Chin. Phys. Lett.  2001, Vol. 18 Issue (12): 1598-1600    DOI:
Original Articles |
Large Third-Order Nonlinear Optical Susceptibility of Rh-Doped BaTiO3 Thin Films Prepared by Pulsed Laser Deposition
YANG Guang;WANG Huan-Hua;TAN Guo-Tai;JIANG An-Quan;ZHOU Yue-Liang;YANG Guo-Zhen;CHEN Zheng-Hao
Laboratory of Optical Physics, Institute of Physics and Center for Condensed Matter Physics, Chinese Academy of Sciences, P. O. Box 603, Beijing 100080
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YANG Guang, WANG Huan-Hua, TAN Guo-Tai et al  2001 Chin. Phys. Lett. 18 1598-1600
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Abstract Rh-doped barium titanate (BaTiO3) epitaxial thin films have been fabricated on SrTiO3 (100) substrates by pulsed laser deposition. The nonlinear optical properties of the films were determined using z-scan method at a wavelength of 532nm with a laser duration of 10ns. The real and imaginary parts of the third-order nonlinear susceptibility x(3) were 5.71 x 10-7 esu and 9.59 x 10-8 esu, respectively. The real part value of x(3) of the Rh:BaTiO3 films is about one order larger than that of Ce-doped BaTiO3 thin films. The results show that Rh:BaTiO3 thin films have great potential applications for nonlinear optical devices.

Keywords: 42.65.-k      61.10.-i      81.15.Fg      77.84.-s     
Published: 01 December 2001
PACS:  42.65.-k (Nonlinear optics)  
  61.10.-i  
  81.15.Fg (Pulsed laser ablation deposition)  
  77.84.-s (Dielectric, piezoelectric, ferroelectric, and antiferroelectric materials)  
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https://cpl.iphy.ac.cn/       OR      https://cpl.iphy.ac.cn/Y2001/V18/I12/01598
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YANG Guang
WANG Huan-Hua
TAN Guo-Tai
JIANG An-Quan
ZHOU Yue-Liang
YANG Guo-Zhen
CHEN Zheng-Hao
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