Chin. Phys. Lett.  2010, Vol. 27 Issue (8): 083202    DOI: 10.1088/0256-307X/27/8/083202
ATOMIC AND MOLECULAR PHYSICS |
Multiphoton Ionization from Multiple Orbitals of N2 in Strong Laser Fields

WANG Yang1,2, KANG Hui-Peng1,2, QUAN Wei1, ZHANG Xiao-Yin1,2, LIN Zhi-Yang1,2, WU Ming-Yan1,2, LIU Hong-Ping1, LIU Xiao-Jun1

1State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics, Wuhan Institute of Physics and Mathematics, Chinese Academy of Sciences, Wuhan 430071 2Graduate School of Chinese Academy of Sciences, Beijing 100049
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WANG Yang, KANG Hui-Peng, QUAN Wei et al  2010 Chin. Phys. Lett. 27 083202
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Abstract

We investigate multiphoton ionization (MPI) of N2 exposed to femtosecond laser fields at 400 nm and 800 nm experimentally. Photoelectron energy spectra are measured with a high resolution photoelectron spectrometer at laser intensities up to 1014 W/cm2. Prominent resonant peaks observed at 400 nm can be attributed to the resonance with molecular Rydberg states corresponding to different molecular orbitals, revealing the importance of the multiple orbitals contribution in strong field molecular dynamics.

Keywords: 32.80.Rm      42.50.Hz     
Received: 23 March 2010      Published: 28 July 2010
PACS:  32.80.Rm (Multiphoton ionization and excitation to highly excited states)  
  42.50.Hz (Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift)  
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https://cpl.iphy.ac.cn/10.1088/0256-307X/27/8/083202       OR      https://cpl.iphy.ac.cn/Y2010/V27/I8/083202
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WANG Yang
KANG Hui-Peng
QUAN Wei
ZHANG Xiao-Yin
LIN Zhi-Yang
WU Ming-Yan
LIU Hong-Ping
LIU Xiao-Jun
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