S et al. 1992 Phys. Rev. Lett. 69 2353 [30] Dong D P, Yang B H, Qian D B, Zhou W C, Zhang S F, and Ma X 2021 Chin. Phys. Lett. 38 083301 [31] Agostini P, Fabre F, Mainfray G, Petite G, and Rahman N K 1979 Phys. Rev. Lett. 42 1127 [32] Agostini P, Kupersztych J, Lompré L, Petite G, and Yergeau A 1987 Phys. Rev. A 36 4111 [33] Bashkansky M, Bucksbaum P H, and Schumacher D W 1988 Phys. Rev. Lett. 60 2458 [34] Kruit P, Kimman J, Muller H G, and van der Wiel M J 1983 Phys. Rev. A 28 248 [35] Freeman R R, Bucks B U P H, Milchberg H, Darack S, Schumacher D, and Geusic M E 1987 Phys. Rev. Lett. 59 1092 [36] Guo D S and Drake G 1992 Phys. Rev. A 45 6622 [37] Nandor M J, Walker M A, and Van Woerkom L D 1998 American Physical Society, DAMOP Meeting , 27–30 May 1998, Santa Fe, New Mexico, p C1.02 [38] Min L, Geng J W, Hong L, Deng Y, Wu C, Peng L Y, Gong Q, and Liu Y 2014 Phys. Rev. Lett. 112 113002 [39] Stephens S L, Walker N R, and Legon A C 2011 Phys. Chem. Chem. Phys. 13 20736 [40] Luo S, Hu W, Yu J, Li X, He L, Wang C, Liu F, and Ding D 2017 J. Phys. Chem. A 121 6547 [41] Suzuki H, Yamamoto S, Ohishi M, Kaifu N, and Takano S 1992 Astrophys. J. 392 551 [42] Cavaliere S, Hannauer J, Demirci U B, Akdim O, and Miele P 2011 Catal. Today 170 3 [43] Queyroux J A, Ninet S, Weck G, Garbarino G, Plisson T, Mezouar M, and Datchi F 2019 Phys. Rev. B 99 134107 [44] Kraus P M and Woerner H J 2013 ChemPhysChem 14 1445 [45] Ashfold M, Dixon R N, and Stickland R J 1984 Chem. Phys. 88 463 [46] Sarka K and Schrötter H W 1996 J. Mol. Spectrosc. 179 195 [47] Song L L, Sun Y N, Wang Y H, Wang X C, He L H, Luo S Z, Hu W H, Tong Q N, Ding D J, and Liu F C 2019 Chin. Phys. B 28 063201 [48] Hui Y, Evans N L, Chatterley A S, Roberts G M, and Ullrich S 2014 J. Phys. Chem. A 118 9438 [49] Foerster J, Plesiat E, Magana A, and Saenz A 2016 Phys. Rev. A 94 043405 [50] Belsa B, Amini K, Liu X, Sanchez A, and Biegert J 2021 Struct. Dyn. 8 014301 [51] Corchado J C, Espinosa-Garcia J, and Yang M 2011 J. Chem. Phys. 135 014303 [52] Sun Y, Wang H, He Z, Qiao B, and Chen X 2021 Phys. Chem. Chem. Phys. 23 4856 [53] Apostolopoulos M I, Taroudakis M I, and Papazoglou D G 2013 Opt. Commun. 296 25 [54] Sun Y N, Wang Y H, Song L L, Du H B, and Liu F C 2020 Chin. Phys. B 29 093201 [55] Tolliver J, Zahedpour S, Wahlstrand J K, Milchberg H M, and Kolesik M 2020 Opt. Lett. 45 5780 [56] Charron E, Sukharev M, and Suzor-Weiner A 2004 Laser Phys. Lett. 1 18 [57] Nolde M, Weitzel K M, and Western C M 2005 Phys. Chem. Chem. Phys. 7 1527 [58] Xie J, Jiang B, Li G, Yang S, Xu J, Sha G, Xu D, Lou N, and Zhang C 2000 Faraday Discuss. 115 127 [59] Vaida V, Mccarthy M I, Engelking P C, Rosmus P, Werner H J, and Botschwina P 1987 J. Chem. Phys. 86 6669 [60] Nieman G C and Colson S D 1979 J. Chem. Phys. 71 571 [61] Glownia J H, Riley S J, Colson S D, and Nieman G C 1980 J. Chem. Phys. 73 4296 [62] Reid K L 2003 Annu. Rev. Phys. Chem. 54 397 [63] Deng Y, Liu Y, Liu X, Liu H, Yang Y, Wu C, and Gong Q 2011 Phys. Rev. A 84 65405 [64] Liu Y, Gerber T, Radi P, Sych Y, and Knopp G 2014 Chem. Phys. Lett. 610 153
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2022, Vol. 39 
