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Universal Scaling Law for Atomic Diffusion and Viscosity in Liquid Metals |
| LI Guang-Xu;LIU Chang-Song;ZHU Zhen-Gang |
| Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences,PO BOX 1129, Hefei 230031 |
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LI Guang-Xu, LIU Chang-Song, ZHU Zhen-Gang 2004 Chin. Phys. Lett. 21 2489-2492 |
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Abstract The recently proposed scaling law relating the diffusion coefficient and the excess entropy of liquid [Samanta A et al. 2004 Phys. Rev. Lett. 92 145901; Dzugutov M 1996 Nature 381 137], and a quasi-universal relationship between the transport coefficients and excess entropy of dense fluids [Rosenfeld Y 1977 it Phys. Rev. A 15 2545], are tested for diverse liquid metals using molecular dynamics simulations. Interatomic potentials derived from the glue potential and second-moment approximation of tight-binding scheme are used to study liquid metals. Our simulation results give sound support to the above-mentioned universal scaling laws. Following Dzugutov, we have also reached a new universal scaling relationship between the viscosity coefficient and excess entropy. The simulation results suggest that the reduced transport coefficients can be expressed approximately in terms of the corresponding packing density.
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66.10.Cb
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Published: 01 December 2004
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