1Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China 2School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100049, China 3Songshan Lake Materials Laboratory, Dongguan 523808, China
Abstract:Distinctive superconducting behaviors between bulk and monolayer FeSe make it challenging to obtain a unified picture of all FeSe-based superconductors. We investigate the ultrafast quasiparticle (QP) dynamics of an intercalated superconductor (Li$_{1-x}$Fe$_{x}$)OHFe$_{1-y}$Se, which is a bulk crystal but shares a similar electronic structure with single-layer FeSe on SrTiO$_{3}$. We obtain the electron-phonon coupling (EPC) constant $\lambda_{{A}_{\rm 1g}}$ ($0.22 \pm 0.04$), which well bridges that of bulk FeSe crystal and single-layer FeSe on SrTiO$_{3}$. Significantly, we find that such a positive correlation between $\lambda_{{A}_{\rm 1g}}$ and superconducting $T_{\rm c}$ holds among all known FeSe-based superconductors, even in line with reported FeAs-based superconductors. Our observation indicates possible universal role of EPC in the superconductivity of all known categories of iron-based superconductors, which is a critical step towards achieving a unified superconducting mechanism for all iron-based superconductors.
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