Chin. Phys. Lett.  2003, Vol. 20 Issue (4): 489-492    DOI:
Original Articles |
Density Distributions of H and H2 in Pulsed Microwave Hydrogen Plasmas
DUAN Xu-Ru1;H. Lange2;QIAN Shang-Jie1;N. Lang2
1Southwestern Institute of Physics, PO Box 432, Chengdu 610041 2Institute of Low Temperature Plasma Physics, Greifswald 17489, Germany
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DUAN Xu-Ru, H. Lange, QIAN Shang-Jie et al  2003 Chin. Phys. Lett. 20 489-492
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Abstract Temporal distribution of the H atom and H2 densities in a pulsed microwave hydrogen plasmas has been measured simultaneously by two-photon absorption laser-induced fluorescence (TALIF). The measurement of the H-atom absolute density obtained by NO2 titration in a flow tube reactor shows that the density of H2 could be determined by the measured effective lifetime of the TALIF signal via the quenching equation. The H-atom density of about 1.5 x 1015cm-3 in both pulsed and stationary phases does not obviously change. It is found that the gas temperature volume effect plays an important role in governing the distributions of the H-atom density and it is mole fraction. The calculated gas temperature is in good consistent with the rotational temperature of H2 measured by optical emission spectroscopy in pulsed phase.


Keywords: 52.70.-m      52.20.-j      31.70.Hq      32.50.+d      33.50.Dq     
Published: 01 April 2003
PACS:  52.70.-m (Plasma diagnostic techniques and instrumentation)  
  52.20.-j (Elementary processes in plasmas)  
  31.70.Hq (Time-dependent phenomena: excitation and relaxation processes, and reaction rates)  
  32.50.+d (Fluorescence, phosphorescence (including quenching))  
  33.50.Dq (Fluorescence and phosphorescence spectra)  
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https://cpl.iphy.ac.cn/       OR      https://cpl.iphy.ac.cn/Y2003/V20/I4/0489
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